Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH3NH3PbI3-xClx prepared onZnO/FTO substrates using a two-step method

doi:10.1088/1674-1056/26/1/017802

Abstract Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH₃NH₃PbI_3-xCl_x films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and absorption characteristics of the films were also studied. Scanning electron microscopy revealed large crystals and substrate coverage. The orthorhombic-to-tetragonal phase transition temperature was ~140 K. The films' exciton binding energy was 77.6±10.9 meV and the energy of optical phonons was 38.8±2.5 meV. These results suggest that perovskite CH₃NH₃PbI_3-xCl_x films have excellent optoelectronic characteristics which further suggests their potential usage in perovskitebased optoelectronic devices.

Keywords: perovskite temperature-dependent photoluminescence two-step method ZnO

Received: 27 August 2016
Revised: 13 October 2016
Accepted manuscript online:

PACS:

78.20.-e 78.55.-m

Fund: Project supported by the International Science and Technology Cooperation Program of Science and Technology Bureau of Changchun City, China (Grant No. 12ZX68).

Corresponding Authors: Baolin Zhang
E-mail: zbl@jlu.edu.cn

Cite this article:

Shiwei Zhuang(庄仕伟), Deqian Xu(徐德前), Jiaxin Xu(徐佳新), Bin Wu(伍斌), Yuantao Zhang(张源涛), Xin Dong(董鑫), Guoxing Li(李国兴), Baolin Zhang(张宝林), Guotong Du(杜国同) Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method 2017 Chin. Phys. B 26 017802

[1]	Xing G, Mathews N, Lim S S, Yantara N, Liu X, Sabba D, Gratzel M, Mhaisalkar S and Sum T C 2014 Nat. Mater. 13 476
[2]	Oga H, Saeki A, Ogomi Y, Hayase S and Seki S 2014 J. Am. Chem. Soc. 136 13818
[3]	Kuppler R J, Timmons D J, Fang Q R, Li J R, Makal T A, Young M D, Yuan D Q, Zhao D, Zhuang W J and Zhou H C 2009 Coordin. Chem. Rev. 253 3042
[4]	Plank N O V, Howard I, Rao A, Wilson M W B, Ducati C, Mane R S, Bendall J S, Louca R R M, Greenham N C, Miura H, Friend R H, Snaith H J and Welland M E 2009 J. Phys. Chem. C 113 18515
[5]	Bi D Q, Wu F, Qu Q Y, Yue W J, Cui Q, Shen W, Chen R Q, Liu C W, Qiu Z L and Wang M T 2011 J. Phys. Chem. C 115 3745
[6]	Chen Q Y, Huang Y, Huang P R, Ma T, Cao C and He Y 2016 Chin. Phys. B 25 027104
[7]	Li J F, Zhao C, Zhang H, Tong J F, Zhang P, Yang C Y, Xia Y J and Fan D W 2016 Chin. Phys. B 25 028402
[8]	Kojima K T A, Shirai Y and Miyasaka T 2009 J. Am. Chem. Soc. 131 6050
[9]	Zhang T K, Yu T and Zou Z G 2015 Physics 44 315
[10]	Jeon N J, Noh J H, Yang W S, Kim Y C, Ryu S, Seo J and Seok S I 2015 Nature 517 476
[11]	Hu X, Zhang X D, Liang L, Bao J, Li S, Yang W L and Xie Y 2014 Adv. Funct. Mater. 24 7373
[12]	Fang H H, Raissa R, Abdu-Aguye M, Adjokatse S, Blake G R, Even J and Loi M A 2015 Adv. Funct. Mater. 25 2378
[13]	Tan Z K, Moghaddam R S, Lai M L, Docampo P, Higler R, Deschler F, Price M, Sadhanala A, Pazos L M, Credgington D, Hanusch F, Bein T, Snaith H J and Friend R H 2014 Nat. Nanotechnol. 9 687
[14]	Huang M H, Mao S, Feick H, Yan H Q, Wu Y Y, Kind H, Weber E, Russo R and Yang P D 2001 Science 292 1897
[15]	He T, Xia Y J, Qin H C, Guan Z S and Li W Y 2011 Physics 4 0
[16]	Yu X X, Zhou Y, Liu J, Jin H B, Fang X Y and Cao M S 2015 Chin. Phys. B 24 127307
[17]	Shi Z F, Zhang Y T, Cai X P, Wang H, Wu B, Zhang J X, Cui X J, Dong X, Liang H W, Zhang B L and Du G T 2014 Cryst. Eng. Comm. 16 455
[18]	Burschka J, Pellet N, Moon S J, Humphry-Baker R, Gao P, Nazeeruddin M K and Gratzel M 2013 Nature 499 316
[19]	Zheng L L, Ma Y Z, Chu S S, Wang S F, Qu B, Xiao L X, Chen Z J, Gong Q H, Wu Z X and Hou X 2014 Nanoscale 6 8171
[20]	Zheng L, Zhang D, Ma Y, Lu Z, Chen Z, Wang S, Xiao L and Gong Q 2015 Dalton T. 44 10582
[21]	Lee M M, Teuscher J, Miyasaka T, Murakami N T and Snaith H J 2012 Science 338 643
[22]	Jaramillo-Quintero O A, Sanchez R S, Rincon M and Mora-Sero I 2014 J. Phys. Chem. Lett. 6 1883
[23]	Wehrenfennig C, Liu M Z, Snaith H J, Johnston M B and Herz L M 2014 APL Mater. 2 081513
[24]	D'Innocenzo V, Grancini G, Alcocer M J P, Kandada A R S, Stranks S D, Lee M M, Lanzani G, Snaith H J and Petrozza A 2014 Nat. Commun. 5 3586
[25]	Kao T S, Chou Y H, Chou C H, Chen F C and Lu T C 2014 Appl. Phys. Lett. 105 231108
[26]	Savenije T J, Ponseca C S, Kunneman L, Abdellah M, Zheng K, Tian Y, Zhu Q, Canton S E, Scheblykin I G, Pullerits T, Yartsev A and Sundstrom V 2014 J. Phys. Chem. Lett. 5 2189
[27]	Georgiev T and Baleva G L M 1990 J. Phys.:Condens. Matter 1 2935
[28]	Wu K, Bera A, Ma C, Du Y M, Yang Y, Li L and Wu T 2014 Phys. Chem. Chem. Phys. 16 22476
[29]	Quarti C, Grancini G, Mosconi E, Bruno P, Ball J M, Lee M M, Snaith H J, Petrozza A and Angelis F D 2014 J. Phys. Chem. Lett. 5 279

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Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH3NH3PbI3-xClx prepared onZnO/FTO substrates using a two-step method

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Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method