Structural evolution of silicone oil liquid exposed to Ar plasma

doi:10.1088/1674-1056/19/6/065205

中国物理B ›› 2010, Vol. 19 ›› Issue (6): 65205-065205.doi: 10.1088/1674-1056/19/6/065205

Structural evolution of silicone oil liquid exposed to Ar plasma

袁圆, 叶超, 黄宏伟, 施国峰, 宁兆元

School of Physics Science and Technology, Jiangsu Key Laboratory of Thin Films, Soochow University, Suzhou 215006, China

收稿日期:2009-11-09 出版日期:2010-06-15 发布日期:2010-06-15
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos. 10975105, 10575074 and 10635010).

Structural evolution of silicone oil liquid exposed to Ar plasma

Yuan Yuan(袁圆), Ye Chao(叶超)^†, Huang Hong-Wei(黄宏伟), Shi Guo-Feng(施国峰), and Ning Zhao-Yuan(宁兆元)

School of Physics Science and Technology, Jiangsu Key Laboratory of Thin Films, Soochow University, Suzhou 215006, China

Received:2009-11-09 Online:2010-06-15 Published:2010-06-15
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 10975105, 10575074 and 10635010).

摘要/Abstract

摘要： Structure properties of silicone oil serving as a liquid substrate exposed to Ar plasma are investigated in this paper. Under the action of energetic Ar ions, the surface of silicone oil liquid substrate exhibits a branch-like fractal aggregation structure, which is related to the structure evolution of silicone oil liquid from Si--O chain to Si--O network. The radicals from the dissociation of silicone oil molecule into the Ar plasma turns the plasma into a reactive environment. Therefore, the structural evolution of silicone oil liquid substrate and the reactive radicals in the plasma space become possible factors to affect the aggregation of nanoparticles and also the structures and the compositions of nanoparticles.

Abstract: Structure properties of silicone oil serving as a liquid substrate exposed to Ar plasma are investigated in this paper. Under the action of energetic Ar ions, the surface of silicone oil liquid substrate exhibits a branch-like fractal aggregation structure, which is related to the structure evolution of silicone oil liquid from Si--O chain to Si--O network. The radicals from the dissociation of silicone oil molecule into the Ar plasma turns the plasma into a reactive environment. Therefore, the structural evolution of silicone oil liquid substrate and the reactive radicals in the plasma space become possible factors to affect the aggregation of nanoparticles and also the structures and the compositions of nanoparticles.

Key words: silicone oil liquid substrate, structure evolution, Ar plasma

中图分类号: (Molecular liquids)

61.25.Em

82.30.Lp (Decomposition reactions (pyrolysis, dissociation, and fragmentation)) 61.46.Df (Structure of nanocrystals and nanoparticles ("colloidal" quantum dots but not gate-isolated embedded quantum dots))

袁圆, 叶超, 黄宏伟, 施国峰, 宁兆元. Structural evolution of silicone oil liquid exposed to Ar plasma[J]. 中国物理B, 2010, 19(6): 65205-065205.

Yuan Yuan(袁圆), Ye Chao(叶超), Huang Hong-Wei(黄宏伟), Shi Guo-Feng(施国峰), and Ning Zhao-Yuan(宁兆元). Structural evolution of silicone oil liquid exposed to Ar plasma[J]. Chin. Phys. B, 2010, 19(6): 65205-065205.

