Resolving multi-orbital effects on high harmonic generation from aligned N2 molecules in linearly and elliptically polarized intense laser fields

doi:10.1088/1674-1056/ab3440

中国物理B ›› 2019, Vol. 28 ›› Issue (9): 94211-094211.doi: 10.1088/1674-1056/ab3440

• ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS • 上一篇下一篇

Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields

Hong-Jing Liang(梁红静), Xin Fan(范鑫), Shuang Feng(冯爽), Li-Yu Shan(单立宇), Qing-Hua Gao(高庆华), Bo Yan(闫博), Ri Ma(马日), Hai-Feng Xu(徐海峰), Da-Jun Ding(丁大军)

Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China

收稿日期:2019-05-15 修回日期:2019-07-02 出版日期:2019-09-05 发布日期:2019-09-05
通讯作者: Ri Ma E-mail:rma@jlu.edu.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos. 91750104, 11127403, and 11474130) and the Natural Science Foundation of Jilin Province, China (Grant No. 20160101332JC).

Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields

Hong-Jing Liang(梁红静), Xin Fan(范鑫), Shuang Feng(冯爽), Li-Yu Shan(单立宇), Qing-Hua Gao(高庆华), Bo Yan(闫博), Ri Ma(马日), Hai-Feng Xu(徐海峰), Da-Jun Ding(丁大军)

Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China

Received:2019-05-15 Revised:2019-07-02 Online:2019-09-05 Published:2019-09-05
Contact: Ri Ma E-mail:rma@jlu.edu.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 91750104, 11127403, and 11474130) and the Natural Science Foundation of Jilin Province, China (Grant No. 20160101332JC).

摘要/Abstract

摘要：

We perform an experimental study of the multi-orbital effect on the high-order harmonic generation (HHG) from aligned N₂ molecules in both linearly and elliptically polarized intense laser fields. Measured by a home-built extreme ultraviolet (XUV) flat grating spectrometer with the pump-probe method, the angular distributions of different orders of HHG are obtained, which show distinctive behaviors for harmonics in the plateau and the cut-off regions. The ellipticity dependence of HHG is investigated by aligning the molecular axis parallel or perpendicular to the laser polarization. Our results indicate that both the highest occupied molecular orbital (HOMO) as well as the lower one (HOMO-1) contribute to the HHG of N₂ molecules, in either linearly or elliptically polarized intense laser field. The study paves the way for understanding the ultrafast electron dynamics of molecules exposed to an intense laser field.

关键词: high-order harmonic generation, aligned molecule, multi-orbital effect, elliptically polarized intense laser

Abstract:

Key words: high-order harmonic generation, aligned molecule, multi-orbital effect, elliptically polarized intense laser

中图分类号: (Frequency conversion; harmonic generation, including higher-order harmonic generation)

42.65.Ky

33.20.Xx (Spectra induced by strong-field or attosecond laser irradiation) 33.80.Rv (Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states))

梁红静, 范鑫, 冯爽, 单立宇, 高庆华, 闫博, 马日, 徐海峰, 丁大军. Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields[J]. 中国物理B, 2019, 28(9): 94211-094211.

Hong-Jing Liang(梁红静), Xin Fan(范鑫), Shuang Feng(冯爽), Li-Yu Shan(单立宇), Qing-Hua Gao(高庆华), Bo Yan(闫博), Ri Ma(马日), Hai-Feng Xu(徐海峰), Da-Jun Ding(丁大军). Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields[J]. Chin. Phys. B, 2019, 28(9): 94211-094211.

