Structure design for high performance n-type polymer thermoelectric materials

doi:10.1088/1674-1056/ac3a64

中国物理B ›› 2022, Vol. 31 ›› Issue (2): 28506-028506.doi: 10.1088/1674-1056/ac3a64

所属专题： SPECIAL TOPIC — Organic and hybrid thermoelectrics

Structure design for high performance n-type polymer thermoelectric materials

Qi Zhang(张奇), Hengda Sun(孙恒达)^†, and Meifang Zhu(朱美芳)

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai 201620, China

收稿日期:2021-08-24 修回日期:2021-11-05 接受日期:2021-11-17 出版日期:2022-01-13 发布日期:2022-01-22
通讯作者: Hengda Sun E-mail:sunhengda@dhu.edu.cn
基金资助:
Project supported by the Fundamental Research Funds for the Central Universities, China (Grant No. 21D110637), the National Natural Science Foundation of China (Grant No. 52173156), the Science and Technology Commission of Shanghai Municipality, China (Grant No. 20JC1414900), and the Chinese Academy of Sciences (Faculty Consultation and Evaluation Project 2020-ZW07-A-017).

Structure design for high performance n-type polymer thermoelectric materials

Qi Zhang(张奇), Hengda Sun(孙恒达)^†, and Meifang Zhu(朱美芳)

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai 201620, China

Received:2021-08-24 Revised:2021-11-05 Accepted:2021-11-17 Online:2022-01-13 Published:2022-01-22
Contact: Hengda Sun E-mail:sunhengda@dhu.edu.cn
Supported by:
Project supported by the Fundamental Research Funds for the Central Universities, China (Grant No. 21D110637), the National Natural Science Foundation of China (Grant No. 52173156), the Science and Technology Commission of Shanghai Municipality, China (Grant No. 20JC1414900), and the Chinese Academy of Sciences (Faculty Consultation and Evaluation Project 2020-ZW07-A-017).

摘要/Abstract

摘要： Organic thermoelectric (OTE) materials have been regarded as a potential candidate to harvest waste heat from complex, low temperature surfaces of objects and convert it into electricity. Recently, n-type conjugated polymers as organic thermoelectric materials have aroused intensive research in order to improve their performance to match up with their p-type counterpart. In this review, we discuss aspects that affect the performance of n-type OTEs, and further focus on the effect of planarity of backbone on the doping efficiency and eventually the TE performance. We then summarize strategies such as implementing rigid n-type polymer backbone or modifying conventional polymer building blocks for more planar conformation. In the outlook part, we conclude forementioned devotions and point out new possibility that may promote the future development of this field.

关键词: organic thermoelectrics, conducting polymers, organic semiconductor doping

Abstract: Organic thermoelectric (OTE) materials have been regarded as a potential candidate to harvest waste heat from complex, low temperature surfaces of objects and convert it into electricity. Recently, n-type conjugated polymers as organic thermoelectric materials have aroused intensive research in order to improve their performance to match up with their p-type counterpart. In this review, we discuss aspects that affect the performance of n-type OTEs, and further focus on the effect of planarity of backbone on the doping efficiency and eventually the TE performance. We then summarize strategies such as implementing rigid n-type polymer backbone or modifying conventional polymer building blocks for more planar conformation. In the outlook part, we conclude forementioned devotions and point out new possibility that may promote the future development of this field.

Key words: organic thermoelectrics, conducting polymers, organic semiconductor doping

中图分类号: (Thermoelectric devices)

85.80.Fi

82.35.Cd (Conducting polymers) 81.05.Fb (Organic semiconductors)

Qi Zhang(张奇), Hengda Sun(孙恒达), and Meifang Zhu(朱美芳). Structure design for high performance n-type polymer thermoelectric materials[J]. 中国物理B, 2022, 31(2): 28506-028506.

Qi Zhang(张奇), Hengda Sun(孙恒达), and Meifang Zhu(朱美芳). Structure design for high performance n-type polymer thermoelectric materials[J]. Chin. Phys. B, 2022, 31(2): 28506-028506.

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Structure design for high performance n-type polymer thermoelectric materials

Structure design for high performance n-type polymer thermoelectric materials

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