中国物理B ›› 2017, Vol. 26 ›› Issue (3): 33702-033702.doi: 10.1088/1674-1056/26/3/033702

• ATOMIC AND MOLECULAR PHYSICS • 上一篇    下一篇

BaF radical: A promising candidate for laser cooling and magneto-optical trapping

Liang Xu(许亮), Bin Wei(魏斌), Yong Xia(夏勇), Lian-Zhong Deng(邓联忠), Jian-Ping Yin(印建平)   

  1. State Key Laboratory of Precision Spectroscopy, School of Physics and Materials Science, East China Normal University, Shanghai 200062, China
  • 收稿日期:2016-11-10 修回日期:2016-12-07 出版日期:2017-03-05 发布日期:2017-03-05
  • 通讯作者: Jian-Ping Yin E-mail:jpyin@phy.ecnu.edu.cn
  • 基金资助:
    Project supported by the National Natural Science Foundation of China (Grant Nos. 91536218, 11374100, 10904037, 10974055, 11034002, and 11274114), the National Key Basic Research and Development Program of China (Grant No. 2011CB921602), and the Natural Science Foundation of Shanghai Municipality, China (Grant No. 13ZR1412800).

BaF radical: A promising candidate for laser cooling and magneto-optical trapping

Liang Xu(许亮), Bin Wei(魏斌), Yong Xia(夏勇), Lian-Zhong Deng(邓联忠), Jian-Ping Yin(印建平)   

  1. State Key Laboratory of Precision Spectroscopy, School of Physics and Materials Science, East China Normal University, Shanghai 200062, China
  • Received:2016-11-10 Revised:2016-12-07 Online:2017-03-05 Published:2017-03-05
  • Contact: Jian-Ping Yin E-mail:jpyin@phy.ecnu.edu.cn
  • Supported by:
    Project supported by the National Natural Science Foundation of China (Grant Nos. 91536218, 11374100, 10904037, 10974055, 11034002, and 11274114), the National Key Basic Research and Development Program of China (Grant No. 2011CB921602), and the Natural Science Foundation of Shanghai Municipality, China (Grant No. 13ZR1412800).

摘要: Recently, there have been great interest and advancement in the field of laser cooling and magneto-optical trapping of molecules. The rich internal structure of molecules naturally lends themselves to extensive and exciting applications. In this paper, the radical 138Ba19F, as a promising candidate for laser cooling and magneto-optical trapping, is discussed in detail. The highly diagonal Franck-Condon factors between the X2Σ1/2+ and A2Π1/2 states are first confirmed with three different methods. Afterwards, with the effective Hamiltonian approach and irreducible tensor theory, the hyperfine structure of the X2Σ1/2+ state is calculated accurately. A scheme for laser cooling is given clearly. Besides, the Zeeman effects of the upper (A2Π1/2) and lower (X2Σ1/2+) levels are also studied, and their respective g factors are obtained under a weak magnetic field. Its large g factor of the upper state A2Π1/2 is advantageous for magneto-optical trapping. Finally, by studying Stark effect of BaF in the X2Σ1/2+, we investigate the dependence of the internal effective electric field on the applied electric field. It is suggested that such a laser-cooled BaF is also a promising candidate for precision measurement of electron electric dipole moment.

关键词: laser cooling, magneto-optical trapping, BaF radical

Abstract: Recently, there have been great interest and advancement in the field of laser cooling and magneto-optical trapping of molecules. The rich internal structure of molecules naturally lends themselves to extensive and exciting applications. In this paper, the radical 138Ba19F, as a promising candidate for laser cooling and magneto-optical trapping, is discussed in detail. The highly diagonal Franck-Condon factors between the X2Σ1/2+ and A2Π1/2 states are first confirmed with three different methods. Afterwards, with the effective Hamiltonian approach and irreducible tensor theory, the hyperfine structure of the X2Σ1/2+ state is calculated accurately. A scheme for laser cooling is given clearly. Besides, the Zeeman effects of the upper (A2Π1/2) and lower (X2Σ1/2+) levels are also studied, and their respective g factors are obtained under a weak magnetic field. Its large g factor of the upper state A2Π1/2 is advantageous for magneto-optical trapping. Finally, by studying Stark effect of BaF in the X2Σ1/2+, we investigate the dependence of the internal effective electric field on the applied electric field. It is suggested that such a laser-cooled BaF is also a promising candidate for precision measurement of electron electric dipole moment.

Key words: laser cooling, magneto-optical trapping, BaF radical

中图分类号:  (Slowing and cooling of molecules)

  • 37.10.Mn
37.10.Pq (Trapping of molecules) 32.10.Fn (Fine and hyperfine structure) 32.60.+i (Zeeman and Stark effects)