参考文献 41

[40]	Lu T and Chen F 2012 J. Comput. Chem. 33 580 doi: 10.1002/jcc.22885
[1]	Frassetto F, Cacho C, Froud C A, Turcu I C E, Villoresi P, Bryan W A, Springate E and Poletto L 2011 Opt. Express 19 19169 doi: 10.1364/OE.19.019169
[41]	Möller M, Cheng Y, Khan S D, Zhao B, Zhao K, Chini M, Paulus G G and Chang Z 2012 Phys. Rev. A 86 011401 doi: 10.1103/PhysRevA.86.011401
[2]	Dakovski G L, Li Y, Durakiewicz T and Rodriguez G 2010 Rev. Sci. Instrum. 81 073108 doi: 10.1063/1.3460267
[3]	Sansone G, Benedetti E, Calegari F, Vozzi C, Avaldi L, Flammini R, Poletto L, Villoresi P, Altucci C, Velotta R, Stagira S, De Silvestri S and Nisoli M 2006 Science 314 443 doi: 10.1126/science.1132838
[4]	Zhao K, Zhang Q, Chini M, Wu Y, Wang X and Chang Z 2012 Opt. Lett. 37 3891 doi: 10.1364/OL.37.003891
[5]	Zou P, Zeng Z N, Zheng Y H, Lu Y Y, Liu P, Li R X and Xu Z Z 2010 Phys. Rev. A 81 033428 doi: 10.1103/PhysRevA.81.033428
[6]	Zhang H D, Guo J, Shi Y, Du H, Liu H F, Huang X R, Liu X S and Jing J 2017 Chin. Phys. Lett. 34 014206 doi: 10.1088/0256-307X/34/1/014206
[7]	Xia C L and Miao X Y 2015 Chin. Phys. Lett. 32 043202 doi: 10.1088/0256-307X/32/4/043202
[8]	Lewenstein M, Balcou P, Ivanov M Y, L'Huillier A and Corkum P B 1994 Phys. Rev. A 49 2117 doi: 10.1103/PhysRevA.49.2117
[9]	Corkum P B 1993 Phys. Rev. Lett. 71 1994 doi: 10.1103/PhysRevLett.71.1994
[10]	Schafer K J, Yang B, DiMauro L F and Kulander K C 1993 Phys. Rev. Lett. 70 1599 doi: 10.1103/PhysRevLett.70.1599
[11]	Rupenyan A, Kraus P M, Schneider J and Wörner H J 2013 Phys. Rev. A 87 31401 doi: 10.1103/PhysRevA.87.031401
[12]	Smirnova O, Mairesse Y, Patchkovskii S, Dudovich N, Villeneuve D, Corkum P and Ivanov M Y 2009 Nature 460 972 doi: 10.1038/nature08253
[13]	Zhang B, Zhao J and Zhao Z X 2018 Chin. Phys. Lett. 35 043201 doi: 10.1088/0256-307X/35/4/043201
[14]	Wong M C H, Le A T, Alharbi A F, Boguslavskiy A E, Lucchese R R, Brichta J P, Lin C D and Bhardwaj V R 2013 Phys. Rev. Lett. 110 033006 doi: 10.1103/PhysRevLett.110.033006
[15]	Bertrland J B, Wörner H J, Hockett P, Villeneuve D M and Corkum P B 2012 Phys. Rev. Lett. 109 143001 doi: 10.1103/PhysRevLett.109.143001
[16]	Kanai T, Minemoto S and Sakai H 2005 Nature 435 470 doi: 10.1038/nature03577
[17]	Vozzi C, Calegari F, Benedetti E, Caumes J P, Sansone G, Stagira S, Nisoli M, Torres R, Heesel E, Kajumba N, Marangos J P, Altucci C and Velotta R 2005 Phys. Rev. Lett. 95 153902 doi: 10.1103/PhysRevLett.95.153902
[18]	Chen Y J, Liu J and Hu B 2009 Phys. Rev. A 79 033405 doi: 10.1103/PhysRevA.79.033405
[19]	Lein M, Hay N, Velotta R, Marangos J P and Knight P L 2002 Phys. Rev. Lett. 88 183903 doi: 10.1103/PhysRevLett.88.183903
[20]	Zhou X X, Tong X M, Zhao Z X and Lin C D 2005 Phys. Rev. A 71 061801 doi: 10.1103/PhysRevA.71.061801
