Cite this article:
Xiaotian Yang, Zijian Guo, Binshuo Zhang, Chao Dong, Wei Xia, Yanfeng Guo, Wenbo Wang. Direct Imaging of the Defect-Mediated Magnetic Phase Transition in a Topological Superlattice MnSb6Te10J. Chin. Phys. B.
| Xiaotian Yang, Zijian Guo, Binshuo Zhang, Chao Dong, Wei Xia, Yanfeng Guo, Wenbo Wang. Direct Imaging of the Defect-Mediated Magnetic Phase Transition in a Topological Superlattice MnSb6Te10J. Chin. Phys. B. |
Direct Imaging of the Defect-Mediated Magnetic Phase Transition in a Topological Superlattice MnSb6Te10
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Abstract
Structural disorder, specifically cation site-mixing, fundamentally dictates the magnetic energy landscape of van der Waals topological insulators. In this work, we resolve the real-space dynamics of the temperature-driven ferromagnetic (FM) to antiferromagnetic (AFM) phase transition in the superlattice MnSb6Te10. We demonstrate that MnSb antisite defects introduce competing interlayer exchange pathways, which trap the system in a metastable FM state at low temperatures. Using cryogenic magnetic force microscopy (MFM), we reveal that this state relaxes upon warming not through homogeneous melting, but via first-order spatial fragmentation into microscale magnetic islands, eventually yielding the intrinsic AFM ground state. Monte Carlo simulations based on a spatially inhomogeneous Heisenberg model reproduce these fragmentation dynamics, identifying defect density as a deterministic control knob for the magnetic phase competition. These results provide a comprehensive nanoscale picture of defect-modulated spin textures, establishing structural site-mixing as a viable strategy for manipulating magnetic symmetry and engineering non-trivial topological phases. -
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