Odd–even harmonic emission from asymmetric molecules: Identifying the mechanism
Chen Jianguo, Yu Shujuan, Li Yanpeng, Wang Shang, Chen Yanjun
       

(color online) Comparisons of odd (solid-black) and even (dashed-red) dipoles for HeH2+ with Ip = 2.25 a.u., Z1/Z2 = 2 at R = 2 a.u. (the left column) and R = 4 a.u. (right), obtained by different methods. In panels (a) and (b), we show the 1D exact dipoles |〈0|x|p〉|2/ω4 for the continuum state |p〉 having the odd-like (corresponding to odd dipoles) or even-like (even dipoles) parity. The continuum state |p〉 has the energy Ep = ωIp. Here, ω = nω0 is the assumed harmonic energy with ω0 = 0.057 a.u. (λ = 800 nm). In panels (c) and (d), we show the dipoles |Dodd(even)(θ, ω)|2/ω4 with θ = 0° obtained using Eqs. (4) and (5) (the previous dipoles). In panels (e) and (f), we show those obtained using Eqs. (6) and (7) (the improved dipoles). The log10 scale is used here.