Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives

doi:10.1088/1674-1056/27/5/054208

中国物理B ›› 2018, Vol. 27 ›› Issue (5): 54208-054208.doi: 10.1088/1674-1056/27/5/054208

• ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS • 上一篇下一篇

Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives

Tong-xing Jin(金桐兴), Jun-yi Yang(杨俊义), Yu Fang(方宇), Yan-bing Han(韩艳兵), Ying-lin Song(宋瑛林)

1 College of Physics, Optoelectronics and Energy, Soochow University, Suzhou 215006, China;
2 Jiangsu Key Laboratory of Micro and Nano Heat Fluid Flow Technology and Energy Application, School of Mathematics and Physics, Suzhou University of Science and Technology, Suzhou 215009, China;
3 Department of Physics, Harbin Institute of Technology, Harbin 150001, China

收稿日期:2017-09-28 修回日期:2018-01-30 出版日期:2018-05-05 发布日期:2018-05-05
通讯作者: Ying-lin Song E-mail:ylsong@hit.edu.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos.U1630103 and 11704273),Natural Science Foundation of Jiangsu Province,China (Grant No.BK20170375),and Natural Science Foundation of the Higher Education Institutions of Jiangsu Province,China (Grant No.17KJB140021).

Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives

Tong-xing Jin(金桐兴)¹, Jun-yi Yang(杨俊义)¹, Yu Fang(方宇)², Yan-bing Han(韩艳兵)³, Ying-lin Song(宋瑛林)^1,3

1 College of Physics, Optoelectronics and Energy, Soochow University, Suzhou 215006, China;
2 Jiangsu Key Laboratory of Micro and Nano Heat Fluid Flow Technology and Energy Application, School of Mathematics and Physics, Suzhou University of Science and Technology, Suzhou 215009, China;
3 Department of Physics, Harbin Institute of Technology, Harbin 150001, China

Received:2017-09-28 Revised:2018-01-30 Online:2018-05-05 Published:2018-05-05
Contact: Ying-lin Song E-mail:ylsong@hit.edu.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos.U1630103 and 11704273),Natural Science Foundation of Jiangsu Province,China (Grant No.BK20170375),and Natural Science Foundation of the Higher Education Institutions of Jiangsu Province,China (Grant No.17KJB140021).

摘要/Abstract

摘要： Two dimethylamino-carbaldehyde derivatives with different π-bridge lengths were prepared, and their transient optical properties and photophysical mechanisms were investigated by transient absorption spectroscopy and Z-scan measurements. Owing to the difference in molecular structures, the two compounds exhibit different populations of locally excited states and, therefore, they also produce different transient absorption spectra. After photoexcitation, both molecular materials exhibit a wide excited state absorption band from 450 nm to 1000 nm. Meanwhile, the excited state lifetimes are dramatically different, 2 ns and 100 ps, for the two molecules. A figure of merit greater than 2 at the wavelength of 1000 nm is obtained. The results show that modulating the population of the locally excited states in this type of molecule can be a promising approach for obtaining optical switching and solar cell materials.

关键词: nonlinear optics, transient absorption spectra, dimethylamino-carbaldehyde derivatives

Abstract: Two dimethylamino-carbaldehyde derivatives with different π-bridge lengths were prepared, and their transient optical properties and photophysical mechanisms were investigated by transient absorption spectroscopy and Z-scan measurements. Owing to the difference in molecular structures, the two compounds exhibit different populations of locally excited states and, therefore, they also produce different transient absorption spectra. After photoexcitation, both molecular materials exhibit a wide excited state absorption band from 450 nm to 1000 nm. Meanwhile, the excited state lifetimes are dramatically different, 2 ns and 100 ps, for the two molecules. A figure of merit greater than 2 at the wavelength of 1000 nm is obtained. The results show that modulating the population of the locally excited states in this type of molecule can be a promising approach for obtaining optical switching and solar cell materials.

Key words: nonlinear optics, transient absorption spectra, dimethylamino-carbaldehyde derivatives

中图分类号: (Optical transient phenomena: quantum beats, photon echo, free-induction decay, dephasings and revivals, optical nutation, and self-induced transparency)

42.50.Md

78.47.jb (Transient absorption) 42.70.Nq (Other nonlinear optical materials; photorefractive and semiconductor materials)

金桐兴, 杨俊义, 方宇, 韩艳兵, 宋瑛林. Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives[J]. 中国物理B, 2018, 27(5): 54208-054208.

