Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train

doi:10.1088/1674-1056/ab33f3

中国物理B ›› 2019, Vol. 28 ›› Issue (9): 93201-093201.doi: 10.1088/1674-1056/ab33f3

• ATOMIC AND MOLECULAR PHYSICS • 上一篇下一篇

Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train

Qiu-Nan Tong(佟秋男), De-Hou Fei(费德厚), Zhen-Zhong Lian(廉振中), Hong-Xia Qi(齐洪霞), Sheng-Peng Zhou(周胜鹏), Si-Zuo Luo(罗嗣佐), Zhou Chen(陈洲), Zhan Hu(胡湛)

1 Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China;
2 Advanced Light Field and Modern Medical Treatment Science and Technology Innovation Center of Jilin Province, Jilin University, Changchun 130012, China

收稿日期:2019-04-30 修回日期:2019-06-25 出版日期:2019-09-05 发布日期:2019-09-05
通讯作者: Zhou Chen, Zhou Chen E-mail:phy_cz@jlu.edu.cn;huzhan@jlu.edu.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant No. 11374124).

Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train

Qiu-Nan Tong(佟秋男)^1,2, De-Hou Fei(费德厚)^1,2, Zhen-Zhong Lian(廉振中)^1,2, Hong-Xia Qi(齐洪霞)^1,2, Sheng-Peng Zhou(周胜鹏)¹, Si-Zuo Luo(罗嗣佐)¹, Zhou Chen(陈洲)^1,2, Zhan Hu(胡湛)^1,2

1 Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China;
2 Advanced Light Field and Modern Medical Treatment Science and Technology Innovation Center of Jilin Province, Jilin University, Changchun 130012, China

Received:2019-04-30 Revised:2019-06-25 Online:2019-09-05 Published:2019-09-05
Contact: Zhou Chen, Zhou Chen E-mail:phy_cz@jlu.edu.cn;huzhan@jlu.edu.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant No. 11374124).

摘要/Abstract

摘要：

Coherent control of fragmentation of CH₃I using shaped femtosecond pulse train is investigated. The dissociation processes can be modulated by changing the separation of the shaped pulse train, and the yield of I⁺ under the irradiation of the optimal pulse is significantly increased compared with that using the transform-limited pulse. We discuss the control mechanism of dissociation processes with coherent interference in time domain. A three-pulse control model is proposed to explain the counterintuitive experimental results.

关键词: coherent control, fragmentation, shaped pulse

Abstract:

Key words: coherent control, fragmentation, shaped pulse

中图分类号: (Multiphoton ionization and excitation to highly excited states)

32.80.Rm

42.50.Hz (Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift)

佟秋男, 费德厚, 廉振中, 齐洪霞, 周胜鹏, 罗嗣佐, 陈洲, 胡湛. Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train[J]. 中国物理B, 2019, 28(9): 93201-093201.

Qiu-Nan Tong(佟秋男), De-Hou Fei(费德厚), Zhen-Zhong Lian(廉振中), Hong-Xia Qi(齐洪霞), Sheng-Peng Zhou(周胜鹏), Si-Zuo Luo(罗嗣佐), Zhou Chen(陈洲), Zhan Hu(胡湛). Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train[J]. Chin. Phys. B, 2019, 28(9): 93201-093201.

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Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train

Coherent control of fragmentation of methyl iodide by shaped femtosecond pulse train

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