中国物理B ›› 2005, Vol. 14 ›› Issue (9): 1873-1878.doi: 10.1088/1009-1963/14/9/033

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Post-deposition dynamics of multiple cluster aggregation on liquid surfaces

许友生1, 吴锋民2, 叶高翔2, 吴自勤3   

  1. (1)College of Mathematics and Physics, Zhejiang Normal University, Jinhua 321004, China; (2)College of Science, Zhejiang University, Hangzhou 310027, China; (3)Department of Astronomy and Applied Physics, University of Science and Technology of China, Hefei 230026, China
  • 收稿日期:2004-11-15 修回日期:2005-04-27 出版日期:2005-09-20 发布日期:2005-09-20
  • 基金资助:
    Project supported by the Natural Science Foundation for Young Scientists of Zhejiang Province, China (Grant No RC02069) and Zhejiang Provincial Natural Science Foundation of China (Grant No 101032).

Post-deposition dynamics of multiple cluster aggregation on liquid surfaces

Wu Feng-Min (吴锋民)ab, Xu You-Sheng (许友生)a, Ye Gao-Xiang (叶高翔)b, Wu Zi-Qin (吴自勤)c   

  1. a College of Mathematics and Physics, Zhejiang Normal University, Jinhua 321004, China; b College of Science, Zhejiang University, Hangzhou 310027, China; c Department of Astronomy and Applied Physics, University of Science and Technology of China, Hefei 230026, China
  • Received:2004-11-15 Revised:2005-04-27 Online:2005-09-20 Published:2005-09-20
  • Supported by:
    Project supported by the Natural Science Foundation for Young Scientists of Zhejiang Province, China (Grant No RC02069) and Zhejiang Provincial Natural Science Foundation of China (Grant No 101032).

摘要: A comprehensive simulation model---deposition, diffusion, rotation and aggregation---is presented to demonstrate the post-deposition phenomena of multiple cluster growth on liquid surfaces, such as post-deposition nucleation, post-deposition growth and post-deposition coalescence. Emphasis is placed on the relaxations of monomer density, dimer density and cluster density as well as combined cluster-plus-monomer density with time after deposition ending. It is shown that post-deposition coalescence largely takes place after deposition due to the large mobility of clusters on liquid surfaces, while the post-deposition nucleation is only possible before the saturation cluster density is reached at the end of the deposition. The deposition flux and the moment of deposition ending play important roles in the post-deposition dynamics.

关键词: post-deposition dynamics, aggregation, liquid surface, simulation

Abstract: A comprehensive simulation model---deposition, diffusion, rotation and aggregation---is presented to demonstrate the post-deposition phenomena of multiple cluster growth on liquid surfaces, such as post-deposition nucleation, post-deposition growth and post-deposition coalescence. Emphasis is placed on the relaxations of monomer density, dimer density and cluster density as well as combined cluster-plus-monomer density with time after deposition ending. It is shown that post-deposition coalescence largely takes place after deposition due to the large mobility of clusters on liquid surfaces, while the post-deposition nucleation is only possible before the saturation cluster density is reached at the end of the deposition. The deposition flux and the moment of deposition ending play important roles in the post-deposition dynamics.

Key words: post-deposition dynamics, aggregation, liquid surface, simulation

中图分类号:  (Diffusion and thermal diffusion)

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