Theoretical estimation of sonochemical yield in bubble cluster in acoustic field

doi:10.1088/1674-1056/ab6108

中国物理B ›› 2020, Vol. 29 ›› Issue (1): 14304-014304.doi: 10.1088/1674-1056/ab6108

• ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS • 上一篇下一篇

Theoretical estimation of sonochemical yield in bubble cluster in acoustic field

Zhuang-Zhi Shen(沈壮志)

School of Physics&Information Technology, Shaanxi Normal University, Shaanxi Key Laboratory of Ultrasonics, Xi'an 710119, China

收稿日期:2019-05-07 修回日期:2019-06-10 出版日期:2020-01-05 发布日期:2020-01-05
通讯作者: Zhuang-Zhi Shen E-mail:szz6@163.com
基金资助:
Project supported by the National Natural Science Foundation of China (Grant No. 11674207).

Theoretical estimation of sonochemical yield in bubble cluster in acoustic field

Zhuang-Zhi Shen(沈壮志)

School of Physics&Information Technology, Shaanxi Normal University, Shaanxi Key Laboratory of Ultrasonics, Xi'an 710119, China

Received:2019-05-07 Revised:2019-06-10 Online:2020-01-05 Published:2020-01-05
Contact: Zhuang-Zhi Shen E-mail:szz6@163.com
Supported by:
Project supported by the National Natural Science Foundation of China (Grant No. 11674207).

摘要/Abstract

摘要： In order to learn more about the physical phenomena occurring in cloud cavitation, the nonlinear dynamics of a spherical cluster of cavitation bubbles and cavitation bubbles in cluster in an acoustic field excited by a square pressure wave are numerically investigated by considering viscosity, surface tension, and the weak compressibility of the liquid. The theoretical prediction of the yield of oxidants produced inside bubbles during the strong collapse stage of cavitation bubbles is also investigated. The effects of acoustic frequency, acoustic pressure amplitude, and the number of bubbles in cluster on bubble temperature and the quantity of oxidants produced inside bubbles are analyzed. The results show that the change of acoustic frequency, acoustic pressure amplitude, and the number of bubbles in cluster have an effect not only on temperature and the quantity of oxidants inside the bubble, but also on the degradation types of pollutants, which provides a guidance in improving the sonochemical degradation of organic pollutants.

关键词: bubble cluster models, bubble cluster dynamics, chemical kinetics, bubble temperature, strong oxidants, acoustic cavitation

Abstract: In order to learn more about the physical phenomena occurring in cloud cavitation, the nonlinear dynamics of a spherical cluster of cavitation bubbles and cavitation bubbles in cluster in an acoustic field excited by a square pressure wave are numerically investigated by considering viscosity, surface tension, and the weak compressibility of the liquid. The theoretical prediction of the yield of oxidants produced inside bubbles during the strong collapse stage of cavitation bubbles is also investigated. The effects of acoustic frequency, acoustic pressure amplitude, and the number of bubbles in cluster on bubble temperature and the quantity of oxidants produced inside bubbles are analyzed. The results show that the change of acoustic frequency, acoustic pressure amplitude, and the number of bubbles in cluster have an effect not only on temperature and the quantity of oxidants inside the bubble, but also on the degradation types of pollutants, which provides a guidance in improving the sonochemical degradation of organic pollutants.

Key words: bubble cluster models, bubble cluster dynamics, chemical kinetics, bubble temperature, strong oxidants, acoustic cavitation

中图分类号: (Nonlinear acoustics)

43.25.+y

43.35.+d (Ultrasonics, quantum acoustics, and physical effects of sound) 44.20.+b (Boundary layer heat flow) 82.20.-w (Chemical kinetics and dynamics)

沈壮志. Theoretical estimation of sonochemical yield in bubble cluster in acoustic field[J]. 中国物理B, 2020, 29(1): 14304-014304.

Zhuang-Zhi Shen(沈壮志). Theoretical estimation of sonochemical yield in bubble cluster in acoustic field[J]. Chin. Phys. B, 2020, 29(1): 14304-014304.

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Theoretical estimation of sonochemical yield in bubble cluster in acoustic field

Theoretical estimation of sonochemical yield in bubble cluster in acoustic field

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