Direct Coulomb explosion of N2O2+ induced by monochromatic extreme ultraviolet photons at 38.5 eV

doi:10.1088/1674-1056/ab8629

中国物理B ›› 2020, Vol. 29 ›› Issue (6): 63302-063302.doi: 10.1088/1674-1056/ab8629

• SPECIAL TOPIC—Recent advances in thermoelectric materials and devices • 上一篇下一篇

Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV

Min Zhang(张敏), B Najjari, Bang Hai(海帮), Dong-Mei Zhao(赵冬梅), Jian-Ting Lei(雷建廷), Da-Pu Dong(董达谱), Shao-Feng Zhang(张少锋), Xin-Wen Ma(马新文)

1 Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000, China;
2 University of Chinese Academy of Sciences, Beijing 100049, China;
3 School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000, China

收稿日期:2020-02-27 修回日期:2020-03-31 出版日期:2020-06-05 发布日期:2020-06-05
通讯作者: Shao-Feng Zhang, Xin-Wen Ma E-mail:zhangshf@impcas.ac.cn;x.ma@impcas.ac.cn
基金资助:
Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0402300).

Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV

Min Zhang(张敏)^1,2, B Najjari¹, Bang Hai(海帮)^1,2, Dong-Mei Zhao(赵冬梅)^1,2, Jian-Ting Lei(雷建廷)³, Da-Pu Dong(董达谱)^1,2, Shao-Feng Zhang(张少锋)^1,2, Xin-Wen Ma(马新文)^1,2

1 Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000, China;
2 University of Chinese Academy of Sciences, Beijing 100049, China;
3 School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000, China

Received:2020-02-27 Revised:2020-03-31 Online:2020-06-05 Published:2020-06-05
Contact: Shao-Feng Zhang, Xin-Wen Ma E-mail:zhangshf@impcas.ac.cn;x.ma@impcas.ac.cn
Supported by:
Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0402300).

摘要/Abstract

摘要： The direct Coulomb explosion of N₂O²⁺ has been investigated experimentally after double-ionization by a single extreme ultraviolet (EUV) photon with an energy of ～38.5 eV. From the ion-ion time-of-flight coincidence spectrum, the de-nitrogenation (N₂O²⁺→N⁺+NO⁺) and de-oxygenation (N₂O²⁺→O⁺+N₂⁺) photodissociation channels of N₂O²⁺ are unequivocally identified. The measured kinetic energy release (KER) distribution of the de-nitrogenation channel presents a major peak accompanied by a shoulder structure. We find that the major peak can be attributed to the direct photodissociation of the 1¹Δ and 1¹Σ⁺ states, while the shoulder structure should be ascribed to the predissociation of the 1¹Δ and 1¹Σ⁺ states via 1³Π state.

关键词: extreme ultraviolet photon, kinetic energy release, photodissociation pathway

Abstract: The direct Coulomb explosion of N₂O²⁺ has been investigated experimentally after double-ionization by a single extreme ultraviolet (EUV) photon with an energy of ～38.5 eV. From the ion-ion time-of-flight coincidence spectrum, the de-nitrogenation (N₂O²⁺→N⁺+NO⁺) and de-oxygenation (N₂O²⁺→O⁺+N₂⁺) photodissociation channels of N₂O²⁺ are unequivocally identified. The measured kinetic energy release (KER) distribution of the de-nitrogenation channel presents a major peak accompanied by a shoulder structure. We find that the major peak can be attributed to the direct photodissociation of the 1¹Δ and 1¹Σ⁺ states, while the shoulder structure should be ascribed to the predissociation of the 1¹Δ and 1¹Σ⁺ states via 1³Π state.

Key words: extreme ultraviolet photon, kinetic energy release, photodissociation pathway

中图分类号: (Photon interactions with molecules)

33.80.-b

张敏, 海帮, 赵冬梅, 雷建廷, 董达谱, 张少锋, 马新文. Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV[J]. 中国物理B, 2020, 29(6): 63302-063302.

Min Zhang(张敏), B Najjari, Bang Hai(海帮), Dong-Mei Zhao(赵冬梅), Jian-Ting Lei(雷建廷), Da-Pu Dong(董达谱), Shao-Feng Zhang(张少锋), Xin-Wen Ma(马新文). Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV[J]. Chin. Phys. B, 2020, 29(6): 63302-063302.