Tong-xing Jin(金桐兴), Jun-yi Yang(杨俊义), Yu Fang(方宇), Yan-bing Han(韩艳兵), Ying-lin Song(宋瑛林). Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives[J]. Chin. Phys. B, 2018, 27(5): 54208-054208.

参考文献 33

[13]	Polli D, Antognazza M R, Brida D, Lanzani G, Cerullo G and De Silvestri S 2008 Chem. Phys. 350 45
[1]	Ehrlich J E, Wu X L, Lee I Y, Hu Z Y, Röckel H, Marder S R and Perry J W 1997 Opt. Lett. 22 1843
[14]	Zewail A H 2000 J. Phys. Chem. A 104 5660
[2]	He G S, Tan L S, Zheng Q and Prasad P N 2008 Chem. Rev. 108 1245
[15]	Feng W K, Feng Y Y, Wang S F, Feng W, Yi W H Y and Gong Q H 2010 Chin. Phys. B 19 113401
[3]	Almosawe A J and Saadon H L 2013 Chin. Opt. Lett. 11 041902
[16]	Lange C, Köster N S, Chatterjee S, Sigg H, Chrastina D, Isella G, von Känel H, Schäfer M, Kira M and Koch S W 2009 Phys. Rev. B 79 201306
[4]	Si J and Hirao K 2007 Appl. Phys. Lett. 91 091105
[17]	Tamaki Y, Furube A, Murai M, Hara K, Katoh R and Tachiya M 2007 Phys. Chem. Chem. Phys. 9 1453
[5]	Tan W, Liu H, Si J and Hou X 2008 Appl. Phys. Lett. 93 051109
[18]	Ruckebusch C, Sliwa M, Pernot P, De Juan A and Tauler R 2012 J. Photochem. Photobiol. C 13 1
[6]	Nguyen V, Si J, Yan L and Hou X 2015 Carbon 95 659
[19]	Zhou F, Shao J, Yang Y, Zhao J, Guo H, Li X, Ji S, Zhang Z and Zhang Z 2011 Eur. J. Org. Chem. 2011 4773
[7]	Staub K, Levina G A, Barlow S, Kowalczyk T C, Lackritz H S, Barzoukas M, Fort A and Marder S R 2003 J. Mater. Chem. 13 825
[20]	Haidekker M A, Brady T P, Lichlyter D and Theodorakis E A 2005 Bioorg. Chem. 33 415
[8]	Huang T H, Yang D, Kang Z H, Miao E L, Lu R, Zhou H P, Wang F, Wang G W, Cheng P F, Wang Y H and Zhang H Z 2013 Opt. Mater. 35 467
[21]	Haidekker M A and Theodorakis E A 2007 Org. Biomol. Chem. 5 1669
[9]	Achelle S, Barsella A, Caro B and Robin-le Guen F 2015 RSC Adv. 5 39218
[22]	Stsiapura V I, Maskevich A A, Kuzmitsky V A, Uversky V N, Kuznetsova I M and Turoverov K K 2008 J. Phys. Chem. B 112 15893
[10]	Reinhardt B A, Brott L L, Clarson S J, Dillard A G, Bhatt J C, Kannan R, Yuan L X, He G S and Prasad P N 1998 Chem. Mater. 10 1863
[23]	Saha S K, Purkayastha P, Das A B and Dhara S 2008 Photochem. Photobiol A:Chem. 199 179
[11]	Belfield K D, Hagan, D J, Van Stryland E W, Schafer K J and Negres R A 1999 Org. Lett. 1 1575
[24]	Hwang Y J and Shin D M 2007 Mol. Cryst. Liq. Cryst. 472 25
[12]	Antonov L, Kamada K, Ohta K and Kamounah F S 2003 Phys. Chem. Chem. Phys. 5 1193
[25]	Klikar M, Bureš F, Pytela O, Mikysek T, Padělková Z, Barsella A, Dorkenoo K and Achelle S 2013 New J. Chem. 37 4230
[13]	Polli D, Antognazza M R, Brida D, Lanzani G, Cerullo G and De Silvestri S 2008 Chem. Phys. 350 45
