Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er0.01YbxY1 - 0.01 - xVO4 crystal

doi:10.1088/1674-1056/19/9/097804

中国物理B ›› 2010, Vol. 19 ›› Issue (9): 97804-097804.doi: 10.1088/1674-1056/19/9/097804

Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_{1 - 0.01 - x}VO₄ crystal

卢建¹, 张蕴芝¹, 冯宝华¹, 陈晓波², 徐小灵², 王策², 杨国建², Gregory J. Salamo³

(1)Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China; (2)Nuclear Science & Technology School and Analytical Testing Center, Applied Optics Beijing Area Major Laboratory, Beijing Normal University, Beijing 100875, China; (3)University Arkansas, Department of Physics, Fayetteville, AR 72701, USA

收稿日期:2009-08-03 修回日期:2010-03-21 出版日期:2010-09-15 发布日期:2010-09-15

Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_1-0.01-xVO₄ crystal

Chen Xiao-Bo(陈晓波)^{a) †}, Lu Jian(卢建)^b), Zhang Yun-Zhi(张蕴芝)^b), Xu Xiao-Ling(徐小灵)^a), Feng Bao-Hua(冯宝华)^b), Wang Ce(王策)^a), Gregory J. Salamo^c), and Yang Guo-Jian(杨国建)^a)

^a Nuclear Science & Technology School and Analytical Testing Center, Applied Optics Beijing Area Major Laboratory, Beijing Normal University, Beijing 100875, China; ^b Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China; ^c University Arkansas, Department of Physics, Fayetteville, AR 72701, USA

Received:2009-08-03 Revised:2010-03-21 Online:2010-09-15 Published:2010-09-15

摘要/Abstract

摘要： The improvement on the calculation of anti-Stokes energy transfer rate is studied in the present work. The additional proportion coefficient between Stokes and anti-Stokes light intensities of quantum Raman scattering theory as compared with the classical Raman theory is introduced to successfully describe the anti-Stokes energy transfer. The theoretical formula for the improvement on the calculation of anti-Stokes energy transfer rate is derived for the first time in this study. The correctness of introducing coefficient exp{ΔE / kT} from well-known Raman scatter theory is demonstrated also. Moreover, the experimental lifetime measurement in Er_0.01Yb_xY_{1 - 0.01 - x}VO₄ crystal is performed to justify the validity of our important improvement in the original phonon-assisted energy transfer theory for the first time.

Abstract: The improvement on the calculation of anti-Stokes energy transfer rate is studied in the present work. The additional proportion coefficient between Stokes and anti-Stokes light intensities of quantum Raman scattering theory as compared with the classical Raman theory is introduced to successfully describe the anti-Stokes energy transfer. The theoretical formula for the improvement on the calculation of anti-Stokes energy transfer rate is derived for the first time in this study. The correctness of introducing coefficient exp{ΔE / kT} from well-known Raman scatter theory is demonstrated also. Moreover, the experimental lifetime measurement in Er_0.01Yb_xY_1-0.01-xVO₄ crystal is performed to justify the validity of our important improvement in the original phonon-assisted energy transfer theory for the first time.

Key words: improvement of anti-Stokes energy transfer, Raman scattering quantum and classical theory, Er_0.01Yb_xY_1-0.01-xVO₄ crystal

中图分类号:

7855

陈晓波, 卢建, 张蕴芝, 徐小灵, 冯宝华, 王策, Gregory J. Salamo, 杨国建. Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_{1 - 0.01 - x}VO₄ crystal[J]. 中国物理B, 2010, 19(9): 97804-097804.

Chen Xiao-Bo(陈晓波), Lu Jian(卢建), Zhang Yun-Zhi(张蕴芝), Xu Xiao-Ling(徐小灵), Feng Bao-Hua(冯宝华), Wang Ce(王策), Gregory J. Salamo, and Yang Guo-Jian(杨国建) . Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_1-0.01-xVO₄ crystal[J]. Chin. Phys. B, 2010, 19(9): 97804-097804.

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Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_{1 - 0.01 - x}VO₄ crystal

Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er_0.01Yb_xY_1-0.01-xVO₄ crystal

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