Highly selective population of two excited states in nonresonant two-photon absorption

doi:10.1088/1674-1056/20/8/083202

中国物理B ›› 2011, Vol. 20 ›› Issue (8): 83202-083202.doi: 10.1088/1674-1056/20/8/083202

• ATOMIC AND MOLECULAR PHYSICS • 上一篇下一篇

Highly selective population of two excited states in nonresonant two-photon absorption

张晖, 张诗按, 孙真荣

State Key Laboratory of Precision Spectroscopy and Department of Physics, East China Normal University, Shanghai 200062, China

收稿日期:2010-11-02 修回日期:2011-03-14 出版日期:2011-08-15 发布日期:2011-08-15
基金资助:
Project partly supported by the Shanghai Leading Academic Discipline Project (Grant No. B408), the Science Foundation of the Ministry of Education of China (Grant No. 30800), the National Natural Science Fundation of China (Grant No. 11004060), and the Shanghai Municipal Science and Technology Commission (Grant Nos. 10XD1401800, 09142200501, 09ZR1409300, 09JC1404700, and 10JC1404500).

Highly selective population of two excited states in nonresonant two-photon absorption

Zhang Hui(张晖), Zhang Shi-An(张诗按)^†, and Sun Zhen-Rong(孙真荣)

State Key Laboratory of Precision Spectroscopy and Department of Physics, East China Normal University, Shanghai 200062, China

Received:2010-11-02 Revised:2011-03-14 Online:2011-08-15 Published:2011-08-15
Supported by:
Project partly supported by the Shanghai Leading Academic Discipline Project (Grant No. B408), the Science Foundation of the Ministry of Education of China (Grant No. 30800), the National Natural Science Fundation of China (Grant No. 11004060), and the Shanghai Municipal Science and Technology Commission (Grant Nos. 10XD1401800, 09142200501, 09ZR1409300, 09JC1404700, and 10JC1404500).

摘要/Abstract

摘要： A nonresonant two-photon absorption process can be manipulated by tailoring the ultra-short laser pulse. In this paper, we theoretically demonstrate a highly selective population of two excited states in the nonresonant two-photon absorption process by rationally designing a spectral phase distribution. Our results show that one excited state is maximally populated while the other state population is widely tunable from zero to the maximum value. We believe that the theoretical results may play an important role in the selective population of a more complex nonlinear process comprising nonresonant two-photon absorption, such as resonance-mediated (2+1)-three-photon absorption and (2+1)-resonant multiphoton ionization.

Abstract: A nonresonant two-photon absorption process can be manipulated by tailoring the ultra-short laser pulse. In this paper, we theoretically demonstrate a highly selective population of two excited states in the nonresonant two-photon absorption process by rationally designing a spectral phase distribution. Our results show that one excited state is maximally populated while the other state population is widely tunable from zero to the maximum value. We believe that the theoretical results may play an important role in the selective population of a more complex nonlinear process comprising nonresonant two-photon absorption, such as resonance-mediated (2+1)-three-photon absorption and (2+1)-resonant multiphoton ionization.

Key words: nonresonant two-photon absorption, selective population, coherent control

中图分类号: (Other multiphoton processes)

32.80.Wr

42.65.Re (Ultrafast processes; optical pulse generation and pulse compression) 32.80.Qk (Coherent control of atomic interactions with photons)

张晖, 张诗按, 孙真荣. Highly selective population of two excited states in nonresonant two-photon absorption[J]. 中国物理B, 2011, 20(8): 83202-083202.

Zhang Hui(张晖), Zhang Shi-An(张诗按), and Sun Zhen-Rong(孙真荣) . Highly selective population of two excited states in nonresonant two-photon absorption[J]. Chin. Phys. B, 2011, 20(8): 83202-083202.

参考文献 26

[1]	Konradi J, Singh A K, Scaria A V and Materny A 2006 J. Raman Spectrosc. 37 697
[2]	Pearson B J, White J L, Weinacht T C and Bucksbaum P H 2001 Phys. Rev. A 63 063412
[3]	Oron D, Dudovich N, Yelin D and Silberberg Y 2002 Phys. Rev. A 65 043408
[4]	Zhang S A, Zhang H, Wang Z G and Sun Z R 2010 Chin. Phys. B 19 043201
[5]	Wollenhaupt M, Pr"akelt A, Sarpe-Tudoran C, Liese D, Bayer T and Baumert T 2006 Phys. Rev. A 73 063409
[6]	Wollenhaupt M, Liese D, Pr"akelt A, Sarpe-Tudoran C and Baumert T 2006 Chem. Phys. Lett. 419 184
[7]	Wollenhaupt M, Pr"akelt A, Sarpe-Tudoran C, Liese D and Bayer T 2005 J. Opt. B 7 S270
[8]	Wollenhaupt M, Engle V and Baumert T 2005 Ann. Rev. Phys. Chem. 56 25
[9]	Krug M, Bayer T, Wollenhaupt M, Sarpe-Tudoran C, Baumert T, Ivanov S S and Vitanov N V 2009 New J. Phys. 11 105051
[10]	Melinger J S, Gandhi Suketu R, Hariharan A, Tull J X and Warren W S 1992 Phys. Rev. Lett. 68 2000
[11]	Zhdanovich S, Shapiro E A, Shapiro M, Hepburn J W and Milner V 2008 Phys. Rev. Lett. 100 103004
[12]	Wollenhaupt M, Pr"akelt A, Sarpe-Tudoran C, Liese D and Baumert T 2006 Appl. Phys. B 82 183
[13]	Balling P, Maas D J and Noordam L D 1994 Phys. Rev. A 50 4276
[14]	Clow S D, Trallero-Herrero C, Bergeman T and Weinacht T 2008 Phys. Rev. Lett. 100 233603
[15]	Chatel B, Degert J, Stock S and Girard B 2003 Phys. Rev. A 68 041402
[16]	Amitay Z, Gandman A, Chuntonov L and Rybak L 2008 Phys. Rev. Lett. 100 193002
[17]	Brixner T, Damrauer N H, Niklaus P and Gerber G 2001 Nature 414 57
[18]	Meshulach D and Silberberg Y 1998 Nature 396 239
[19]	Meshulach D and Silberberg Y 1999 Phys. Rev. A 60 1287
[20]	Dayan B, Peér A, Friesem A A and Silberberg Y 2004 Phys. Rev. Lett. 93 023005
[21]	Lozovoy V V, Pastirk I, Walowicz K A and Dantus M 2003 J. Chem. Phys. 118 3187
[22]	Zhang S A, Wang Z G and Sun Z R 2008 Chin. Phys. B 17 2914
[23]	Ando T, Urakami T, Itoh H and Tsuchiya Y 2002 Appl. Phys. Lett. 80 4265
[24]	Hornung T, Meier R, Zeidler D, Kompa K L, Proch D and Motzkus M 2000 Appl. Phys. B 71 277
[25]	Comstock M, Lozovoy V V, Pastirk I and Dantus M 2004 Opt. Express 12 1061
[26]	Pr"akelt A, Wollenhaupt M, Sarpe-Tudoran C and Baumert T 2004 Phys. Rev. A 70 063407

Highly selective population of two excited states in nonresonant two-photon absorption

Highly selective population of two excited states in nonresonant two-photon absorption

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