Steady and transient behavior of perylene under high pressure

doi:10.1088/1674-1056/abf923

中国物理B ›› 2021, Vol. 30 ›› Issue (11): 118201-118201.doi: 10.1088/1674-1056/abf923

Steady and transient behavior of perylene under high pressure

Ting-Ting Wang(王亭亭)¹, Yu Zhang(张宇)¹, Hong-Yu Tu(屠宏宇)¹, Lu Han(韩露)¹, Ji-Chao Cheng(程基超)¹, Xin Wang(王鑫)¹, Fang-Fei Li(李芳菲)¹, Ling-Yun Pan(潘凌云)^1,†, and Tian Cui(崔田)^1,2,‡

1 State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, China;
2 School of Physical Science and Technology, Ningbo University, Ningbo 315211, China

收稿日期:2021-02-10 修回日期:2021-03-31 接受日期:2021-04-19 出版日期:2021-10-13 发布日期:2021-11-03
通讯作者: Ling-Yun Pan, Tian Cui E-mail:ply@jlu.edu.cn;cuitian@nbu.edu.cn
基金资助:
Project supported by the National Key Research and Development Program of China (Grant Nos. 2018YFA0305900 and 2017YFA0403704), the National Natural Science Foundation of China (Grant Nos. 61575079, 51632002, 11804113, and 51720105007), the Natural Science Foundation of Jilin Province, China (Grant No. 20180101230JC), and the Program for Changjiang Scholars and Innovative Research Team in University, China (Grant No. IRT_15R23).

Steady and transient behavior of perylene under high pressure

1 State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, China;
2 School of Physical Science and Technology, Ningbo University, Ningbo 315211, China

Received:2021-02-10 Revised:2021-03-31 Accepted:2021-04-19 Online:2021-10-13 Published:2021-11-03
Contact: Ling-Yun Pan, Tian Cui E-mail:ply@jlu.edu.cn;cuitian@nbu.edu.cn
Supported by:
Project supported by the National Key Research and Development Program of China (Grant Nos. 2018YFA0305900 and 2017YFA0403704), the National Natural Science Foundation of China (Grant Nos. 61575079, 51632002, 11804113, and 51720105007), the Natural Science Foundation of Jilin Province, China (Grant No. 20180101230JC), and the Program for Changjiang Scholars and Innovative Research Team in University, China (Grant No. IRT_15R23).

摘要/Abstract

摘要： Pressure can reduce the distances among atoms, thereby modifying the overall optical characteristics of molecules. In this article, the excited state behavior of perylene is carefully observed under isotropic pressure and non-complexing condition. In a steady state, absorption peak shows red shift and spectral width are broadened with pressure increasing, which is ascribed to the π-electron delocalization between molecules. In a transient state, the transition dynamics presents a wavelike tendency with pressure increasing because the shift of self-tapping exciton state is contrary to that of Y-state with pressure increasing. The results conduce to understanding the influence of inter-molecule interaction on excited state behavior with inter-molecule distance decreasing, which contributes to studying the materials under extreme condition.

关键词: perylene, high-pressure, ultrafast spectroscopy

Abstract: Pressure can reduce the distances among atoms, thereby modifying the overall optical characteristics of molecules. In this article, the excited state behavior of perylene is carefully observed under isotropic pressure and non-complexing condition. In a steady state, absorption peak shows red shift and spectral width are broadened with pressure increasing, which is ascribed to the π-electron delocalization between molecules. In a transient state, the transition dynamics presents a wavelike tendency with pressure increasing because the shift of self-tapping exciton state is contrary to that of Y-state with pressure increasing. The results conduce to understanding the influence of inter-molecule interaction on excited state behavior with inter-molecule distance decreasing, which contributes to studying the materials under extreme condition.

Key words: perylene, high-pressure, ultrafast spectroscopy

中图分类号: (Shock wave initiated reactions, high-pressure chemistry)

82.40.Fp

33.20.-t (Molecular spectra) 82.53.-k (Femtochemistry)

Ting-Ting Wang(王亭亭), Yu Zhang(张宇), Hong-Yu Tu(屠宏宇), Lu Han(韩露), Ji-Chao Cheng(程基超), Xin Wang(王鑫), Fang-Fei Li(李芳菲), Ling-Yun Pan(潘凌云), and Tian Cui(崔田). Steady and transient behavior of perylene under high pressure[J]. 中国物理B, 2021, 30(11): 118201-118201.

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Steady and transient behavior of perylene under high pressure

Steady and transient behavior of perylene under high pressure

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