An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H2O2 chemiluminescence system and its potential analytical application

doi:10.1088/1674-1056/23/4/048103

中国物理B ›› 2014, Vol. 23 ›› Issue (4): 48103-048103.doi: 10.1088/1674-1056/23/4/048103

• INTERDISCIPLINARY PHYSICS AND RELATED AREAS OF SCIENCE AND TECHNOLOGY • 上一篇下一篇

An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application

王闻硕^a, 何大伟^a, 王继红^b, 段嘉华^a, 彭洪尚^a, 吴洪鹏^a, 富鸣^a, 王永生^a, 张希清^a

a Key Laboratory of Luminescence and Optical Information, Ministry of Education, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, China;
b School of Science, China University of Petroleum, Beijing 102249, China

收稿日期:2013-09-12 修回日期:2013-10-30 出版日期:2014-04-15 发布日期:2014-04-15
基金资助:
Project supported by the National Key Basic Research Program, China (Grant Nos. 2011CB932700 and 2011CB932703), the National Natural Science Foundation of China (Grant Nos. 61378073, 61335006, 91123025, and 61077044), and the Beijing Natural Science FundProject, China (Grant No. 4132031).

An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application

Wang Wen-Shuo (王闻硕)^a, He Da-Wei (何大伟)^a, Wang Ji-Hong (王继红)^b, Duan Jia-Hua (段嘉华)^a, Peng Hong-Shang (彭洪尚)^a, Wu Hong-Peng (吴洪鹏)^a, Fu Ming (富鸣)^a, Wang Yong-Sheng (王永生)^a, Zhang Xi-Qing (张希清)^a

a Key Laboratory of Luminescence and Optical Information, Ministry of Education, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, China;
b School of Science, China University of Petroleum, Beijing 102249, China

Received:2013-09-12 Revised:2013-10-30 Online:2014-04-15 Published:2014-04-15
Contact: He Da-Wei, Zhang Xi-Qing E-mail:dwhe@bjtu.edu.cn;xqzhang@bjtu.edu.cn
About author:81.05.ue; 78.67.Bf; 78.60.Ps; 87.85.fk
Supported by:
Project supported by the National Key Basic Research Program, China (Grant Nos. 2011CB932700 and 2011CB932703), the National Natural Science Foundation of China (Grant Nos. 61378073, 61335006, 91123025, and 61077044), and the Beijing Natural Science FundProject, China (Grant No. 4132031).

摘要/Abstract

摘要： The chemiluminescence (CL) performance of luminol is improved using reduced graphene oxide/gold nanoparticle (rGO-AuNP) nano-composites as catalyst. To prepare this catalyst, we propose a linker free, one-step method to in-situ synthesize rGO-AuNP nano-composites. Various measurements are utilized to characterize the resulting rGO-AuNP samples, and it is revealed that rGO could improve the stability and conductivity. Furthermore, we investigate the CL signals of luminal catalyzed by rGO-AuNP. Afterwards, the size effect of particle and the assisted enhancement effect of rGO are studied and discussed in detail. Based on the discussion, an optimal, sensitive and stable rGO-AuNP-luminon-H₂O₂ CL system is proposed. Finally, we utilize the system as a sensor to detect hydrogen peroxide and organic compounds containing amino, hydroxyl, or thiol groups. The CL system might provide a more attractive platform for various analytical devices with CL detection in the field of biosensors, bioassays, and immunosensors.

关键词: graphene, nanoparticles, chemiluminescence, biosensers

Abstract: The chemiluminescence (CL) performance of luminol is improved using reduced graphene oxide/gold nanoparticle (rGO-AuNP) nano-composites as catalyst. To prepare this catalyst, we propose a linker free, one-step method to in-situ synthesize rGO-AuNP nano-composites. Various measurements are utilized to characterize the resulting rGO-AuNP samples, and it is revealed that rGO could improve the stability and conductivity. Furthermore, we investigate the CL signals of luminal catalyzed by rGO-AuNP. Afterwards, the size effect of particle and the assisted enhancement effect of rGO are studied and discussed in detail. Based on the discussion, an optimal, sensitive and stable rGO-AuNP-luminon-H₂O₂ CL system is proposed. Finally, we utilize the system as a sensor to detect hydrogen peroxide and organic compounds containing amino, hydroxyl, or thiol groups. The CL system might provide a more attractive platform for various analytical devices with CL detection in the field of biosensors, bioassays, and immunosensors.

Key words: graphene, nanoparticles, chemiluminescence, biosensers

中图分类号: (Graphene)

81.05.ue

78.67.Bf (Nanocrystals, nanoparticles, and nanoclusters) 78.60.Ps (Chemiluminescence) 87.85.fk (Biosensors)

王闻硕, 何大伟, 王继红, 段嘉华, 彭洪尚, 吴洪鹏, 富鸣, 王永生, 张希清. An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application[J]. 中国物理B, 2014, 23(4): 48103-048103.

Wang Wen-Shuo (王闻硕), He Da-Wei (何大伟), Wang Ji-Hong (王继红), Duan Jia-Hua (段嘉华), Peng Hong-Shang (彭洪尚), Wu Hong-Peng (吴洪鹏), Fu Ming (富鸣), Wang Yong-Sheng (王永生), Zhang Xi-Qing (张希清). An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application[J]. Chin. Phys. B, 2014, 23(4): 48103-048103.

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An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application

An optimized, sensitive and stable reduced graphene oxide-gold nanoparticle-luminol-H₂O₂ chemiluminescence system and its potential analytical application

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