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ARPES study of Y2O2Bi single crystals: Intrinsic electronic structure of Bi square nets
Yun-Bo Wu(吴云波), Tong-Rui Li(李彤瑞), Zhi-Peng Cao(曹志鹏), Zhan-Feng Liu(刘站锋), Yu-Liang Li(李昱良), Zheng-Ming Shang(尚政明), Xin Zheng(郑新), Hui Tian(田慧), Zong-Yi Wang(王宗一), Yu-Tong Bi(毕雨桐), Hao-Yang Zhou(周浩洋), Yi Liu(刘毅), Guo-Bin Zhang(张国斌), Zheng-Tai Liu(刘正太), Da-Wei Shen(沈大伟), Li-Dong Zhang(张李东), Sheng-Tao Cui(崔胜涛), and Zhe Sun(孙喆)
2026 (4):
47101-047101.
doi: 10.1088/1674-1056/ae04d9
摘要
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The Bi square net, a structural motif in a diverse array of layered compounds, has emerged as a desirable system for investigating the interplay between strong spin—orbit coupling, reduced dimensionality, and magnetism. We present a comprehensive study of Y2O2Bi single crystals using high-resolution angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations to elucidate the intrinsic electronic structure of the Bi square net. Our findings reveal a pronounced two-dimensional character of the electronic states, with the Bi square net dominating the low-energy electronic structure. While Y2O2Bi itself exhibits no topological features, DFT calculations on related Bi square net compounds reveal that the surrounding crystal environment can induce non-trivial topology, as exemplified by the topological insulator LiBi. This comparative study establishes a crucial benchmark for understanding Bi square net physics and informs the design of future Bi square net-based quantum materials.
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