[26]	Wu X, Xiao J, Sun R, Jin T, Yang J, Shi G, Wang Y, Zhang X and Song Y 2017 Adv. Opt. Mater. 5 1600712
[14]	Zewail A H 2000 J. Phys. Chem. A 104 5660
[27]	Albinsson B, Eng M P, Pettersson K and Winters M U 2007 Phys. Chem. Chem. Phys. 9 5847
[15]	Feng W K, Feng Y Y, Wang S F, Feng W, Yi W H Y and Gong Q H 2010 Chin. Phys. B 19 113401
[28]	Frisch M J, Trucks G W, Schlegel H B, Scuseria G E, Robb M A, Cheeseman J R and Nakatsuji H 2010 Gaussian development version. Revision h, 1
[16]	Lange C, Köster N S, Chatterjee S, Sigg H, Chrastina D, Isella G, von Känel H, Schäfer M, Kira M and Koch S W 2009 Phys. Rev. B 79 201306
[29]	Hagberg D P, Marinado T, Karlsson K M, Nonomura K, Qin P, Boschloo G, Brinck T, Hagfeldt A and Sun L 2007 J. Org. Chem. 72 9550
[17]	Tamaki Y, Furube A, Murai M, Hara K, Katoh R and Tachiya M 2007 Phys. Chem. Chem. Phys. 9 1453
[30]	Ajayaghosh A 2003 Chem. Soc. Rev. 32 181
[18]	Ruckebusch C, Sliwa M, Pernot P, De Juan A and Tauler R 2012 J. Photochem. Photobiol. C 13 1
[31]	Xia T, Dogariu A, Mansour K, Hagan D J, Said A A, Van Stryland E W and Shi S 1998 JOSA B 15 1497
[19]	Zhou F, Shao J, Yang Y, Zhao J, Guo H, Li X, Ji S, Zhang Z and Zhang Z 2011 Eur. J. Org. Chem. 2011 4773
[32]	Ehlers F, Wild D A, Lenzer T and Oum K 2007 J. Phys. Chem. A 111 2257
[20]	Haidekker M A, Brady T P, Lichlyter D and Theodorakis E A 2005 Bioorg. Chem. 33 415
[33]	Liu X, Osgood R M, Vlasov Y A and Green W M 2010 Nat. Photon. 4 557
[21]	Haidekker M A and Theodorakis E A 2007 Org. Biomol. Chem. 5 1669
[22]	Stsiapura V I, Maskevich A A, Kuzmitsky V A, Uversky V N, Kuznetsova I M and Turoverov K K 2008 J. Phys. Chem. B 112 15893
[23]	Saha S K, Purkayastha P, Das A B and Dhara S 2008 Photochem. Photobiol A:Chem. 199 179
[24]	Hwang Y J and Shin D M 2007 Mol. Cryst. Liq. Cryst. 472 25
[25]	Klikar M, Bureš F, Pytela O, Mikysek T, Padělková Z, Barsella A, Dorkenoo K and Achelle S 2013 New J. Chem. 37 4230
[26]	Wu X, Xiao J, Sun R, Jin T, Yang J, Shi G, Wang Y, Zhang X and Song Y 2017 Adv. Opt. Mater. 5 1600712
[27]	Albinsson B, Eng M P, Pettersson K and Winters M U 2007 Phys. Chem. Chem. Phys. 9 5847
[28]	Frisch M J, Trucks G W, Schlegel H B, Scuseria G E, Robb M A, Cheeseman J R and Nakatsuji H 2010 Gaussian development version. Revision h, 1
[29]	Hagberg D P, Marinado T, Karlsson K M, Nonomura K, Qin P, Boschloo G, Brinck T, Hagfeldt A and Sun L 2007 J. Org. Chem. 72 9550
[30]	Ajayaghosh A 2003 Chem. Soc. Rev. 32 181
[31]	Xia T, Dogariu A, Mansour K, Hagan D J, Said A A, Van Stryland E W and Shi S 1998 JOSA B 15 1497
[32]	Ehlers F, Wild D A, Lenzer T and Oum K 2007 J. Phys. Chem. A 111 2257
[33]	Liu X, Osgood R M, Vlasov Y A and Green W M 2010 Nat. Photon. 4 557

Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives

Modulation and mechanism of ultrafast transient spectroscopy based on dimethylamino-carbaldehyde derivatives

RichHTML

PDF (PC)

赞

可视化

摘要/Abstract

引用本文

使用本文

参考文献 33

相关文章 15

Metrics

本文评价

推荐阅读 0

[1]	Lei Chen(陈磊), Pan Li(李磐), He-Shan Liu(刘河山), Jin Yu(余锦), Chang-Jun Ke(柯常军), and Zi-Ren Luo(罗子人). Coupled-generalized nonlinear Schrödinger equations solved by adaptive step-size methods in interaction picture[J]. 中国物理B, 2023, 32(2): 24213-024213.
[2]	Chenxi Yu(于晨曦), Long Gao(高龙), Wentong Li(李文彤), Qian Wang(王倩), Meng Wang(王萌), and Jiaqi Zhang(张佳旗). Scanning the optical characteristics of lead-free cesium titanium bromide double perovskite nanocrystals[J]. 中国物理B, 2022, 31(5): 54218-054218.
[3]	Ji Wang(王佶), Yanqing Zheng(郑燕青), and Yunlin Chen(陈云琳). Noncollinear phase-matching geometries in ultra-broadband quasi-parametric amplification[J]. 中国物理B, 2022, 31(5): 54213-054213.
[4]	Zi-Yuan Li(李子元), Qi Li(李骐), and Zhou Li(李舟). High-order harmonic generations in tilted Weyl semimetals[J]. 中国物理B, 2022, 31(12): 124204-124204.
[5]	Zheng Ge(葛正), Chen Yang(杨琛), Yin-Hai Li(李银海), Yan Li(李岩), Shi-Kai Liu(刘世凯), Su-Jian Niu(牛素俭), Zhi-Yuan Zhou(周志远), and Bao-Sen Shi(史保森). Up-conversion detection of mid-infrared light carrying orbital angular momentum[J]. 中国物理B, 2022, 31(10): 104210-104210.
[6]	Jiacheng Liu(刘嘉成), Chao Wu(吴超), Gongyu Xia(夏功榆), Qilin Zheng(郑骑林), Zhihong Zhu(朱志宏), and Ping Xu(徐平). Bandwidth-tunable silicon nitride microring resonators[J]. 中国物理B, 2022, 31(1): 14201-014201.
[7]	Lu-Lu Xu(徐路路), Ying-Ying Wang(王莹莹), Li Jiang(江丽), Pei-Long Yang(杨佩龙), Lei Zhang(张磊), and Shi-Xun Dai(戴世勋). A low-threshold multiwavelength Brillouin fiber laser with double-frequency spacing based on a small-core fiber[J]. 中国物理B, 2021, 30(8): 84210-084210.
[8]	Yingcong Zhang(张颖聪), Wenjuan Cai(蔡文娟), Xianping Wang(王贤平), Wen Yuan(袁文), Cheng Yin(殷澄), Jun Li(李俊), Haimei Luo(罗海梅), and Minghuang Sang(桑明煌). Low-threshold bistable reflection assisted by oscillating wave interaction with Kerr nonlinear medium[J]. 中国物理B, 2021, 30(8): 84203-084203.
[9]	Meng Shang(尚萌), Pei-Ling Li(李培玲), Yu-Hua Wang(王玉华), and Jing-Wei Luo(罗经纬). Third-order nonlinear optical properties of graphene composites: A review[J]. 中国物理B, 2021, 30(8): 80703-080703.
[10]	Jing Wang(王静), Chun-Hui Zhang(张春辉), Jing-Yang Liu(刘靖阳), Xue-Rui Qian(钱雪瑞), Jian Li(李剑), and Qin Wang(王琴). Improving the purity of heralded single-photon sources through spontaneous parametric down-conversion process[J]. 中国物理B, 2021, 30(7): 70304-070304.
[11]	王弘耿, 宋其迎, 蔡懿, 林庆钢, 陆小微, 上官煌城, 艾月霞, 徐世祥. Recent advances in generation of terahertz vortex beams andtheir applications[J]. 中国物理B, 2020, 29(9): 97404-097404.
[12]	王瑞敏, Irfan Ahmed, Faizan Raza, 李昌彪, 张彦鹏. Light slowing and all-optical time division multiplexing of hybrid four-wave mixing signal in nitrogen-vacancy center[J]. 中国物理B, 2020, 29(5): 54204-054204.
[13]	王玉龙, 赵波, 闵长俊, 张聿全, 杨建军, 郭春雷, 袁小聪. Research progress of femtosecond surface plasmon polariton[J]. 中国物理B, 2020, 29(2): 27302-027302.
[14]	韩杰, 常圣东, 吕彦佳, 刘永. Numerical investigation on coherent mid-infrared supercontinuum generation in chalcogenide PCFs with near-zero flattened all-normal dispersion profiles[J]. 中国物理B, 2019, 28(10): 104204-104204.
[15]	游琪, 蒋乐勇, 戴小玉, 项元江. Enhancement and control of the Goos-Hänchen shift bynonlinear surface plasmon resonance in graphene[J]. 中国物理B, 2018, 27(9): 94211-094211.