Effect of electrical discharge in water on concentration of nitrate solution

doi:10.1088/1674-1056/26/2/025101

中国物理B ›› 2017, Vol. 26 ›› Issue (2): 25101-025101.doi: 10.1088/1674-1056/26/2/025101

• PHYSICS OF GASES, PLASMAS, AND ELECTRIC DISCHARGES • 上一篇下一篇

Effect of electrical discharge in water on concentration of nitrate solution

F Sohbatzadeh, H Bagheri, R Safari

Department of Atomic and Molecular Physics, Faculty of Basic Sciences, University of Mazandaran, Babolsar, Iran

收稿日期:2016-09-04 修回日期:2016-10-12 出版日期:2017-02-05 发布日期:2017-02-05
通讯作者: F Sohbatzadeh E-mail:F.sohbat@umz.ac.ir

Effect of electrical discharge in water on concentration of nitrate solution

F Sohbatzadeh, H Bagheri, R Safari

Department of Atomic and Molecular Physics, Faculty of Basic Sciences, University of Mazandaran, Babolsar, Iran

Received:2016-09-04 Revised:2016-10-12 Online:2017-02-05 Published:2017-02-05
Contact: F Sohbatzadeh E-mail:F.sohbat@umz.ac.ir

摘要/Abstract

摘要： In this work, the effect of electrical discharge on nitrate concentration is considered in aqueous solution. The atmospheric pressure plasma was produced by a high-voltage power supply at 27 kHz using pin-to-pin configuration. Air, argon, and argon/methane mixture were used to study the working gas effect. UV-VIS spectroscopy and ion chromatography were used to analyze the effect of the electrical discharge on nitrate concentration in deionized water. Optical emission spectroscopy (OES) was applied to diagnose active species inside and on the surface of the deionized water solution. The results of the present work showed that the atmospheric pressure electric discharge with air increases nitrate concentration while it remains constant using argon and argon/methane electrical discharges. It was also revealed that in the presence of air, the electrical discharge reduces pH, acidifying the solution and increasing solution conductivity due to production of extra nitrate ions. On the other hand, argon electrical discharge increases pH and conductivity due to production of OH^- ion in water.

关键词: electric discharge, nitrate solution, optical spectroscopy

Abstract: In this work, the effect of electrical discharge on nitrate concentration is considered in aqueous solution. The atmospheric pressure plasma was produced by a high-voltage power supply at 27 kHz using pin-to-pin configuration. Air, argon, and argon/methane mixture were used to study the working gas effect. UV-VIS spectroscopy and ion chromatography were used to analyze the effect of the electrical discharge on nitrate concentration in deionized water. Optical emission spectroscopy (OES) was applied to diagnose active species inside and on the surface of the deionized water solution. The results of the present work showed that the atmospheric pressure electric discharge with air increases nitrate concentration while it remains constant using argon and argon/methane electrical discharges. It was also revealed that in the presence of air, the electrical discharge reduces pH, acidifying the solution and increasing solution conductivity due to production of extra nitrate ions. On the other hand, argon electrical discharge increases pH and conductivity due to production of OH^- ion in water.

Key words: electric discharge, nitrate solution, optical spectroscopy

中图分类号: (Electrical properties)

51.50.+v

52.25.-b (Plasma properties) 52.80.Hc (Glow; corona) 52.90.+z (Other topics in physics of plasmas and electric discharges)

F Sohbatzadeh, H Bagheri, R Safari. Effect of electrical discharge in water on concentration of nitrate solution[J]. 中国物理B, 2017, 26(2): 25101-025101.

F Sohbatzadeh, H Bagheri, R Safari. Effect of electrical discharge in water on concentration of nitrate solution[J]. Chin. Phys. B, 2017, 26(2): 25101-025101.

