Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

doi:10.1088/1674-1056/25/11/117806

中国物理B ›› 2016, Vol. 25 ›› Issue (11): 117806-117806.doi: 10.1088/1674-1056/25/11/117806

• CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES • 上一篇下一篇

Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

A E Ershov, A P Gavrilyuk, S V Karpov, S P Polyutov

1 Institute of Computational Modeling, Russian Academy of Sciences, Krasnoyarsk 660036, Russia;
2 L. V. Kirensky Institute of Physics of the Russian Academy of Sciences, Krasnoyarsk 660036, Russia;
3 Siberian Federal University, Krasnoyarsk 660028, Russia;
4 Siberian State Aerospace University, Krasnoyarsk 660037, Russia

收稿日期:2016-04-11 修回日期:2016-07-06 出版日期:2016-11-05 发布日期:2016-11-05
通讯作者: S V Karpov E-mail:karpov@iph.krasn.ru

Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

A E Ershov^1,3,4, A P Gavrilyuk^1,3, S V Karpov^2,3,4, S P Polyutov³

1 Institute of Computational Modeling, Russian Academy of Sciences, Krasnoyarsk 660036, Russia;
2 L. V. Kirensky Institute of Physics of the Russian Academy of Sciences, Krasnoyarsk 660036, Russia;
3 Siberian Federal University, Krasnoyarsk 660028, Russia;
4 Siberian State Aerospace University, Krasnoyarsk 660037, Russia

Received:2016-04-11 Revised:2016-07-06 Online:2016-11-05 Published:2016-11-05
Contact: S V Karpov E-mail:karpov@iph.krasn.ru

摘要/Abstract

摘要： We have studied processes of interaction of pulsed laser radiation with resonant groups of plasmonic nanoparticles (resonant domains) in large colloidal nanoparticle aggregates having different interparticle gaps and particle size distributions. These processes are responsible for the origin of nonlinear optical effects and photochromic reactions in multiparticle aggregates. To describe photo-induced transformations in resonant domains and alterations in their absorption spectra remaining after the pulse action, we introduce the factor of spectral photomodification. Based on calculation of changes in thermodynamic, mechanical, and optical characteristics of the domains, the histograms of the spectrum photomodification factor have been obtained for various interparticle gaps, an average particle size, and the degree of polydispersity. Variations in spectra have been analyzed depending on the intensity of laser radiation and various combinations of size characteristics of domains. The obtained results can be used to predict manifestation of photochromic effects in composite materials containing different plasmonic nanoparticle aggregates in pulsed laser fields.

关键词: optodynamics, nanoparticle, surface plasmon, laser radiation

Abstract: We have studied processes of interaction of pulsed laser radiation with resonant groups of plasmonic nanoparticles (resonant domains) in large colloidal nanoparticle aggregates having different interparticle gaps and particle size distributions. These processes are responsible for the origin of nonlinear optical effects and photochromic reactions in multiparticle aggregates. To describe photo-induced transformations in resonant domains and alterations in their absorption spectra remaining after the pulse action, we introduce the factor of spectral photomodification. Based on calculation of changes in thermodynamic, mechanical, and optical characteristics of the domains, the histograms of the spectrum photomodification factor have been obtained for various interparticle gaps, an average particle size, and the degree of polydispersity. Variations in spectra have been analyzed depending on the intensity of laser radiation and various combinations of size characteristics of domains. The obtained results can be used to predict manifestation of photochromic effects in composite materials containing different plasmonic nanoparticle aggregates in pulsed laser fields.

Key words: optodynamics, nanoparticle, surface plasmon, laser radiation

中图分类号: (Nanoaggregates; nanocomposites)

78.67.Sc

73.20.Mf (Collective excitations (including excitons, polarons, plasmons and other charge-density excitations))

A E Ershov, A P Gavrilyuk, S V Karpov, S P Polyutov. Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields[J]. 中国物理B, 2016, 25(11): 117806-117806.

A E Ershov, A P Gavrilyuk, S V Karpov, S P Polyutov. Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields[J]. Chin. Phys. B, 2016, 25(11): 117806-117806.

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Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

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