中国物理B ›› 2024, Vol. 33 ›› Issue (10): 106101-106101.doi: 10.1088/1674-1056/ad625a

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Direct observation of shock-induced phase transformation in polycrystalline iron via in situ x-ray diffraction

Fan Zhang(张帆)1,2,†, Jia-Qin Dong(董佳钦)2, Zhi-Yong Xie(谢志勇)2, Zhi-Yu He(贺芝宇)2, Hua Shu(舒桦)2, Rui-Rong Wang(王瑞荣)2, Jun Xiong(熊俊)2, Guo Jia(贾果)2, Zhi-Heng Fang(方智恒)2, Wei Wang(王伟)2, Da-Wu Xiao(肖大武)3, An-Le Lei(雷安乐)2, Jie Chen(陈洁)1, and Xiu-Guang Huang(黄秀光)2,‡   

  1. 1 Collaborative Innovation Center of IFSA (CICIFSA), School of Physics and Astronomy, Center for Ultrafast Science and Technology, Key Laboratory for Laser Plasmas (Ministry of Education), Shanghai Jiao Tong University, Shanghai 200240, China;
    2 Shanghai Institute of Laser Plasma, China Academy of Engineering Physics, Shanghai 201800, China;
    3 Institute of Materials, China Academy of Engineering Physics, Mianyang 621700, China
  • 收稿日期:2024-03-21 修回日期:2024-06-04 接受日期:2024-07-12 出版日期:2024-10-15 发布日期:2024-10-15
  • 通讯作者: Fan Zhang, Xiu-Guang Huang E-mail:zhang_fan@sjtu.edu.cn;huangxiuguang@sohu.com
  • 基金资助:
    This work was supported by the National Natural Science Foundation of China (Grant Nos. 12304033, 12072328, and 11991073).

Direct observation of shock-induced phase transformation in polycrystalline iron via in situ x-ray diffraction

Fan Zhang(张帆)1,2,†, Jia-Qin Dong(董佳钦)2, Zhi-Yong Xie(谢志勇)2, Zhi-Yu He(贺芝宇)2, Hua Shu(舒桦)2, Rui-Rong Wang(王瑞荣)2, Jun Xiong(熊俊)2, Guo Jia(贾果)2, Zhi-Heng Fang(方智恒)2, Wei Wang(王伟)2, Da-Wu Xiao(肖大武)3, An-Le Lei(雷安乐)2, Jie Chen(陈洁)1, and Xiu-Guang Huang(黄秀光)2,‡   

  1. 1 Collaborative Innovation Center of IFSA (CICIFSA), School of Physics and Astronomy, Center for Ultrafast Science and Technology, Key Laboratory for Laser Plasmas (Ministry of Education), Shanghai Jiao Tong University, Shanghai 200240, China;
    2 Shanghai Institute of Laser Plasma, China Academy of Engineering Physics, Shanghai 201800, China;
    3 Institute of Materials, China Academy of Engineering Physics, Mianyang 621700, China
  • Received:2024-03-21 Revised:2024-06-04 Accepted:2024-07-12 Online:2024-10-15 Published:2024-10-15
  • Contact: Fan Zhang, Xiu-Guang Huang E-mail:zhang_fan@sjtu.edu.cn;huangxiuguang@sohu.com
  • Supported by:
    This work was supported by the National Natural Science Foundation of China (Grant Nos. 12304033, 12072328, and 11991073).

摘要: Phase transition of polycrystalline iron compressed along the Hugoniot is studied by combining laser-driven shock with in situ x-ray diffraction technique. It is suggested that polycrystalline iron changes from an initial body-centered cubic structure to a hexagonal close-packed structure with increasing pressure (i.e., a phase transition from $\alpha$ to $\varepsilon$). The relationship between density and pressure for polycrystalline iron obtained from the present experiments is found to be in good agreement with the gas-gun Hugoniot data. Our results show that experiments with samples at lower temperatures under static loading, such as in a diamond anvil cell, lead to higher densities measured than those found under dynamic loading. This means that extrapolating results of static experiments may not predict the dynamic responses of materials accurately. In addition, neither the face-centered cubic structure seen in previous molecular-dynamics simulations or two-phase coexistence are found within our experimental pressure range.

关键词: in situ x-ray diffraction, phase transition, polycrystalline iron

Abstract: Phase transition of polycrystalline iron compressed along the Hugoniot is studied by combining laser-driven shock with in situ x-ray diffraction technique. It is suggested that polycrystalline iron changes from an initial body-centered cubic structure to a hexagonal close-packed structure with increasing pressure (i.e., a phase transition from $\alpha$ to $\varepsilon$). The relationship between density and pressure for polycrystalline iron obtained from the present experiments is found to be in good agreement with the gas-gun Hugoniot data. Our results show that experiments with samples at lower temperatures under static loading, such as in a diamond anvil cell, lead to higher densities measured than those found under dynamic loading. This means that extrapolating results of static experiments may not predict the dynamic responses of materials accurately. In addition, neither the face-centered cubic structure seen in previous molecular-dynamics simulations or two-phase coexistence are found within our experimental pressure range.

Key words: in situ x-ray diffraction, phase transition, polycrystalline iron

中图分类号:  (X-ray diffraction)

  • 61.05.cp
64.70.K (Solid-solid transitions) 62.50.-p (High-pressure effects in solids and liquids)