Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors

doi:10.1088/1674-1056/24/2/028505

中国物理B ›› 2015, Vol. 24 ›› Issue (2): 28505-028505.doi: 10.1088/1674-1056/24/2/028505

• INTERDISCIPLINARY PHYSICS AND RELATED AREAS OF SCIENCE AND TECHNOLOGY • 上一篇下一篇

Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors

吴双红^a, 李文连^b, 陈志^{a c}, 李世彬^a, 王晓晖^a, 魏雄邦^a

a School of Optoelectronic Information and State Key Laboratory of Electronic Thin Films & Integrated Devices, University of Electronic Science and Technology of China (UESTC), Chengdu 610054, China;
b State Key Laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China;
c Department of Electrical & Computer Engineering, University of Kentucky, Lexington, KY 40506, USA

收稿日期:2014-05-15 修回日期:2014-08-26 出版日期:2015-02-05 发布日期:2015-02-05
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos. 61371046, 61405026, 61474016, and 61421002) and China Postdoctoral Science Foundation (Grant No. 2014M552330).

Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors

Wu Shuang-Hong (吴双红)^a, Li Wen-Lian (李文连)^b, Chen Zhi (陈志)^{a c}, Li Shi-Bin (李世彬)^a, Wang Xiao-Hui (王晓晖)^a, Wei Xiong-Bang (魏雄邦)^a

a School of Optoelectronic Information and State Key Laboratory of Electronic Thin Films & Integrated Devices, University of Electronic Science and Technology of China (UESTC), Chengdu 610054, China;
b State Key Laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China;
c Department of Electrical & Computer Engineering, University of Kentucky, Lexington, KY 40506, USA

Received:2014-05-15 Revised:2014-08-26 Online:2015-02-05 Published:2015-02-05
Contact: Wu Shuang-Hong, Chen Zhi E-mail:shwu@uestc.edu.cn;zhichen@engr.uky.edu
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 61371046, 61405026, 61474016, and 61421002) and China Postdoctoral Science Foundation (Grant No. 2014M552330).

摘要/Abstract

摘要： We choose 8-hydroxyquinoline derivative-metal complexes (Beq, Mgq, and Znq) as the acceptors (A) and 4,4',4”-tri-(2-methylphenyl phenylamino) triphenylaine (m-MTDATA) as the donor (D) respectively to study the existing energy transfer process in the organic ultraviolet (UV) photodetector (PD), which has an important influence on the sensitivity of PDs. The energy transfer process from D to A without exciplex formation is discussed, differing from the working mechanism of previous PDs with Gaq [Zisheng Su, Wenlian Li, Bei Chu, Tianle Li, Jianzhuo Zhu, Guang Zhang, Fei Yan, Xiao Li, Yiren Chen and Chun-Sing Lee 2008 Appl. Phys. Lett. 93 103309)] and REq [J. B. Wang, W. L. Li, B. Chu, L. L. Chen, G. Zhang, Z. S. Su, Y. R. Chen, D. F. Yang, J. Z. Zhu, S. H. Wu, F. Yan, H. H. Liu, C. S. Lee 2010 Org. Electron. 11 1301] used as an A material. Under 365-nm UV irradiation with an intensity of 1.2 mW/cm², the m-MTDATA:Beq blend device with a weight ratio of 1:1 shows a response of 192 mA/W with a detectivity of 6.5×10¹¹ Jones, which exceeds those of PDs based on Mgq (146 mA/W) and Znq (182 mA/W) due to better energy level alignment between m-MTDATA/Beq and lower radiative decay. More photophysics processes of the PDs involved are discussed in detail.

关键词: organic photodetector, energy transfer, ultraviolet

Abstract: We choose 8-hydroxyquinoline derivative-metal complexes (Beq, Mgq, and Znq) as the acceptors (A) and 4,4',4”-tri-(2-methylphenyl phenylamino) triphenylaine (m-MTDATA) as the donor (D) respectively to study the existing energy transfer process in the organic ultraviolet (UV) photodetector (PD), which has an important influence on the sensitivity of PDs. The energy transfer process from D to A without exciplex formation is discussed, differing from the working mechanism of previous PDs with Gaq [Zisheng Su, Wenlian Li, Bei Chu, Tianle Li, Jianzhuo Zhu, Guang Zhang, Fei Yan, Xiao Li, Yiren Chen and Chun-Sing Lee 2008 Appl. Phys. Lett. 93 103309)] and REq [J. B. Wang, W. L. Li, B. Chu, L. L. Chen, G. Zhang, Z. S. Su, Y. R. Chen, D. F. Yang, J. Z. Zhu, S. H. Wu, F. Yan, H. H. Liu, C. S. Lee 2010 Org. Electron. 11 1301] used as an A material. Under 365-nm UV irradiation with an intensity of 1.2 mW/cm², the m-MTDATA:Beq blend device with a weight ratio of 1:1 shows a response of 192 mA/W with a detectivity of 6.5×10¹¹ Jones, which exceeds those of PDs based on Mgq (146 mA/W) and Znq (182 mA/W) due to better energy level alignment between m-MTDATA/Beq and lower radiative decay. More photophysics processes of the PDs involved are discussed in detail.

Key words: organic photodetector, energy transfer, ultraviolet

中图分类号: (Photodetectors (including infrared and CCD detectors))

85.60.Gz

95.55.Aq (Charge-coupled devices, image detectors, and IR detector arrays) 42.79.Pw (Imaging detectors and sensors)

吴双红, 李文连, 陈志, 李世彬, 王晓晖, 魏雄邦. Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors[J]. 中国物理B, 2015, 24(2): 28505-028505.

Wu Shuang-Hong (吴双红), Li Wen-Lian (李文连), Chen Zhi (陈志), Li Shi-Bin (李世彬), Wang Xiao-Hui (王晓晖), Wei Xiong-Bang (魏雄邦). Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors[J]. Chin. Phys. B, 2015, 24(2): 28505-028505.

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Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors

Energy transfer ultraviolet photodetector with 8-hydroxyquinoline derivative-metal complexes as acceptors

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