Nonlinear optical properties of 75TeO2－20Nb2O5－5ZnO glasses doped with CeO2

doi:10.1088/1009-1963/13/8/018

中国物理B ›› 2004, Vol. 13 ›› Issue (8): 1287-1290.doi: 10.1088/1009-1963/13/8/018

Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂

林健¹, 黄文旵¹, 张诗按², 孙真荣², 王宇飞², 曾和平², 王祖赓², 徐至展³, 李儒新³

(1)Department of Materials Science and Engineering, Tongji University, Shanghai 200092, China; (2)Key Laboratory of Optical and Magnetic Resonance Spectroscopy, and Department of Physics, East China Normal University, Shanghai 200062, China; (3)Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

收稿日期:2003-10-08 修回日期:2004-03-30 出版日期:2004-06-21 发布日期:2005-06-22
基金资助:
Project supported by the Shanghai Priority Academic Discipline, the National Natural Science Foundation of China (Grant No 10234030 and 10074015), and the State Key Development Programme for Basic Research of China (Grant No 1999075204), the Programme Fou

Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂

Zhang Shi-An (张诗按)^a, Sun Zhen-Rong (孙真荣)^a, Wang Yu-Fei (王宇飞)^a, Zeng He-Ping (曾和平)^a, Wang Zu-Geng (王祖赓)^b, Lin Jian (林健)^b, Huang Wen-Hai (黄文旵)^b, Xu Zhi-Zhan (徐至展)^c, Li Ru-Xin (李儒新)^c

^a Key Laboratory of Optical and Magnetic Resonance Spectroscopy, and Department of Physics, East China Normal University, Shanghai 200062, China; ^b Department of Materials Science and Engineering, Tongji University, Shanghai 200092, China; ^c Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

Received:2003-10-08 Revised:2004-03-30 Online:2004-06-21 Published:2005-06-22
Supported by:
Project supported by the Shanghai Priority Academic Discipline, the National Natural Science Foundation of China (Grant No 10234030 and 10074015), and the State Key Development Programme for Basic Research of China (Grant No 1999075204), the Programme Fou

摘要/Abstract

摘要： Nonlinear optical properties of 75TeO_2－20Nb_2O_5－5ZnO glasses doped with CeO_2 have been investigated with a self-diffracted time-resolved degenerate four-wave mixing (DFWM) technique at different excitation intensities and lattice temperatures. The DFWM signal exhibits three peaks at higher excitation intensities, where a main peak appears at zero delay time and two rather weak side peaks are located symmetrically at the negative and positive time delay. Due to destructive interferences between the fifth- and third-order polarizations, the line-shape of the main peak around the zero time delay evolves from single peak into a double-peak structure with increasing excitation intensity. Two side peaks emerge at the positive and negative time delay and gradually intensify with increasing excitation intensity or lattice temperature, and their positions are independent of the pulse duration, temperature and excitation intensity, which are attributed to the many-body Coulomb interaction.

关键词: tellurite glasses, CeO_2, degenerate four-wave mixing (DFWM), local-field corrections, many-body Coulomb interaction

Abstract: Nonlinear optical properties of 75TeO$_2$－20Nb$_2$O$_5$－5ZnO glasses doped with CeO$_2$ have been investigated with a self-diffracted time-resolved degenerate four-wave mixing (DFWM) technique at different excitation intensities and lattice temperatures. The DFWM signal exhibits three peaks at higher excitation intensities, where a main peak appears at zero delay time and two rather weak side peaks are located symmetrically at the negative and positive time delay. Due to destructive interferences between the fifth- and third-order polarizations, the line-shape of the main peak around the zero time delay evolves from single peak into a double-peak structure with increasing excitation intensity. Two side peaks emerge at the positive and negative time delay and gradually intensify with increasing excitation intensity or lattice temperature, and their positions are independent of the pulse duration, temperature and excitation intensity, which are attributed to the many-body Coulomb interaction.

Key words: tellurite glasses, CeO₂, degenerate four-wave mixing (DFWM), local-field corrections, many-body Coulomb interaction

中图分类号: (Glasses, quartz)

42.70.Ce

42.65.Hw (Phase conjugation; photorefractive and Kerr effects) 78.66.Jg (Amorphous semiconductors; glasses)

张诗按, 孙真荣, 王宇飞, 曾和平, 王祖赓, 林健, 黄文旵, 徐至展, 李儒新. Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂[J]. 中国物理B, 2004, 13(8): 1287-1290.

Zhang Shi-An (张诗按), Sun Zhen-Rong (孙真荣), Wang Yu-Fei (王宇飞), Zeng He-Ping (曾和平), Wang Zu-Geng (王祖赓), Lin Jian (林健), Huang Wen-Hai (黄文旵), Xu Zhi-Zhan (徐至展), Li Ru-Xin (李儒新). Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂[J]. Chinese Physics, 2004, 13(8): 1287-1290.

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Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂

Nonlinear optical properties of 75TeO₂－20Nb₂O₅－5ZnO glasses doped with CeO₂

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