参考文献 32

[1]	Forster B P 2007 Climate Change 2007: The Physical Science Basis (New York: Cambridge University Press) pp. 1-21
[2]	Ravishankara A R, Daniel J S and Portmannand R W 2009 Science 326 123 doi: 10.1126/science.1176985
[3]	Thompson R L, Lassaletta L, Patra P K, Wilson C, Wells K C, Gressent A, Koffi E N, Chipperfield M P, Winiwarter W, Davidson E A, Tian H and Ganadell J G 2019 Nat. Clim. Chang. 9 993 doi: 10.1038/s41558-019-0613-7
[4]	Kotsina N, Kaziannis S, Danakas S and Kosmidis C 2013 J. Chem. Phys. 139 104313 doi: 10.1063/1.4820531
[5]	Kübel M, Alnaser A S, Bergues B, Pischke T, Schmidt J, Deng Y, Jendrzejewski C, Ullrich J, Paulus G G, Azzeer A M, Kleineberg U, Moshammer R and Kling M F 2014 New J. Phys. 16 065017 doi: 10.1088/1367-2630/16/6/065017
[6]	Price S D, Eland J H D, Fournier P G, Fournier J and Millie P 1988 J. Chem. Phys. 88 1511 doi: 10.1063/1.454129
[7]	Bhatt P, Singh R, Yadav N and Shanker R 2012 Phys. Rev. A 86 052708 doi: 10.1103/PhysRevA.86.052708
[8]	Chen L, Shan X, Zhao X, Zhu X L, Hu X Q, Wu Y, Feng W T, Guo D L, Zhang R T, Gao Y, Huang Z K, Wang J G, Ma X W and Chen X J 2019 Phys. Rev. A 99 012710 doi: 10.1103/PhysRevA.99.012710
[9]	Murphy R and Eberhardt W 1988 J. Chem. Phys. 89 4054 doi: 10.1063/1.454839
[10]	Eland J H D and Murphy V J 1991 Rapid Commun. Mass Spectrom. 5 221 doi: 10.1002/rcm.1290050502
[11]	Love N A and Price S D 2004 Phys. Chem. Chem. Phys. 6 4558 doi: 10.1039/b408853k
[12]	Khan A and Misra D 2016 J. Phys. B: At. Mol. Opt. Phys 49 055201 doi: 10.1088/0953-4075/49/5/055201
[13]	Siegmann B, Werner U, Lutz H and Mann R 2003 GSI Scientific Report 2002 (Darmstadt: GSI), p. 100
[14]	Hishikawa A, Iwamae A, Hoshina K, Kono M and Yamanouchi K 2005 J. Chem. Phys. 123 154305 doi: 10.1063/1.2032988
[15]	Ueyama M, Hasegawa H, Hishikawa A and Yamanouchi K 2005 J. Chem. Phys. 123 154305 doi: 10.1063/1.2032988
[16]	Ma J Y, Lin K, Ji Q Y, Zhang W B, Li H X, Sun F H, Qiang J J, Lu P X, Li H, Gong X C and Wu J 2019 Chin. Phys. B 28 093301 doi: 10.1088/1674-1056/ab38aa
[17]	Curtis D and Eland J 2007 J. Chem. Phys. 126 201101 doi: 10.1063/1.2743616
[18]	Alagia M, Candori P, Falcinelli S, Lavollée M, Pirani F, Richter R, Stranges S and Vecchiocattivi F 2007 J. Chem. Phys. 126 201101 doi: 10.1063/1.2743616
[19]	Falcinelli S, Rosi M, Candori P, Vecchiocattivi F, Farrar J M, Pirani F, Balucani N, Alagia M, Richter R and Stranges S 2016 Atmosphere 7 112 doi: 10.3390/atmos7090112
[20]	Falcinelli S, Pirani F, Alagia M, Schio L, Richter R, Stranges S, Balucani N and Vecchiocattivi F 2016 Atmosphere 7 112 doi: 10.3390/atmos7090112
[21]	Alagia M, Candori P, Falcinelli S, Lavollée M, Pirani F, Richter R, Stranges S and Vecchiocattivi F 2006 J. Chem. Phys. 124 204319 doi: 10.1063/1.2192517
[22]	Taylor S, Eland J H D and Hochlaf M 2006 J. Chem. Phys. 124 204319 doi: 10.1063/1.2192517
[23]	KMLABS https://www.kmlabs.com/
[24]	L'Huillier A and Balcou P 1993 Phys. Rev. Lett. 70 774 doi: 10.1103/PhysRevLett.70.774
[25]	Gagnon E, Sandhu A S, Paul A, Hagen K, Czasch A, Jahnke T, Ranitovic P, Cocke C L, Walker B, Murnane M M and Kapteyn H C 2008 Rev. Sci. Instrum. 79 063102 doi: 10.1063/1.2930869
[26]	Niu Y, Liang H J, Liu Y, Liu F Y, Ma R and Ding D J 2008 Chin. Phys. B 26 074222
[27]	Schmidt H T, Cederquist H, Schuch R, Bagge L, Källberg A, Hilke J, Rensfelt K G, Mergel V, Achler M, Dörner R, Spielberger L, Jagutzki O, Schmidt-Böcking H, Ullrich J, Reich H, Unverzagt M, Schmitt W and Moshammer R 2003 Rep. Prog. Phys 66 1463 doi: 10.1088/0034-4885/66/9/203
[28]	Ullrich J, Moshammer R, Dorn A, Dörner R, Schmidt L Ph H and Schmidt-Böcking H 2003 Rep. Prog. Phys 66 1463 doi: 10.1088/0034-4885/66/9/203
[29]	Ma X W, Zhang R T, Zhang S F, Zhu X L, Feng W T, Guo D L, Li B, Liu H P, Li C Y, Wang J G, Yan S C, Zhang P J and Wang Q 2011 Phys. Rev. A 83 052707 doi: 10.1103/PhysRevA.83.052707
[30]	Guo D L, Ma X W, Feng W T, Zhang S F and Zhu X L 2012 Acta Phys. Sin. 60 11341 (in Chinese)
[31]	Zhou X, Ranitovic P, Hogle C W, Eland J H D, Kapteyn H C and Murnane M M 2012 Nat. Phys. 8 232 doi: 10.1038/nphys2211
[32]	Eland J H 2003 Chem. Phys. 294 171 doi: 10.1016/j.chemphys.2003.08.001

Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV

Direct Coulomb explosion of N₂O²⁺ induced by monochromatic extreme ultraviolet photons at 38.5 eV

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