参考文献 32

[1]	Bárdos L, Baránková H 2010 Thin Solid Films 518 6705
[2]	Kolb J F, Mohamed A A H, Price R O, Swanson R J, Bowman A, Chiavarini, R L, Stacey M and Schoenbach K H 2008 Appl. Phys. Lett. 92 241501
[3]	Akitsu T, Ohkawa H, Tsuji M, Kimura H and Kogoma M 2005 Surf. Coatings Technol. 193 29
[4]	Tendero C, Tixier C, Tristant P, Desmaison J and Leprince P 2006 Spectrochimica Acta Part B: Atomic Spectroscopy 61 2
[5]	Lloyd G, Friedman G, Jafri S, Schultz G, Fridman A and Harding K 2010 Plasma Processes and Polymers 7 194
[6]	Moreau M, Orange N and Feuilloley M G J Biotechnology Vdvances 26 610
[7]	Ehlbeck J, Schnabel U, Polak M, Winter J, Von Woedtke T, Brandenburg R, Von dem Hagen T and Weltmann K D 2011 J. Phys. D: Appl. Phys. 44 013002
[8]	Sohbatzadeh F, Mirzanejhad S, Ghasemi M and Talebzadeh M 2013 J. Electrostatics 71 875
[9]	Ghasemi M, Sohbatzadeh F and Mirzanejhad S 2015 J. Theor. Appl. Phys. 9 177
[10]	Rumbach P, Witzke M, Sankaran R M and Go D B 2013 J. Am. Chem. Soc. 135 16264
[11]	Shainsky N, Dobrynin D, Ercan U, Joshi S G, Ji H, Brooks A and Friedman G 2012 Plasma Processes and Polymers 9(6)
[12]	Bruggeman P and Leys C 2009 J. Phys. D: Appl. Phys. 42 053001
[13]	Bruggeman P, Van Slycken J, Degroote J, Vierendeels J, Verleysen P and Leys C 2008 IEEE Trans. Plasma Sci. 36 1138
[14]	Vanraes P, Nikiforov A and Leys C 2012 J. Phys. D: Appl. Phys. 45 245206
[15]	Jiang B, Zheng J, Qiu S, Wu M, Zhang Q, Yan Z and Xue Q 2014 Chem. Eng. J. 236 348
[16]	Zhang J, Zheng Z, Zhang Y, Feng J and Li J 2008 J. Hazardous Mater. 154 506
[17]	Piroi D, Magureanu M, Mandache N B and Parvulescu V I 2009 19th International Symposium on Plasma Chemistry, Bochum, Germany
[18]	Gershman S, Mozgina O, Belkind A, Becker K and Kunhardt E 2007 Contributions to Plasma Physics 47 19
[19]	Magureanu M, Piroi D, Mandache N B, David V, Medvedovici A, Bradu C and Parvulescu V I 2011 Water Research 45 3407
[20]	Mozgina O, Gershman S, Belkind A, Becker K and Christodoulatos C 2005 in Plasma Science, 2005. ICOPS'05. IEEE Conference Record-Abstracts. IEEE International Conference, p. 320
[21]	http://www.hach.com, United States, Hach Company, P. O. Box 389, Loveland, Colorado, 80539-0389
[22]	Raizer Y P and Allen J E 1997 Gas discharge physics (Berlin: Springer)
[23]	Bashir M, Rees J M, Bashir S and Zimmerman W B 2014 Phys. Lett. A 8 2395
[24]	Laroussi M and Leipold F 2004 International Journal of Mass Spectrometry 233 81
[25]	Burlica R, Kirkpatrick M J and Locke B R 2006 Journal of Electrostatics 64 35
[26]	Akiyama H 2000 IEEE Transactions on Dielectrics and Electrical Insulation 7 646
[27]	Miichi T, Ihara S, Satoh S and Yamabe C 2000 Vacuum 59 236
[28]	Atkinson R, Baulch D L, Cox R A, Hampson R F Jr, Kerr J A, Rossi M J and Troe J 2004 Atmospheric Chemistry and Physics 4 1461
[29]	Lee B H, Nazarenko O B and Shubin B G 2005 Nat. Sci. 216
[30]	Parvulescu V I, Magureanu M and Lukes P 2012 Plasma Chemistry and Catalysis in Gases and Liquids (John Wiley & Sons)
[31]	Shin W T, Yiacoumi S, Tsouris C and Dai S 2000 Industrial & Engineering Chemistry Research 39 4408
[32]	Zhang J F, BianX C, Chen Q, Liu F P and Liu Z W 2009 Chin. Phys. Lett. 26 035203

Effect of electrical discharge in water on concentration of nitrate solution

Effect of electrical discharge in water on concentration of nitrate solution

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