Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8

doi:10.1088/1674-1056/ac81aa

中国物理B ›› 2023, Vol. 32 ›› Issue (5): 54208-054208.doi: 10.1088/1674-1056/ac81aa

Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8

Yuyi Zhang(张钰伊)¹, Yajie Bian(卞亚杰)¹, Wei Zhang(张炜)¹, Yiting Liu(刘易婷)¹, Xiaolei Zhang(张晓磊)^1,2,†, Mengdi Chen(陈梦迪)^1,‡, Bingwen Hu(胡炳文)¹, and Qingyuan Jin(金庆原)^1,3,§

1 State Key Laboratory of Precision Spectroscopy, Shanghai Key Laboratory of Magnetic Resonance, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China;
2 Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China;
3 Department of Optical Science and Engineering, Fudan University, Shanghai 200433, China

收稿日期:2022-05-28 修回日期:2022-07-14 接受日期:2022-07-18 出版日期:2023-04-21 发布日期:2023-05-09
通讯作者: Xiaolei Zhang, Mengdi Chen, Qingyuan Jin E-mail:xlzhang@admin.ecnu.edu.cn;mdchen@lps.ecnu.edu.cn;qyjin@fudan.edu.cn

Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8

1 State Key Laboratory of Precision Spectroscopy, Shanghai Key Laboratory of Magnetic Resonance, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China;
2 Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China;
3 Department of Optical Science and Engineering, Fudan University, Shanghai 200433, China

Received:2022-05-28 Revised:2022-07-14 Accepted:2022-07-18 Online:2023-04-21 Published:2023-05-09
Contact: Xiaolei Zhang, Mengdi Chen, Qingyuan Jin E-mail:xlzhang@admin.ecnu.edu.cn;mdchen@lps.ecnu.edu.cn;qyjin@fudan.edu.cn

1. 附件.pdf(114KB)

摘要/Abstract

摘要： Noble metal nanoparticles exhibit unique surface plasmon resonance dependent optical properties. On this basis, gold nanoparticles (AuNPs) encapsulated in metal-organic frameworks (MOFs) can form AuNPs@MOFs composites to modulate the optical properties of fluorescent molecules, which is less reported. In this paper, based on the fluorescence enhancement effect of AuNPs on 2-(2-hydroxyphenyl)-1H-benzimidazole (HPBI) molecules, zeolitic imidazolate framework-8 (ZIF-8) crystals with structural stability were introduced. AuNPs@ZIF-8 exhibited a significantly pronounced fluorescence enhancement of the HPBI molecules. In addition, by comparing the fluorescence characteristics of the HPBI molecules adsorbed on AuNPs@ZIF-8 and those captured in AuNPs@ZIF-8, we found that the ZIF-8 can act as a spacer layer with highly effective near-field enhancement. All our preliminary results shed light on future research on the composite structures of noble metal particles and MOFs for fluorescent probes and sensing applications.

关键词: ZIF-8, gold nanoparticles, fluorescence spectra, fluorescence lifetime

Abstract: Noble metal nanoparticles exhibit unique surface plasmon resonance dependent optical properties. On this basis, gold nanoparticles (AuNPs) encapsulated in metal-organic frameworks (MOFs) can form AuNPs@MOFs composites to modulate the optical properties of fluorescent molecules, which is less reported. In this paper, based on the fluorescence enhancement effect of AuNPs on 2-(2-hydroxyphenyl)-1H-benzimidazole (HPBI) molecules, zeolitic imidazolate framework-8 (ZIF-8) crystals with structural stability were introduced. AuNPs@ZIF-8 exhibited a significantly pronounced fluorescence enhancement of the HPBI molecules. In addition, by comparing the fluorescence characteristics of the HPBI molecules adsorbed on AuNPs@ZIF-8 and those captured in AuNPs@ZIF-8, we found that the ZIF-8 can act as a spacer layer with highly effective near-field enhancement. All our preliminary results shed light on future research on the composite structures of noble metal particles and MOFs for fluorescent probes and sensing applications.

Key words: ZIF-8, gold nanoparticles, fluorescence spectra, fluorescence lifetime

中图分类号: (Optical materials)

42.70.-a

Yuyi Zhang(张钰伊), Yajie Bian(卞亚杰), Wei Zhang(张炜), Yiting Liu(刘易婷), Xiaolei Zhang(张晓磊),Mengdi Chen(陈梦迪), Bingwen Hu(胡炳文), and Qingyuan Jin(金庆原). Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8[J]. 中国物理B, 2023, 32(5): 54208-054208.

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Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8

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