Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

doi:10.1088/1674-1056/24/4/043303

中国物理B ›› 2015, Vol. 24 ›› Issue (4): 43303-043303.doi: 10.1088/1674-1056/24/4/043303

• ATOMIC AND MOLECULAR PHYSICS • 上一篇下一篇

Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

陈洲, 佟秋男, 张丛丛, 胡湛

Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China

收稿日期:2014-10-07 修回日期:2014-11-05 出版日期:2015-04-05 发布日期:2015-04-05
基金资助:
Project supported by the National Basic Research Program of China (Grant No. 2013CB922200) and the National Natural Science Foundation of China (Grant No. 11374124).

Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

Chen Zhou (陈洲), Tong Qiu-Nan (佟秋男), Zhang Cong-Cong (张丛丛), Hu Zhan (胡湛)

Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China

Received:2014-10-07 Revised:2014-11-05 Online:2015-04-05 Published:2015-04-05
Contact: Hu Zhan E-mail:huzhan@jlu.edu.cn
Supported by:
Project supported by the National Basic Research Program of China (Grant No. 2013CB922200) and the National Natural Science Foundation of China (Grant No. 11374124).

摘要/Abstract

摘要：

Identification of acetone and its two isomers, and the control of their ionization and dissociation processes are performed using a dual-mass-spectrometer scheme. The scheme employs two sets of time of flight mass spectrometers to simultaneously acquire the mass spectra of two different molecules under the irradiation of identically shaped femtosecond laser pulses. The optimal laser pulses are found using closed-loop learning method based on a genetic algorithm. Compared with the mass spectra of the two isomers that are obtained with the transform limited pulse, those obtained under the irradiation of the optimal laser pulse show large differences and the various reaction pathways of the two molecules are selectively controlled. The experimental results demonstrate that the scheme is quite effective and useful in studies of two molecules having common mass peaks, which makes a traditional single mass spectrometer unfeasible.

关键词: shaped femtosecond pulse, identification, ionization and dissociation

Abstract:

Key words: shaped femtosecond pulse, identification, ionization and dissociation

中图分类号: (Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states))

33.80.Rv

42.25.Kb (Coherence)

陈洲, 佟秋男, 张丛丛, 胡湛. Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization[J]. 中国物理B, 2015, 24(4): 43303-043303.

Chen Zhou (陈洲), Tong Qiu-Nan (佟秋男), Zhang Cong-Cong (张丛丛), Hu Zhan (胡湛). Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization[J]. Chin. Phys. B, 2015, 24(4): 43303-043303.

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Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

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