中国物理B ›› 2024, Vol. 33 ›› Issue (11): 117301-117301.doi: 10.1088/1674-1056/ad7670

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Nonvolatile ferroelectric control of electronic properties of Bi2Te3

Xusheng Ding(丁旭升), Yunfei Li(李云飞), Chaoyang Kang(康朝阳), Ye-Heng Song(宋业恒)†, and Weifeng Zhang(张伟风)‡   

  1. Henan Key Laboratory of Quantum Materials and Quantum Energy, Center for Topological Functional Materials, School of Future Technology, Henan University, Kaifeng 475004, China
  • 收稿日期:2024-05-08 修回日期:2024-08-31 接受日期:2024-09-03 出版日期:2024-11-15 发布日期:2024-11-15
  • 基金资助:
    Project supported by the National Natural Science Foundation of China (Grant Nos. 12004099 and 11974099), the Zhongyuan Leading Talents, Plan for Leading Talent of Fundamental Research of the Central China in 2020, and the Intelligence Introduction Plan of Henan Province in 2021 (Grant No. CXJD2021008).

Nonvolatile ferroelectric control of electronic properties of Bi2Te3

Xusheng Ding(丁旭升), Yunfei Li(李云飞), Chaoyang Kang(康朝阳), Ye-Heng Song(宋业恒)†, and Weifeng Zhang(张伟风)‡   

  1. Henan Key Laboratory of Quantum Materials and Quantum Energy, Center for Topological Functional Materials, School of Future Technology, Henan University, Kaifeng 475004, China
  • Received:2024-05-08 Revised:2024-08-31 Accepted:2024-09-03 Online:2024-11-15 Published:2024-11-15
  • Contact: Ye-Heng Song, Weifeng Zhang E-mail:yehengsong@henu.edu.cn;wfzhang@henu.edu.cn
  • Supported by:
    Project supported by the National Natural Science Foundation of China (Grant Nos. 12004099 and 11974099), the Zhongyuan Leading Talents, Plan for Leading Talent of Fundamental Research of the Central China in 2020, and the Intelligence Introduction Plan of Henan Province in 2021 (Grant No. CXJD2021008).

摘要: Nonvolatile electric-field control of the unique physical characteristics of topological insulators (TIs) is essential for the fundamental research and development of practical electronic devices. Electrically tunable transport properties through gating materials have been extensively investigated. However, the relatively weak and volatile tunability limits its practical applications in spintronics. Here, we demonstrate the nonvolatile electric-field control of Bi$_{2}$Te$_{3}$ transport properties via constructing ferroelectric Rashba architectures, i.e., 2D Bi$_{2}$Te$_{3}/\alpha $-In$_{2}$Se$_{3}$ ferroelectric field-effect transistors. By switching the polarization states of $\alpha $-In$_{2}$Se$_{3}$, the Fermi level, resistance, Fermi wave vector, carrier mobility, carrier density and magnetoresistance (MR) of the Bi$_{2}$Te$_{3}$ film can be effectively modulated. Importantly, a shift of the Fermi level towards a band gap with a surface state occurs as switching to a negative polarization state, the contribution of the surface state to the conductivity then increases, thereby increasing the carrier mobility and electron coherence length significantly, resulting in the enhanced weak anti-localization (WAL) effect. These results provide a nonvolatile electric-field control method to tune the electronic properties of TI and can further extend to quantum transport properties.

关键词: topological insulator, weak anti-localization effect, $\alpha $-In$_{2}$Se$_{3}$, electrical transport characteristics

Abstract: Nonvolatile electric-field control of the unique physical characteristics of topological insulators (TIs) is essential for the fundamental research and development of practical electronic devices. Electrically tunable transport properties through gating materials have been extensively investigated. However, the relatively weak and volatile tunability limits its practical applications in spintronics. Here, we demonstrate the nonvolatile electric-field control of Bi$_{2}$Te$_{3}$ transport properties via constructing ferroelectric Rashba architectures, i.e., 2D Bi$_{2}$Te$_{3}/\alpha $-In$_{2}$Se$_{3}$ ferroelectric field-effect transistors. By switching the polarization states of $\alpha $-In$_{2}$Se$_{3}$, the Fermi level, resistance, Fermi wave vector, carrier mobility, carrier density and magnetoresistance (MR) of the Bi$_{2}$Te$_{3}$ film can be effectively modulated. Importantly, a shift of the Fermi level towards a band gap with a surface state occurs as switching to a negative polarization state, the contribution of the surface state to the conductivity then increases, thereby increasing the carrier mobility and electron coherence length significantly, resulting in the enhanced weak anti-localization (WAL) effect. These results provide a nonvolatile electric-field control method to tune the electronic properties of TI and can further extend to quantum transport properties.

Key words: topological insulator, weak anti-localization effect, $\alpha $-In$_{2}$Se$_{3}$, electrical transport characteristics

中图分类号:  (Electronic transport phenomena in thin films)

  • 73.50.-h
77.84.-s (Dielectric, piezoelectric, ferroelectric, and antiferroelectric materials) 81.15.Hi (Molecular, atomic, ion, and chemical beam epitaxy) 72.15.Rn (Localization effects (Anderson or weak localization))