Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O3 ceramic

doi:10.1088/1674-1056/20/9/097702

中国物理B ›› 2011, Vol. 20 ›› Issue (9): 97702-097702.doi: 10.1088/1674-1056/20/9/097702

Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic

徐卓¹, 高俊杰¹, 姚熹¹, 张崇辉², 朱长军²

(1)Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education, Xi'an Jiaotong University, Xi'an 710048, China; (2)School of Science, Xi'an Polytechnic University, Xi'an 710048, China

收稿日期:2010-10-25 修回日期:2011-04-09 出版日期:2011-09-15 发布日期:2011-09-15

Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic

Zhang Chong-Hui(张崇辉)^a)b)^†, Xu Zhuo(徐卓)^b), Gao Jun-Jie(高俊杰)^b), Zhu Chang-Jun(朱长军)^a), and Yao Xi(姚熹)^b)

^a School of Science, Xi'an Polytechnic University, Xi'an 710048, China; ^b Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education, Xi'an Jiaotong University, Xi'an 710048, China

Received:2010-10-25 Revised:2011-04-09 Online:2011-09-15 Published:2011-09-15

摘要/Abstract

摘要： Antiferroelectric—ferroelectric (AFE—FE) phase transition in ceramic Pb_0.97La_0.02(Zr_0.75Sn_0.136Ti_0.114)O₃ (PLZST) was studied by dielectric spectroscopy as functions of frequency (10²—10⁵ Hz) and pressure (0—500 MPa) under a DC electric field. The hydrostatic pressure-dependent remnant polarization and dielectric constant were measured. The results show that remnant polarization of the metastable rhombohedral ferroelectric PLZST poled ceramic decreases sharply and depoles completely at phase transition under hydrostatic pressure. The dielectric constant undergoes an abrupt jump twice during a load and unload cycle under an electric field. The two abrupt jumps correspond to two phase transitions, FE—AFE and AFE—FE.

关键词: antiferroelectric ceramic, dielectric constant, hydrostatic pressure, phase transition

Abstract: Antiferroelectric—ferroelectric (AFE—FE) phase transition in ceramic Pb_0.97La_0.02(Zr_0.75Sn_0.136Ti_0.114)O₃ (PLZST) was studied by dielectric spectroscopy as functions of frequency (10²—10⁵ Hz) and pressure (0—500 MPa) under a DC electric field. The hydrostatic pressure-dependent remnant polarization and dielectric constant were measured. The results show that remnant polarization of the metastable rhombohedral ferroelectric PLZST poled ceramic decreases sharply and depoles completely at phase transition under hydrostatic pressure. The dielectric constant undergoes an abrupt jump twice during a load and unload cycle under an electric field. The two abrupt jumps correspond to two phase transitions, FE—AFE and AFE—FE.

Key words: antiferroelectric ceramic, dielectric constant, hydrostatic pressure, phase transition

中图分类号: (Ferroelectricity and antiferroelectricity)

77.80.-e

77.22.Ch (Permittivity (dielectric function)) 62.50.-p (High-pressure effects in solids and liquids)

张崇辉, 徐卓, 高俊杰, 朱长军, 姚熹. Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic[J]. 中国物理B, 2011, 20(9): 97702-097702.

Zhang Chong-Hui(张崇辉), Xu Zhuo(徐卓), Gao Jun-Jie(高俊杰), Zhu Chang-Jun(朱长军), and Yao Xi(姚熹) . Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic[J]. Chin. Phys. B, 2011, 20(9): 97702-097702.

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Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic

Electromechanical-induced antiferroelectric–ferroelectric phase transition in PbLa(Zr,Sn,Ti)O₃ ceramic

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