参考文献 24

[1]	Torimoto T, Okazaki K, Kiyama T, Hirahara K, Tanaka N and Kuwabata S 2006 Appl. Phys. Lett. 89 243117
[2]	Ye G X, Michely T, Weidenhof V, Friedrich I and Wuttig M 1998 Phys. Rev. Lett. 81 622
[3]	Wagener M and Gunther B 1999 J. Magn. Magn. Mater. 201 41
[4]	Ye Q L, Feng C M, Xu X J, Jin J S, Xia A G and Ye G X 2005 J. Appl. Phys. 98 013906
[5]	Zhang Y J, Yu S J, Ge H L, Wu L N and Cui Y J 2006 Acta Phys. Sin. 55 5444 (in Chinese)
[6]	Mao M, Wang S, Dai Z L and Wang Y N 2007 Chin. Phys. 16 2044
[7]	Xu X, Li L S, Liu F, Zhou Q H and Liang R Q 2008 Chin. Phys. B 17 4242
[8]	Ji H H, Yu M, Ren L M, Zhang X, Huang R and Zhang Y G 2008 Chin. Phys. B 17 3428
[9]	Wu J, Zhang P Y, Sun J Z, Zhang J, Ding Z F and Wang D Z 2008 Chin. Phys. B 17 1848
[10]	Ye C, Ning Z Y, Shen M R, Wang H and Gan Z Q 1997 Appl. Phys. Lett. 71 336
[11]	Ye C, Ning Z Y, Shen M R, Cheng S H and Gan Z Q 1998 J. Appl. Phys. 83 5978
[12]	Zhou N N 2000 Introduction of Organosilicon Polymer (Beijing: Science Press) (in Chinese)
[13]	Xu Y J, Ye C, Huang X J, Yuan J, Xing Z Y and Ning Z Y 2008 Chin. Phys. Lett. 25 2942
[14]	Georgieva V and Bogaerts A 2005 J. Appl. Phys. 98 023308
[15]	Li X S, Bi Z H, Chang D L, Li Z C, Wang S, Xu X, Xu Y, Lu W Q, Zhu A M and Wang Y N 2008 Appl. Phys. Lett. 93 031504
[16]	Jones R A L 2008 Soft Condensed Matter (Beijing: Science Press)
[17]	Ke Y K and Dong H R 1998 Handbook of Analytical Chemistry: Optical Spectroscopy Analysis (2nd edition) (Beijing: Chemical Industry Press) (in Chinese)
[18]	Hsiao H L, Hwang H L, Yang A B, Chen L W and Yew T R 1999 Appl. Surf. Sci. 142 316
[19]	Kholodkov A V, Golant K M and Nikolin I V 2003 Microelectron. Eng. 69 365
[20]	Clay K J, Speakman S P, Amaratunga G A J and Silva S R P 1996 J. Appl. Phys. 79 7227
[21]	Escobar-Alarón L, Camps E, Haro-Poniatowski E, Villagran M and Sanchez C 2002 Appl. Surf. Sci. 197--198 192
[22]	Samukawa S and Furuoya S 1993 Appl. Phys. Lett. 63 2044
[23]	Nicolazo F, Goullet A, Granier A, Vallé e C, Turban G and Grolleau B 1998 Surf. Coat. Technol. 98 1578
[24]	Zambrano G, Riascos H, Prieto P, Restrepo E, Devia A and Rinón C 2003 Surf. Coat. Technol. 172 144

Structural evolution of silicone oil liquid exposed to Ar plasma

Structural evolution of silicone oil liquid exposed to Ar plasma

PDF (PC)

赞

可视化

摘要/Abstract

引用本文

使用本文

参考文献 24

相关文章 12

Metrics

本文评价

推荐阅读 0

[1]	李明儒, 张楠, 张丰收. A simulation study of water property changes using geometrical alteration in SPC/E[J]. 中国物理B, 2018, 27(8): 83103-083103.
[2]	王畅, 吴红琳, 宋云飞, 杨延强. Structural deformation of nitro group of nitromethane molecule in liquid phase in an intense femtosecond laser field[J]. 中国物理B, 2017, 26(9): 94208-094208.
[3]	王畅, 吴红琳, 宋云飞, 何兴, 杨延强, 谭多旺. Tracking molecular structure deformation of nitrobenzene and its torsion vibration coupling by intense pumping CARS[J]. 中国物理B, 2016, 25(11): 114210-114210.
[4]	吴红琳, 宋云飞, 于国洋, 杨延强. Transient grating study of the intermolecular dynamics of liquid nitrobenzene[J]. 中国物理B, 2016, 25(10): 107802-107802.
[5]	欧阳顺利, 吴楠楠, 刘靖尧, 孙成林, 里佐威, 高淑琴. Investigation of hydrogen bonding in neat dimethyl sulfoxide and binary mixture (dimethyl sulfoxide + water) by concentration-dependent Raman study and ab initio calculation[J]. 中国物理B, 2010, 19(12): 123101-123101.
[6]	蒋秀兰, 杨光, 李东飞, 周密, 孙成林, 高淑琴, 里佐威. Influence of pressure effect on Fermi resonance in binary solution[J]. 中国物理B, 2010, 19(10): 103301-103301.
[7]	房文汇, 门志伟, 孙成林, 曲冠男, 杨光, 里佐威, 高淑琴, 陆国会. Study of second-order nonlinear hyperpolarisability of all-trans-β-carotene in solutions by linear spectroscopic technique[J]. 中国物理B, 2010, 19(6): 64213-064213.
[8]	刘伟龙, 王德敏, 郑植仁, 李艾华, 苏文辉. Solvent effects on the S₀→S₂ absorption spectra of β-carotene[J]. 中国物理B, 2010, 19(1): 13102-013102.
[9]	曹达鹏, 程礼盛, 汪文川. Density functional theory for molecular orientation of hard rod fluids in hard slits[J]. 中国物理B, 2007, 16(8): 2296-2303.
[10]	周晓艳, 陆杭军. The structure and dynamics of water inside armchair carbon nanotube[J]. 中国物理B, 2007, 16(2): 335-339.
[11]	刘长松, 梁云峰, 朱震刚, 黎光旭. A molecular level study of liquid water with a flexible water model[J]. 中国物理B, 2005, 14(4): 785-790.
[12]	朱俊, 芶清泉. CALCULATION OF HIGHLY EXCITED VIBRATIONAL ENERGY LEVELS OF CH₃CN MOLECULE BY NON-LINEAR QUANTUM THEORY[J]. 中国物理B, 1999, 8(6): 430-433.