Electron localization of linear symmetric molecular ion H32+

doi:10.1088/1674-1056/26/1/013203

中国物理B ›› 2017, Vol. 26 ›› Issue (1): 13203-013203.doi: 10.1088/1674-1056/26/1/013203

• SPECIAL TOPIC—Soft matter and biological physics (Review) • 上一篇下一篇

Electron localization of linear symmetric molecular ion H₃²⁺

Zheng-Mao Jia(贾正茂), Zhi-Nan Zeng(曾志男), Ru-Xin Li(李儒新)

State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

收稿日期:2016-09-11 修回日期:2016-10-24 出版日期:2017-01-05 发布日期:2017-01-05
通讯作者: Zhi-Nan Zeng E-mail:zhinan_zeng@mail.siom.ac.cn
基金资助:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11127901, 61521093, 11134010, 11227902, 11222439, and 11274325) and the National Basic Research Program of China (Grant No. 2011CB808103).

Electron localization of linear symmetric molecular ion H₃²⁺

Zheng-Mao Jia(贾正茂), Zhi-Nan Zeng(曾志男), Ru-Xin Li(李儒新)

State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

Received:2016-09-11 Revised:2016-10-24 Online:2017-01-05 Published:2017-01-05
Contact: Zhi-Nan Zeng E-mail:zhinan_zeng@mail.siom.ac.cn
Supported by:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11127901, 61521093, 11134010, 11227902, 11222439, and 11274325) and the National Basic Research Program of China (Grant No. 2011CB808103).

摘要/Abstract

摘要：

Electron localization in the dissociation of the symmetric linear molecular ion H₃²⁺ is investigated. The numerical simulation shows that the electron localization distribution is dependent on the central frequency and peak electric field amplitude of the external ultrashort ultraviolet laser pulse. When the electrons of the ground state are excited onto the 2pσ²Σ_u⁺ by a one-photon process, most electrons of the dissociation states are localized at the protons on both sides symmetrically. Almost no electron is stabilized at the middle proton due to the odd symmetry of the wave function. With the increase of the frequency of the external ultraviolet laser pulse, the electron localization ratio of the middle proton increases, for more electrons of the ground state are excited onto the higher 3pσ²Σ_u⁺ state. 50.9% electrons of all the dissociation events can be captured by the middle Coulomb potential well through optimizing the central frequency and peak electric field amplitude of the ultraviolet laser pulse. Besides, a direct current (DC) electric field can be utilized to control the electron motions of the dissociation states after the excitation of an ultraviolet laser pulse, and 68.8% electrons of the dissociation states can be controlled into the middle proton.

关键词: dissociation localization, time-dependent Schrödinger equation, Coulomb potential, ultraviolet laser pulse

Abstract:

Key words: dissociation localization, time-dependent Schrö, dinger equation, Coulomb potential, ultraviolet laser pulse

中图分类号: (Multiphoton ionization and excitation to highly excited states)

32.80.Rm

33.80.Rv (Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)) 42.50.Hz (Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift) 42.65.Ky (Frequency conversion; harmonic generation, including higher-order harmonic generation)

贾正茂, 曾志男, 李儒新. Electron localization of linear symmetric molecular ion H₃²⁺[J]. 中国物理B, 2017, 26(1): 13203-013203.

Zheng-Mao Jia(贾正茂), Zhi-Nan Zeng(曾志男), Ru-Xin Li(李儒新). Electron localization of linear symmetric molecular ion H₃²⁺[J]. Chin. Phys. B, 2017, 26(1): 13203-013203.

参考文献 21

[1]	Gaire B, McKenna J, Zohrabi M, Carnes K D, Esry B D and Ben Itzhak I 2000 Phys. Rev. A 85 023419
[2]	Roudnev V and Esry B D 2007 Phys. Rev. A 76 023403
[3]	Roudnev V, Esry B D and Ben Itzhak I 2004 Phys. Rev. Lett. 93 163601
[4]	McKenna J, Anis F, Sayler A M, Gaire B, Johnson Nora G, Parke E, Carnes K D, Esry B D and Ben Itzhak I 2010 Phys. Rev. A 85 023405
[5]	Fischer B, Kremer M, Pfeifer T, Feuerstein B, Sharma V, Thumm U, Schröter C D, Moshammer R and Ullrich J 2010 Phys. Rev. Lett. 105 223001
[6]	He F 2012 Phys. Rev. A 86 063415
[7]	Kling M F, Siedschlag Ch, Znakovskaya I, Verhoef A J, Zherebtsov S, Krausz F, Lezius M and Vrakking M J J 2008 Mole. Phys. 106 455
[8]	Kling M F, Siedschlag Ch, Verhoef A J, Khan J I, Schultze M, Uphues Th, Ni Y, Uiberacker M, Drescher M, Krausz F and Vrakking M J J 2006 Science 312 246
[9]	Sansone G, Kelkensberg F, Pérez Torres J F, Morales F, Kling M F, Siu W, Ghafur O, Johnsson, Swoboda P M, Benedetti E, Ferrari, Lépine F F, Sanz Vicario J L, Zherebtsov S, Znakovskaya I, L'Huillier A, Ivanov M Yu, Nisoli M, Martín F and Vrakking M J J 2010 Nature 465 763
[10]	Dietrich P, Ivanov M Yu, Ilkov F A and Corkum P B 1996 Phys. Rev. Lett. 77 4150
[11]	Niikura H, Corkum P B and Villeneuve D M 2003 Phys. Rev. Lett. 90 203601
[12]	Niikura H, Villeneuve D M and Corkum P B 2004 Phys. Rev. Lett. 92 133002
[13]	Zuo T and Bandrauk A D 1995 Phys. Rev. A 51 R26
[14]	Turbiner A V and López Vieyra J C 2006 Phys. Rep. 424 309
[15]	Bandrauk A, Barmaki S and Kamta G L 2007 Phys. Rev. Lett. 98 013001
[16]	Jia Z M, Zeng Z N, Li R X, Xu Z Z and Deng Y P 2014 Phys. Rev. A 89 023419
[17]	Jia Z M, Zeng Z N, Li R X and Xu Z Z 2014 Chin. Phys. B 23 083201
[18]	Jia Z M, Zeng Z N, Li R X, Xu Z Z and Deng Y P 2015 Chin. Phys. B 24 013204
[19]	Bian X B, Peng L Y and Shi T Y 2008 Phys. Rev. A 78 053408
[20]	Herzberg G 1953 Molecular Spectra and Molecular Structure I Spectra of Diamotic Molecules, 2th edn. (New York:D. VAN NOSTRAND) pp. 321-324
[21]	Jia Z M, Zeng Z N, Li R X and Xu Z Z 2016 J. Phys. B 49 215604

Electron localization of linear symmetric molecular ion H₃²⁺

Electron localization of linear symmetric molecular ion H₃²⁺

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