Morphological modifications of C60 crystal rods under hydrothermal conditions

doi:10.1088/1674-1056/abc0d8

中国物理B ›› 2020, Vol. 29 ›› Issue (12): 128102-.doi: 10.1088/1674-1056/abc0d8

收稿日期:2020-06-08 修回日期:2020-08-28 接受日期:2020-10-14 出版日期:2020-12-01 发布日期:2020-11-13

Morphological modifications of C₆₀ crystal rods under hydrothermal conditions

Ming-Run Du(杜明润)¹, Shi-Xin Liu(刘士鑫)¹, Jia-Jun Dong(董家君)², Ze-Peng Li(李泽朋)^1,†, Ming-Chao Wang (王明超)¹, Tong Wei(魏通)¹, Qing-Jun Zhou(周青军)¹, Xiong Yang(杨雄)¹, and Peng-fei Shen(申鹏飞)³

¹ College of Science, Civil Aviation University of China, Tianjin 300300, China; ² State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, China; ³ Academy for Advanced Interdisciplinary Studies, Southern University of Science and Technology, Shenzhen 519055, China

Received:2020-06-08 Revised:2020-08-28 Accepted:2020-10-14 Online:2020-12-01 Published:2020-11-13
Contact: ^†Corresponding author. E-mail: li_zepeng@163.com
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11804384, 51802343, and 51772326), the Fundamental Research Funds for the Central Universities, China (Grant No. 3122018L006), the Scientific Research Project of Tianjin Education Commission (Grant No. 2019ZD19), the National Natural Science Foundation of China and the Civil Aviation Administration of China (Grant No. U1933109), and Open Project of State Key Laboratory of Superhard Materials (Jilin University) (Grant No. 201803).

1. Supporting Information.pdf(634KB)

摘要/Abstract

Abstract: We observed morphological modification of rod-shaped C₆₀ solvate crystals using a facile hydrothermal method. The initial C₆₀ rods were changed from smooth rods to rough rods, porous rods or pieces under different hydrothermal conditions. During the hydrothermal treatment, the initial samples underwent a decomposition-recrystallization process, which can be tuned by the content of alcohol in the hydrothermal solution, thereby leading to modification of the morphological properties of the initial C₆₀ rods. In addition, the rough and porous C₆₀ rods prepared in our work exhibit excellent photoluminescence intensities that are approximately 7 and 3 times higher than those of pure C₆₀ powders, respectively. Our results suggest that the hydrothermal method is a potential route for fabricating fullerene materials with controllable morphologies and novel functions.

Key words: fullerene crystals, morphological modification, porous materials, hydrothermal method

中图分类号: (Fullerenes and related materials)

81.05.ub

81.10.-h (Methods of crystal growth; physics and chemistry of crystal growth, crystal morphology, and orientation) 81.05.Rm (Porous materials; granular materials) 61.48.-c (Structure of fullerenes and related hollow and planar molecular structures)

. [J]. 中国物理B, 2020, 29(12): 128102-.

Ming-Run Du(杜明润), Shi-Xin Liu(刘士鑫), Jia-Jun Dong(董家君), Ze-Peng Li(李泽朋), Ming-Chao Wang (王明超), Tong Wei(魏通), Qing-Jun Zhou(周青军), Xiong Yang(杨雄), and Peng-fei Shen(申鹏飞). Morphological modifications of C₆₀ crystal rods under hydrothermal conditions[J]. Chin. Phys. B, 2020, 29(12): 128102-.

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Morphological modifications of C₆₀ crystal rods under hydrothermal conditions

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