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Chin. Phys. B, 2015, Vol. 24(10): 108701    DOI: 10.1088/1674-1056/24/10/108701
INTERDISCIPLINARY PHYSICS AND RELATED AREAS OF SCIENCE AND TECHNOLOGY Prev   Next  

Ultrafast structural dynamics studied by kilohertz time-resolved x-ray diffraction

Guo Xin (郭鑫)a b, Jiang Zhou-Ya (江舟亚)c d, Chen Long (陈龙)c d, Chen Li-Ming (陈黎明)b d, Xin Jian-Guo (辛建国)a, Peter M. Rentzepise, Chen Jie (陈洁)c d
a School of Optoelectronics, Beijing Institute of Technology, Beijing 100081, China;
b Beijing National Laboratory of Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China;
c Key Laboratory for Laser Plasmas (Ministry of Education) and Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China;
d IFSA Collaborative Innovation Center, Shanghai Jiao Tong University, Shanghai 200240, China;
e Electrical & Computer Engineering, Texas A & M University, College Station, TX 77843, USA
Abstract  Ultrashort multi-keV x-ray pulses are generated by electron plasma produced by the irradiation of femtosecond pulses on metals. These sub-picosecond x-ray pulses have extended the field of x-ray spectroscopy into the femtosecond time domain. However, pulse-to-pulse instability and long data acquisition time restrict the application of ultrashort x-ray systems operating at low repetition rates. Here we report on the performance of a femtosecond laser plasma-induced hard x-ray source that operates at 1-kHz repetition rate, and provides a flux of 2.0×1010photons/s of Cu Kα radiation. Using this system for time-resolved x-ray diffraction experiments, we record in real time, the transient processes and structural changes induced by the interaction of 400-nm femtosecond pulse with the surface of a 200-nm thick Au (111) single crystal.
Keywords:  ultrafast x-ray diffraction      transient structures      lattice deformation  
Received:  29 January 2015      Revised:  21 May 2015      Accepted manuscript online: 
PACS:  87.15.ht (Ultrafast dynamics; charge transfer)  
  67.80.de (Structure, lattice dynamics and sound)  
  63.70.+h (Statistical mechanics of lattice vibrations and displacive phase transitions)  
Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 61222509 and 11421064) and the W. M. Keck Foundation.
Corresponding Authors:  Chen Jie     E-mail:  jiec@sjtu.edu.cn

Cite this article: 

Guo Xin (郭鑫), Jiang Zhou-Ya (江舟亚), Chen Long (陈龙), Chen Li-Ming (陈黎明), Xin Jian-Guo (辛建国), Peter M. Rentzepis, Chen Jie (陈洁) Ultrafast structural dynamics studied by kilohertz time-resolved x-ray diffraction 2015 Chin. Phys. B 24 108701

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