Efficiently enhanced energy storage performance of Ba2Bi4Ti5O18 film by co-doping Fe3+ and Ta5+ ion with larger radius

doi:10.1088/1674-1056/ac5393

中国物理B ›› 2022, Vol. 31 ›› Issue (9): 97701-097701.doi: 10.1088/1674-1056/ac5393

Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius

Qiong Wu(吴琼), Lei Zhao(赵雷), Xinghao Chen(陈兴豪), and Shifeng Zhao(赵世峰)^†

Inner Mongolia Key Laboratory of Nanoscience and Nanotechnology, &School of Physical Science and Technology, Inner Mongolia University, Hohhot 010021, China

收稿日期:2021-11-26 修回日期:2022-01-17 接受日期:2022-02-10 出版日期:2022-08-19 发布日期:2022-08-24
通讯作者: Shifeng Zhao E-mail:zhsf@imu.edu.cn
基金资助:
This work was financially supported by the National Natural Science Foundation of China (Grant Nos. 12074204, 11864028, and 11904054) and the Natural Science Foundation of Inner Mongolia, China (Grant No. 2022ZD06).

Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius

Qiong Wu(吴琼), Lei Zhao(赵雷), Xinghao Chen(陈兴豪), and Shifeng Zhao(赵世峰)^†

Inner Mongolia Key Laboratory of Nanoscience and Nanotechnology, &School of Physical Science and Technology, Inner Mongolia University, Hohhot 010021, China

Received:2021-11-26 Revised:2022-01-17 Accepted:2022-02-10 Online:2022-08-19 Published:2022-08-24
Contact: Shifeng Zhao E-mail:zhsf@imu.edu.cn
Supported by:
This work was financially supported by the National Natural Science Foundation of China (Grant Nos. 12074204, 11864028, and 11904054) and the Natural Science Foundation of Inner Mongolia, China (Grant No. 2022ZD06).

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摘要/Abstract

摘要： We present an efficient strategy, that is the co-substitution of Fe³⁺ and Ta⁵⁺ ions with large radius for Ti⁴⁺ ion, to enhance energy storage performance of Ba₂Bi₄Ti₅O₁₈ film. For the films co-doped with Fe³⁺ and Ta⁵⁺ ions, the maximum polarization under the same external electric field is improved because the radius of Fe³⁺ and Ta⁵⁺ ions is larger than that of Ti⁴⁺ ion. Moreover, due to the composition and chemical disorder, the relaxor properties are also slightly improved, which can not be achieved by the film doped with Fe³⁺ ions only. What is more, for the films doped with Fe³⁺ ion only, the leakage current density increases greatly due to the charge imbalance, resulting in a significant decrease in breakdown strength. It is worth mentioning that the breakdown strength of Fe³⁺ and Ta⁵⁺ ions co-doped film does not decrease due to the charge balance. Another important point is the recoverable energy storage density of the films co-doped with Fe³⁺ and Ta⁵⁺ ions has been greatly improved based on the fact that the maximum external electric field does not decrease and the maximum polarization under the same external electric field increases. On top of that, the hysteresis of the polarization has also been improved. Finally, the co-doped films with Fe³⁺ and Ta⁵⁺ ions have good frequency and temperature stability.

关键词: Ba₂Bi₄Ti₅O₁₈ film, ferroelectrics, energy storage, co-doped, radius

Abstract: We present an efficient strategy, that is the co-substitution of Fe³⁺ and Ta⁵⁺ ions with large radius for Ti⁴⁺ ion, to enhance energy storage performance of Ba₂Bi₄Ti₅O₁₈ film. For the films co-doped with Fe³⁺ and Ta⁵⁺ ions, the maximum polarization under the same external electric field is improved because the radius of Fe³⁺ and Ta⁵⁺ ions is larger than that of Ti⁴⁺ ion. Moreover, due to the composition and chemical disorder, the relaxor properties are also slightly improved, which can not be achieved by the film doped with Fe³⁺ ions only. What is more, for the films doped with Fe³⁺ ion only, the leakage current density increases greatly due to the charge imbalance, resulting in a significant decrease in breakdown strength. It is worth mentioning that the breakdown strength of Fe³⁺ and Ta⁵⁺ ions co-doped film does not decrease due to the charge balance. Another important point is the recoverable energy storage density of the films co-doped with Fe³⁺ and Ta⁵⁺ ions has been greatly improved based on the fact that the maximum external electric field does not decrease and the maximum polarization under the same external electric field increases. On top of that, the hysteresis of the polarization has also been improved. Finally, the co-doped films with Fe³⁺ and Ta⁵⁺ ions have good frequency and temperature stability.

Key words: Ba₂Bi₄Ti₅O₁₈ film, ferroelectrics, energy storage, co-doped, radius

中图分类号: (Ferroelectricity and antiferroelectricity)

77.80.-e

68.55.-a (Thin film structure and morphology) 84.60.Ve (Energy storage systems, including capacitor banks)

Qiong Wu(吴琼), Lei Zhao(赵雷), Xinghao Chen(陈兴豪), and Shifeng Zhao(赵世峰)^†. Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius[J]. 中国物理B, 2022, 31(9): 97701-097701.

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Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius

Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius

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