Periodical polarization reversal modulation in multiferroic MnWO4 under high magnetic fields

doi:10.1088/1674-1056/acca07

中国物理B ›› 2023, Vol. 32 ›› Issue (12): 127505-127505.doi: 10.1088/1674-1056/acca07

Periodical polarization reversal modulation in multiferroic MnWO₄ under high magnetic fields

Congbin Liu(刘从斌)¹, Jinbing Cheng(程晋炳)¹, Junbao He(何俊宝)¹, Yongsheng Zhu(朱永胜)¹, Wan Chang(常婉)¹, Xiaoyu Lu(路晓宇)¹, Junfeng Wang(王俊峰)², Meiyan Cui(崔美艳)³, Jinshu Huang(黄金书)¹, Dawei Zhou(周大伟)¹, Rui Chen(陈瑞)⁴, Hao Jiang(江浩)¹, Chuangchuang Ma(马创创)¹, Chao Dong(董超)^2,†, and Yongsong Luo(罗永松)^1,4,‡

1 Henan International Joint Laboratory of MXene Materials Microstructure, College of Physics and Electronic Engineering, Nanyang Normal University, Nanyang 473061, China;
2 Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China;
3 State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China;
4 Key Laboratory of Microelectronics and Energy of Henan Province, Henan Joint International Research Laboratory of New Energy Storage Technology, Xinyang Normal University, Xinyang 464000, China

收稿日期:2022-12-29 修回日期:2023-03-24 接受日期:2023-04-04 出版日期:2023-11-14 发布日期:2023-11-22
通讯作者: Chao Dong, Yongsong Luo E-mail:dongchao@hust.edu.cn;ysluo@xynu.edu.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos.12074135, 12104388, and 52272219), Nanyang Normal University, the Natural Science Foundation of Henan Province (Grant Nos.222300420255 and 232300421220), and the Key Scientific and Technological Projiect of Technology Depeartment of Henan Province of China (Grant Nos.222102230105 and 212102210448). Congbin Liu acknowledges Wanxin Liu at the WHMFC for help with the data measured in pulsed fields.

Periodical polarization reversal modulation in multiferroic MnWO₄ under high magnetic fields

1 Henan International Joint Laboratory of MXene Materials Microstructure, College of Physics and Electronic Engineering, Nanyang Normal University, Nanyang 473061, China;
2 Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China;
3 State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China;
4 Key Laboratory of Microelectronics and Energy of Henan Province, Henan Joint International Research Laboratory of New Energy Storage Technology, Xinyang Normal University, Xinyang 464000, China

Received:2022-12-29 Revised:2023-03-24 Accepted:2023-04-04 Online:2023-11-14 Published:2023-11-22
Contact: Chao Dong, Yongsong Luo E-mail:dongchao@hust.edu.cn;ysluo@xynu.edu.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos.12074135, 12104388, and 52272219), Nanyang Normal University, the Natural Science Foundation of Henan Province (Grant Nos.222300420255 and 232300421220), and the Key Scientific and Technological Projiect of Technology Depeartment of Henan Province of China (Grant Nos.222102230105 and 212102210448). Congbin Liu acknowledges Wanxin Liu at the WHMFC for help with the data measured in pulsed fields.

摘要/Abstract

摘要： We report polarization reversal periodically controlled by the electric field in multiferroic MnWO₄ with a pulsed field up to 52 T. The electric polarization cannot be reversed by successive opposite electric fields in low magnetic fields (< 14 T) at 4.2 K, whereas polarization reversal is directly achieved by two opposite electric fields under high magnetic fields (< 45 T). Interestingly, the polarization curve of rising and falling fields for H||u (magnetic easy axis) is irreversible when the magnetic field is close to 52 T. In this case, the rising and falling polarization curves can be individually reversed by the electric field, and thus require five cycles to recover to the initial condition by the order of the applied electric fields (+E, -E, -E, +E, +E). In addition, we find that ferroelectric phase IV can be tuned from parallel to antiparallel in relation to ferroelectric phase AF2 by applying a magnetic field approximated to the c axis.

关键词: polarization reversal, periodical modulation, high magnetic field

Abstract: We report polarization reversal periodically controlled by the electric field in multiferroic MnWO₄ with a pulsed field up to 52 T. The electric polarization cannot be reversed by successive opposite electric fields in low magnetic fields (< 14 T) at 4.2 K, whereas polarization reversal is directly achieved by two opposite electric fields under high magnetic fields (< 45 T). Interestingly, the polarization curve of rising and falling fields for H||u (magnetic easy axis) is irreversible when the magnetic field is close to 52 T. In this case, the rising and falling polarization curves can be individually reversed by the electric field, and thus require five cycles to recover to the initial condition by the order of the applied electric fields (+E, -E, -E, +E, +E). In addition, we find that ferroelectric phase IV can be tuned from parallel to antiparallel in relation to ferroelectric phase AF2 by applying a magnetic field approximated to the c axis.

Key words: polarization reversal, periodical modulation, high magnetic field

中图分类号: (Magnetoelectric effects, multiferroics)

75.85.+t

77.80.Fm (Switching phenomena) 77.22.Ej (Polarization and depolarization)

Congbin Liu(刘从斌), Jinbing Cheng(程晋炳), Junbao He(何俊宝), Yongsheng Zhu(朱永胜), Wan Chang(常婉), Xiaoyu Lu(路晓宇), Junfeng Wang(王俊峰), Meiyan Cui(崔美艳), Jinshu Huang(黄金书), Dawei Zhou(周大伟), Rui Chen(陈瑞), Hao Jiang(江浩),Chuangchuang Ma(马创创), Chao Dong(董超), and Yongsong Luo(罗永松). Periodical polarization reversal modulation in multiferroic MnWO₄ under high magnetic fields[J]. 中国物理B, 2023, 32(12): 127505-127505.

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Periodical polarization reversal modulation in multiferroic MnWO₄ under high magnetic fields

Periodical polarization reversal modulation in multiferroic MnWO₄ under high magnetic fields

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