中国物理B ›› 2014, Vol. 23 ›› Issue (9): 97803-097803.doi: 10.1088/1674-1056/23/9/097803

• CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES • 上一篇    下一篇

Silica-covered Au nanoresonators for fluorescence modulating of a graphene quantum dot

王素凤, 何大伟, 王永生, 胡音, 段嘉华, 富鸣, 王闻硕   

  1. Key Laboratory of Luminescence and Optical Information of the Ministry of Education, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, China
  • 收稿日期:2014-01-18 修回日期:2014-03-10 出版日期:2014-09-15 发布日期:2014-09-15
  • 基金资助:
    Project supported by the National Basic Research Program of China (Grant Nos. 2011CB932700 and 2011CB932703), the National Natural Science Foundation of China (Grant Nos. 61378073, 61335006, 91123025, and 61077044), and the Beijing Natural Science Foundation, China (Grant No. 4132031).

Silica-covered Au nanoresonators for fluorescence modulating of a graphene quantum dot

Wang Su-Feng (王素凤), He Da-Wei (何大伟), Wang Yong-Sheng (王永生), Hu Yin (胡音), Duan Jia-Hua (段嘉华), Fu Ming (富鸣), Wang Wen-Shuo (王闻硕)   

  1. Key Laboratory of Luminescence and Optical Information of the Ministry of Education, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, China
  • Received:2014-01-18 Revised:2014-03-10 Online:2014-09-15 Published:2014-09-15
  • Contact: He Da-Wei, Wang Wen-Shuo E-mail:dwhe@bjtu.edu.cn;wangwinsome@gmail.com
  • Supported by:
    Project supported by the National Basic Research Program of China (Grant Nos. 2011CB932700 and 2011CB932703), the National Natural Science Foundation of China (Grant Nos. 61378073, 61335006, 91123025, and 61077044), and the Beijing Natural Science Foundation, China (Grant No. 4132031).

摘要: We synthesize Au@SiO2 composite particles with a core-shell structure, and utilize the Au@SiO2 nanoparticles to modulate the fluorescence emission of the graphene quantum dot (GQD) through varying the silica shell thickness. The silica shell thickness can be easily controlled by varying the coating time. After silica coating, we investigate the influence of the silica thickness on the fluorescence emission of the GQD and find that the fluorescence property of the GQD can be changed as expected by varying the thickness of the silica shell. We propose an optimized coating time for the silica shell under the interaction of fluorescence quenching and enhancement.

关键词: graphene quantum dot, fluorescence, nanoparticles

Abstract: We synthesize Au@SiO2 composite particles with a core-shell structure, and utilize the Au@SiO2 nanoparticles to modulate the fluorescence emission of the graphene quantum dot (GQD) through varying the silica shell thickness. The silica shell thickness can be easily controlled by varying the coating time. After silica coating, we investigate the influence of the silica thickness on the fluorescence emission of the GQD and find that the fluorescence property of the GQD can be changed as expected by varying the thickness of the silica shell. We propose an optimized coating time for the silica shell under the interaction of fluorescence quenching and enhancement.

Key words: graphene quantum dot, fluorescence, nanoparticles

中图分类号:  (Optical properties of graphene)

  • 78.67.Wj
73.63.Kv (Quantum dots) 87.64.kv (Fluorescence) 78.67.Bf (Nanocrystals, nanoparticles, and nanoclusters)