Two-dimensional materials for ultrafast lasers
Wang Fengqiu
       

(color online) (a) Pump-probe spectroscopy performed with 390 nm pump and 660 nm probe on a mechanically exfoliated MoS2 sample (transferred onto a SO2/Si substrate), showing a carrier lifetime of .[83] (b) Time-resolved differential transmission spectra performed on a liquid phase exfoliated few-layer WS2 sample with degenerate 635 nm pump and probe beam, showing a fast PB signal (∼ 5 ps), followed by an emerging PA signature.[84] (c) Transient differential transmission performed with 10 fs visible pulses on a few-layer MoS2 sample grown by CVD method. Carrier thermalization occurs within 20 fs and the subsequent cooling of Fermi–Dirac carrier distribution occurs on the ∼ 0.6 ps timescale.[85] (d) Pump–probe spectroscopy performed on mechanically exfoliated MoS2 sample with 452 nm pump and 905 nm probe, showing the dependence of the timescales on the layer number. Different curves are scaled in magnitude for clarity.[86]