Metal-to-insulator transition in two-dimensional ferromagnetic monolayer induced by substrate*

Project supported by the National Natural Science Foundation of China (Grant No. 11574223), the Natural Science Foundation of Jiangsu Province, China (Grant No. BK20150303), and the Jiangsu Specially-Appointed Professor Program of Jiangsu Province, China.

Qi Can1, 2, Hu Jun1, 2, †
       

(color online) The top view (top panels) and side view (bottom panels) of atomic structures of (a) TaX2 monolayer, (b) TaX monolayer, and (c) TaX/Al2O3. The blue, brown, purple, and red spheres represent Ta, X (S, Se, or Te), Al, and O atoms, respectively. d1, d2, and d3 denote the Ta–X, X–O, and Ta–Al bond lengths, respectively. Δh indicates the buckling distance of the TaX monolayer. (d) Density of states (DOS) of the Al2O3(0001) surface. The Fermi energy is set to be the zero point of energy.