Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects

doi:10.1088/1674-1056/ac9608

中国物理B ›› 2022, Vol. 31 ›› Issue (12): 127801-127801.doi: 10.1088/1674-1056/ac9608

所属专题： SPECIAL TOPIC — The third carbon: Carbyne with one-dimensional sp-carbon

Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects

Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg^†

Institut für Physik and IRIS Adlershof, Humboldt Universität zu Berlin, 12489 Berlin, Germany

收稿日期:2022-07-01 修回日期:2022-09-22 接受日期:2022-09-29 出版日期:2022-11-11 发布日期:2022-12-05
通讯作者: Sebastian Heeg E-mail:sebastian.heeg@physik.hu-berlin.de
基金资助:
Johannes M. A. Lechner, Pablo Hernandez López, and Sebastian Heeg acknowledge funding from the Deutsche Forschungsgemeinschaft (DFG) under the Emmy Noether Initiative (HE 8642/1-1).

Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects

Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg^†

Institut für Physik and IRIS Adlershof, Humboldt Universität zu Berlin, 12489 Berlin, Germany

Received:2022-07-01 Revised:2022-09-22 Accepted:2022-09-29 Online:2022-11-11 Published:2022-12-05
Contact: Sebastian Heeg E-mail:sebastian.heeg@physik.hu-berlin.de
Supported by:
Johannes M. A. Lechner, Pablo Hernandez López, and Sebastian Heeg acknowledge funding from the Deutsche Forschungsgemeinschaft (DFG) under the Emmy Noether Initiative (HE 8642/1-1).

摘要/Abstract

摘要： Carbyne is an infinitely long linear chain of carbon atoms with sp¹ hybridization and the truly one-dimensional allotrope of carbon. While obtaining freestanding carbyne is still an open challenge, the study of confined carbyne, linear chains of carbon encapsulated in carbon nanotubes, provides a pathway to explore carbyne and its remarkable properties in a well-defined environment. In this review, we discuss the basics and recent advances in studying single confined carbyne chains by Raman spectroscopy, which is their primary spectroscopic characterization method. We highlight where single carbyne chain studies are needed to advance our understanding of confined carbyne as a material system and provide an overview of the open questions that need to be addressed and of those aspects currently under debate.

关键词: carbyne, linear carbon chains, carbon nanotubes, Raman spectroscopy

Abstract: Carbyne is an infinitely long linear chain of carbon atoms with sp¹ hybridization and the truly one-dimensional allotrope of carbon. While obtaining freestanding carbyne is still an open challenge, the study of confined carbyne, linear chains of carbon encapsulated in carbon nanotubes, provides a pathway to explore carbyne and its remarkable properties in a well-defined environment. In this review, we discuss the basics and recent advances in studying single confined carbyne chains by Raman spectroscopy, which is their primary spectroscopic characterization method. We highlight where single carbyne chain studies are needed to advance our understanding of confined carbyne as a material system and provide an overview of the open questions that need to be addressed and of those aspects currently under debate.

Key words: carbyne, linear carbon chains, carbon nanotubes, Raman spectroscopy

中图分类号: (Nanotubes)

78.67.Ch

78.67.Uh (Nanowires)

Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg. Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects[J]. 中国物理B, 2022, 31(12): 127801-127801.

Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg. Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects[J]. Chin. Phys. B, 2022, 31(12): 127801-127801.

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Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects

Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects

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