[21]	Li J W, Liu P, Yang H, Song L W, Zhao S T, Lu H, Li R X and Xu Z Z 2013 Opt. Express 21 7599 doi: 10.1364/OE.21.007599
[22]	Li G H, Xie H Q, Yao J P, Chu W, Cheng Y, Liu X J, Chen J and Xie X H 2016 Acta Phys. Sin. 65 224208(in Chinese)
[23]	Nalda R D, Heesel E, Lein M, Hay N, Velotta R, Springate E, Castillejo M and Marangos J 2004 Phys. Rev. A 69 031804 doi: 10.1103/PhysRevA.69.031804
[24]	Shan B, Ghimire S and Chang Z 2004 Phys. Rev. A 69 021404 doi: 10.1103/PhysRevA.69.021404
[25]	Torres R, Siegel T, Brugnera L, Procino I, Underwood J G, Altucci C, Velotta R, Springate E, Froud C, Turcu I C E, Yu M, Smirnova O and Marangos J P 2010 Opt. Express 18 3174 doi: 10.1364/OE.18.003174
[26]	Negro M, Devetta M, Faccialá D, De Silvestri S, Vozzi C and Stagira S 2014 Faraday Discuss. 171 133 doi: 10.1039/C4FD00033A
[27]	Torres R, Kajumba N, Underwood J G, Robinson J S, Baker S, Tisch J W G, de R, Bryan W A, Velotta R, Altucci C, Turcu I C E and Marangos J P 2007 Phys. Rev. Lett. 98 203007 doi: 10.1103/PhysRevLett.98.203007
[28]	McFarland B K, Farrell J P, Bucksbaum P H and Gühr M 2008 Science 322 1232 doi: 10.1126/science.1162780
[29]	Le A T, Lucchese R R and Lin C D 2009 J. Phys. B 42 211001 doi: 10.1088/0953-4075/42/21/211001
[30]	Diveki Z, Camper A, Haessler S, Auguste T, Ruchon T, Carré B, Saliéres P, Guichard R, Caillat J, Maquet A and Taïeb R 2012 New J. Phys. 14 023062 doi: 10.1088/1367-2630/14/2/023062
[31]	Troå J, Ren X, Makhija V, Mondal S, Kumarappan V and Trallero-Herrero C A 2017 Phys. Rev. A 95 033419 doi: 10.1103/PhysRevA.95.033419
[32]	Niu Y, Liang H J, Liu Y, Liu F Y, Ma R and Ding D J 2017 Chin. Phys. B 26 074222 doi: 10.1088/1674-1056/26/7/074222
[33]	Niu Y, Liu F Y, Liu Y, Liang H J, Yang Y J, Ma R and Ding D J 2017 Opt. Comm. 397 118 doi: 10.1016/j.optcom.2017.03.059
[34]	Liang H J, Wang Q X, Fan X, Shan L Y, Feng S, Yan B, Ma R and Xu H F 2018 Chin. J. Chem. Phys. 31 471 doi: 10.1063/1674-0068/31/cjcp1805117
[35]	Krause J L, Schafer K J and Kulander K C 1992 Phys. Rev. Lett. 68 3535 doi: 10.1103/PhysRevLett.68.3535
[36]	Stapelfeldt H and Seideman T 2003 Rev. Mod. Phys. 75 543 doi: 10.1103/RevModPhys.75.543
[37]	Miyazaki K, Kaku M, Miyaji G, Abdurrouf A and Faisal F H M 2005 Phys. Rev. Lett. 95 243903 doi: 10.1103/PhysRevLett.95.243903
[38]	Seideman T and Hamilton E 2005 Adv. At. Mol. Opt. Phys. 52 289 doi: 10.1016/S1049-250X(05)52006-8
[39]	Frisch M J, Trucks G W, Schlegel H B, et al. 2004 Gaussian 03 Revision E.01 (Wallingford CT:Gaussian Inc.)
[40]	Lu T and Chen F 2012 J. Comput. Chem. 33 580 doi: 10.1002/jcc.22885
[41]	Möller M, Cheng Y, Khan S D, Zhao B, Zhao K, Chini M, Paulus G G and Chang Z 2012 Phys. Rev. A 86 011401 doi: 10.1103/PhysRevA.86.011401

Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields

Resolving multi-orbital effects on high harmonic generation from aligned N₂ molecules in linearly and elliptically polarized intense laser fields

RichHTML

PDF (PC)

赞

可视化

摘要/Abstract

引用本文

使用本文

参考文献 41

相关文章 15

Metrics

本文评价

推荐阅读 0

[1]	Chang-Tong Liang(梁畅通), Jing-Jing Zhang(张晶晶), and Peng-Cheng Li(李鹏程). Phase-coherence dynamics of frequency-comb emission via high-order harmonic generation in few-cycle pulse trains[J]. 中国物理B, 2023, 32(3): 33201-033201.
[2]	Dong-Dong Cao(曹冬冬), Xue-Fei Pan(潘雪飞), Jun Zhang(张军), and Xue-Shen Liu(刘学深). Spectral shift of solid high-order harmonics from different channels in a combined laser field[J]. 中国物理B, 2023, 32(3): 34204-034204.
[3]	Shu-Shan Zhou(周书山), Yu-Jun Yang(杨玉军), Yang Yang(杨扬), Ming-Yue Suo(索明月), Dong-Yuan Li(李东垣), Yue Qiao(乔月), Hai-Ying Yuan(袁海颖), Wen-Di Lan(蓝文迪), and Mu-Hong Hu(胡木宏). High-order harmonic generation of the cyclo[18]carbon molecule irradiated by circularly polarized laser pulse[J]. 中国物理B, 2023, 32(1): 13201-013201.
[4]	Yanbo Chen(陈炎波), Baochang Li(李保昌), Xuhong Li(李胥红), Xiangyu Tang(唐翔宇), Chi Zhang(张弛), and Cheng Jin(金成). Effect of laser focus in two-color synthesized waveform on generation of soft x-ray high harmonics[J]. 中国物理B, 2023, 32(1): 14203-014203.
[5]	Long Lin(林龙), Tong-Gang Jia(贾铜钢), Zhi-Bin Wang(王志斌), and Peng-Cheng Li(李鹏程). Probing subcycle spectral structures and dynamics of high-order harmonic generation in crystals[J]. 中国物理B, 2022, 31(9): 93202-093202.
[6]	Yue Qiao(乔月), Jun Wang(王俊), Yan Yan(闫妍), Simeng Song(宋思蒙), Zhou Chen(陈洲), Aihua Liu(刘爱华), Jigen Chen(陈基根), Fuming Guo(郭福明), and Yujun Yang(杨玉军). Tunable spectral shift of high-order harmonic generation in atoms using a sinusoidally phase-modulated pulse[J]. 中国物理B, 2022, 31(6): 64214-064214.
[7]	Cai-Ping Zhang(张彩萍) and Xiang-Yang Miao(苗向阳). Decoding the electron dynamics in high-order harmonic generation from asymmetric molecular ions in elliptically polarized laser fields[J]. 中国物理B, 2022, 31(4): 43301-043301.
[8]	Yueying Liang(梁玥瑛), Xinkui He(贺新奎), Kun Zhao(赵昆), Hao Teng(滕浩), and Zhiyi Wei(魏志义). Enhancement of isolated attosecond pulse generation by using long gas medium[J]. 中国物理B, 2022, 31(4): 43302-043302.
[9]	Fan Yang(杨帆), Yinghui Zheng(郑颖辉), Luyao Zhang(张路遥), Xiaochun Ge(葛晓春), and Zhinan Zeng(曾志男). Orientation and ellipticity dependence of high-order harmonic generation in nanowires[J]. 中国物理B, 2022, 31(4): 44204-044204.
[10]	Dong Tang(唐栋) and Xue-Bin Bian(卞学滨). Multiple collisions in crystal high-order harmonic generation[J]. 中国物理B, 2022, 31(12): 123202-123202.
[11]	Bo Yan(闫博), Yi-Chen Wang(王一琛), Qing-Hua Gao(高庆华), Fang-Jing Cheng(程方晶), Qiu-Shuang Jing(景秋霜), Hong-Jing Liang(梁红静), and Ri Ma(马日). Minimum structure of high-harmonic spectrafrom aligned O₂ and N₂ molecules[J]. 中国物理B, 2021, 30(11): 114213-114213.
[12]	申许许, 王俊, 郭福明, 陈基根, 杨玉军. Role of potential on high-order harmonic generation from atoms irradiated by bichromatic counter-rotating circularly polarized laser fields[J]. 中国物理B, 2020, 29(8): 83201-083201.
[13]	李鹏程, Shih-I Chu. Multiphoton quantum dynamics of many-electron atomic and molecular systems in intense laser fields[J]. 中国物理B, 2020, 29(8): 83202-083202.
[14]	齐桐, 霍晓鑫, 张军, 刘学深. Semi-integer harmonic generation from an argon atom by bichromatic counter-rotating circularly polarized laser field[J]. 中国物理B, 2020, 29(5): 53201-053201.
[15]	马泽慧, 张彩萍, 马俊琳, 苗向阳. Controlling paths of high-order harmonic generation by orthogonal two-color fields[J]. 中国物理B, 2020, 29(4): 43201-043201.