Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

doi:10.1088/1674-1056/19/4/043201

中国物理B ›› 2010, Vol. 19 ›› Issue (4): 43201-043201.doi: 10.1088/1674-1056/19/4/043201

Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

张诗按, 张晖, 王祖赓, 孙真荣

State Key Laboratory of Precision Spectroscopy (East China Normal University), and Department of Physics, East China Normal University, Shanghai 200062, China

收稿日期:2009-06-29 修回日期:2009-08-03 出版日期:2010-04-15 发布日期:2010-04-15
基金资助:
Project supported by Programme for Changjiang Scholars and Innovative Research Team in University (PCSIRT), Shanghai Leading Academic Discipline Project (Grant No.~B408), National Key Project for Basic Research of China (Grant Nos.~2006CB806006 and 2006CB

Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

Zhang Shi-An(张诗按), Zhang Hui(张晖), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣)^†

State Key Laboratory of Precision Spectroscopy (East China Normal University), and Department of Physics, East China Normal University, Shanghai 200062, China

Received:2009-06-29 Revised:2009-08-03 Online:2010-04-15 Published:2010-04-15
Supported by:
Project supported by Programme for Changjiang Scholars and Innovative Research Team in University (PCSIRT), Shanghai Leading Academic Discipline Project (Grant No.~B408), National Key Project for Basic Research of China (Grant Nos.~2006CB806006 and 2006CB

摘要/Abstract

摘要： Femtosecond coherent anti-Stokes Raman scattering (CARS) suffers from poor selectivity between neighbouring Raman levels due to the large bandwidth of the femtosecond pulses. This paper provides a new method to realize the selective excitation and suppression of femtosecond CARS by manipulating both the probe and pump (or Stokes) spectra. These theoretical results indicate that the CARS signals between neighbouring Raman levels are differentiated from their indistinguishable femtosecond CARS spectra by tailoring the probe spectrum, and then their selective excitation and suppression can be realized by supplementally manipulating the pump (or Stokes) spectrum with the $\pi $ spectral phase step.

Abstract: Femtosecond coherent anti-Stokes Raman scattering (CARS) suffers from poor selectivity between neighbouring Raman levels due to the large bandwidth of the femtosecond pulses. This paper provides a new method to realize the selective excitation and suppression of femtosecond CARS by manipulating both the probe and pump (or Stokes) spectra. These theoretical results indicate that the CARS signals between neighbouring Raman levels are differentiated from their indistinguishable femtosecond CARS spectra by tailoring the probe spectrum, and then their selective excitation and suppression can be realized by supplementally manipulating the pump (or Stokes) spectrum with the $\pi $ spectral phase step.

Key words: coherent anti-Stokes Raman scattering (CARS), selective excitation, selective suppression, pulse shaping

中图分类号: (Stimulated Raman scattering; CARS)

42.65.Dr

42.65.Re (Ultrafast processes; optical pulse generation and pulse compression)

张诗按, 张晖, 王祖赓, 孙真荣. Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses[J]. 中国物理B, 2010, 19(4): 43201-043201.

Zhang Shi-An(张诗按), Zhang Hui(张晖), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣). Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses[J]. Chin. Phys. B, 2010, 19(4): 43201-043201.

参考文献 19

[1]	Chen T, Vierheilig A, P Waltner, Heid M, Kiefer W and Materny A 2000 Chem. Phys. Lett. 326 375
[2]	Rubner O, Schmitt M, Knopp G and Materny A 1998 J. Phys. Chem. A 102 9734
[3]	Hashimoto M, Araki T and Kawata S 2000 Opt. Lett. 25 1768
[4]	Yuan J H, Xiao F R, Wang G Y and Xu Z Z 2005 Chin. Phys. 14 935
[5]	Zumbusch A, Holtom G R and Xie X S 1999 Phys. Rev. Lett. 82 4142
[6]	Müller M, Squier J, Lange C A de and Brakenhoff G J 2000 J. Microsc. 197] 150
[7]	Wang Y H, Peng Y J, He X, Song Y F and Yang Y Q 2009 Chin. Phys. B 18 1463
[8]	Ujj L, Coates C G, Kelly J M, Kruger P E, McGarvey J J and Atkinson G H 2002 J. Phys. Chem. B 106 4854
[9]	Cheng J, Volkmer A, Book L D and Xie X S 2001 J. Phys. Chem. B 105 1277
[10]	Song J J, Eesley G L and Levenson M D 1976 Appl. Phys. Lett. 29 567
[11]	Oron D, Dudovich N, Yelin D and Silberberg Y 2002 Phys. Rev. A 65 043408
[12]	Oron D, Dudovich N, Yelin D and Silberberg Y 2002 Phys. Rev. Lett. 88 063004
[13]	Pearson B J, White J L, Weinacht T C and Bucksbaum P H 2001 Phys. Rev. A 63] 063412
[14]	Konradi J, Singh A K, Scaria A V and Materny A 2006 J. Raman Spectrosc. 37 697
[15]	Konradi J, Singh A K and Materny A 2006 J. Photochem. Photobio. 180 289
[16]	Zhang S, Zhang L, Zhang X, Ding L, Chen G, Sun Z and Wang Z 2007 Chem. Phys. Lett. 433 416
[17]	Müller M and Schins J M 2002 J. Phys. Chem. B 106 3715
[18]	Zhang S A, Wang Z G and Sun Z R 2008 Chin. Phys. Lett. 25 3260
[19]	Malinovskaya S A, Bucksbaum P H and Berman P R 2004 Phys. Rev. A, 69 013801

Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

PDF (PC)

赞

可视化

摘要/Abstract

引用本文

使用本文

参考文献 19

相关文章 15

Metrics

本文评价

推荐阅读 0

[1]	Wei Liu(刘伟), Shuai Ren(任帅), Pengfei Ma(马鹏飞), and Pu Zhou(周朴). Impact of amplified spontaneous emission noise on the SRS threshold of high-power fiber amplifiers[J]. 中国物理B, 2023, 32(3): 34202-034202.
[2]	Zhongyang Li(李忠洋), Qianze Yan(颜钤泽), Pengxiang Liu(刘鹏翔), Binzhe Jiao(焦彬哲), Gege Zhang(张格格), Zhiliang Chen(陈治良), Pibin Bing(邴丕彬), Sheng Yuan(袁胜), Kai Zhong(钟凯), and Jianquan Yao(姚建铨). THz wave generation by repeated and continuous frequency conversions from pump wave to high-order Stokes waves[J]. 中国物理B, 2022, 31(7): 74209-074209.
[3]	Zhong-Yang Li(李忠洋), Jia Zhao(赵佳), Sheng Yuan(袁胜), Bin-Zhe Jiao(焦彬哲), Pi-Bin Bing(邴丕彬), Hong-Tao Zhang(张红涛), Zhi-Liang Chen(陈治良), Lian Tan(谭联), and Jian-Quan Yao(姚建铨). Creation of multi-frequency terahertz waves by optimized cascaded difference frequency generation[J]. 中国物理B, 2022, 31(4): 44205-044205.
[4]	Yuye Wang(王与烨), Gang Nie(聂港), Changhao Hu(胡常灏), Kai Chen(陈锴), Chao Yan(闫超), Bin Wu(吴斌), Junfeng Zhu(朱军峰), Degang Xu(徐德刚), and Jianquan Yao(姚建铨). High-sensitive terahertz detection by parametric up-conversion using nanosecond pulsed laser[J]. 中国物理B, 2022, 31(2): 24204-024204.
[5]	Liangwei Wang(王亮伟), Jia Guan(关佳), Chengjie Zhu(朱成杰), Runbing Li(李润兵), and Jing Shi(石兢). A low noise, high fidelity cross phase modulation in multi-level atomic medium[J]. 中国物理B, 2021, 30(11): 114204-114204.
[6]	. [J]. 中国物理B, 2021, 30(4): 44211-.
[7]	. [J]. 中国物理B, 2021, 30(2): 24209-0.
[8]	刘喆, 杨博, 赵洪亮, 李占龙, 门志伟, 王晓峰, 王宁, 曹献文, 汪胜晗, 孙成林. Forward-headed structure change of acetic acid-water binary system by stimulated Raman scattering[J]. 中国物理B, 2019, 28(9): 94206-094206.
[9]	王文岩, 隋宁, 张里荃, 王英惠, 王琳, 王权, 王娇, 康智慧, 杨延强, 周强, 张汉壮. Scanning the energy dissipation process of energetic materials based on excited state relaxation and vibration-vibration coupling[J]. 中国物理B, 2018, 27(10): 104205-104205.
[10]	王畅, 吴红琳, 宋云飞, 杨延强. Structural deformation of nitro group of nitromethane molecule in liquid phase in an intense femtosecond laser field[J]. 中国物理B, 2017, 26(9): 94208-094208.
[11]	白金海, 李建军, 吴令安, 傅盘铭, 王如泉, 左战春. Autler-Townes spectroscopy of high-lying state by phase conjugate six-wave mixing[J]. 中国物理B, 2017, 26(4): 44204-044204.
[12]	马红梅, 陈丽清, 袁春华. Cascade correlation-enhanced Raman scattering in atomic vapors[J]. 中国物理B, 2016, 25(12): 124206-124206.
[13]	王畅, 吴红琳, 宋云飞, 何兴, 杨延强, 谭多旺. Tracking molecular structure deformation of nitrobenzene and its torsion vibration coupling by intense pumping CARS[J]. 中国物理B, 2016, 25(11): 114210-114210.
[14]	王梦, 芦小刚, 白金海, 裴丽娅, 缪兴绪, 高艳磊, 吴令安, 傅盘铭, 杨世平, 庞兆广, 王如泉, 左战春. Kramers-Kronig relation in a Doppler-broadened Λ -type three-level system[J]. 中国物理B, 2015, 24(11): 114205-114205.
[15]	张一弛, 陈伟, 孙世林, 孟洲. Effect of stimulated Brillouin scattering on the gain saturation of distributed fiber Raman amplifier and its suppression by phase modulation[J]. 中国物理B, 2015, 24(9): 94209-094209.