Quantum interference of multi-orbital effects in high-harmonic spectra from aligned carbon dioxide and nitrous oxide |
Ratio of the 27th harmonic intensity between aligned (S) and unaligned (S0) samples of CO2 (a) and N2O (b) molecules as a function of the delay time between the two laser beams. The polarization of the driving laser is parallel to that of the aligning laser. The Trot/2 (half revival) and Trot (full revival) are indicated in the figure. |