中国物理B ›› 2020, Vol. 29 ›› Issue (8): 87804-087804.doi: 10.1088/1674-1056/ab9c07
所属专题: SPECIAL TOPIC — Water at molecular level
Jinbing Zhang(张晋兵), Qiang Wang(王强), Zexian Cao(曹则贤)
收稿日期:
2020-04-24
修回日期:
2020-06-01
出版日期:
2020-08-05
发布日期:
2020-08-05
通讯作者:
Qiang Wang, Zexian Cao
E-mail:qwang@iphy.ac.cn;zxcao@iphy.ac.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11974385 and 91956101), the Fund from the Chinese Academy of Sciences (Grant No. 1731300500030), and the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB07030100).
Jinbing Zhang(张晋兵)1,2, Qiang Wang(王强)2, Zexian Cao(曹则贤)2,3
Received:
2020-04-24
Revised:
2020-06-01
Online:
2020-08-05
Published:
2020-08-05
Contact:
Qiang Wang, Zexian Cao
E-mail:qwang@iphy.ac.cn;zxcao@iphy.ac.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11974385 and 91956101), the Fund from the Chinese Academy of Sciences (Grant No. 1731300500030), and the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB07030100).
摘要:
Transport properties and the associated structural heterogeneity of room temperature aqueous ionic liquids and especially of super-concentrated electrolyte aqueous solutions have received increasing attention, due to their potential application in ionic battery. This paper briefly reviews the results reported mainly since 2010 about the liquid-liquid separation, aggregation of polar and apolar domains in neat RTILs, and solvent clusters and 3D networks chiefly constructed by anions in super-concentrated electrolyte solutions. At the same time, the dominating effect of desolvation process of metal ions at electrode/electrolyte interface upon the transport of metal ions is stressed. This paper also presents the current understanding of how water affects the anion-cation interaction, structural heterogeneities, the structure of primary coordination sheath of metal ions and consequently their transport properties in free water-poor electrolytes.
中图分类号: (Solutions and ionic liquids)
张晋兵, 王强, 曹则贤. Effects of water on the structure and transport properties of room temperature ionic liquids and concentrated electrolyte solutions[J]. 中国物理B, 2020, 29(8): 87804-087804.
Jinbing Zhang(张晋兵), Qiang Wang(王强), Zexian Cao(曹则贤). Effects of water on the structure and transport properties of room temperature ionic liquids and concentrated electrolyte solutions[J]. Chin. Phys. B, 2020, 29(8): 87804-087804.
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