Spin orbit torques in Pt-based heterostructures with van der Waals interface

Spin orbit torques (SOTs) in ferromagnet/heavy-metal heterostructures have provided great opportunities for efficient manipulation of spintronic devices. However, deterministically field-free switching of perpendicular magnetization with SOTs is forbidden because of the global two-fold rotational symmetry in conventional heavy-metal such as Pt. Here, we engineer the interface of Pt/Ni heterostructures by inserting a monolayer MoTe₂ with low crystal symmetry. It is demonstrated that the spin orbit efficiency, as well as the out-of-plane magnetic anisotropy and the Gilbert damping of Ni are enhanced, due to the effect of orbital hybridization and the increased spin scatting at the interface induced by MoTe₂. Particularly, an out-of-plane damping-like torque is observed when the current is applied perpendicular to the mirror plane of the MoTe₂ crystal, which is attributed to the interfacial inversion symmetry breaking of the system. Our work provides an effective route for engineering the SOT in Pt-based heterostructures, and offers potential opportunities for van der Waals interfaces in spintronic devices.