How to measure the internuclear vector from photoelectron angular distributions

doi:10.1088/1674-1056/19/2/023202

中国物理B ›› 2010, Vol. 19 ›› Issue (2): 23202-023202.doi: 10.1088/1674-1056/19/2/023202

How to measure the internuclear vector from photoelectron angular distributions

J. T.Wang¹, D. S.Guo¹, 任向河², 张敬涛², 王懿², 徐至展²

(1)Department of Physics, Southern University and A & M College, Baton Rouge, Louisiana 70813 USA; (2)State Key Laboratory for High-Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

收稿日期:2009-04-07 修回日期:2009-05-22 出版日期:2010-02-15 发布日期:2010-02-15
基金资助:
Project supported by the National Natural Science Foundation of China (Grant No.~10774153), the National Basic Research Program of China (Grant No.~2006CD806000), the Shanghai ``Phosphor'' Science Foundation, China (Grant No.~08QH1402400).

How to measure the internuclear vector from photoelectron angular distributions

Ren Xiang-He(任向河)^a), Zhang Jing-Tao(张敬涛)^a)†, Wang Yi(王懿)^a), Xu Zhi-Zhan(徐至展)^a), J.~T. Wang^b), and D.~S. Guo^b)

^a State Key Laboratory for High-Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China; ^b Department of Physics, Southern University and A & M College, Baton Rouge, Louisiana 70813 USA

Received:2009-04-07 Revised:2009-05-22 Online:2010-02-15 Published:2010-02-15
Supported by:
Project supported by the National Natural Science Foundation of China (Grant No.~10774153), the National Basic Research Program of China (Grant No.~2006CD806000), the Shanghai ``Phosphor'' Science Foundation, China (Grant No.~08QH1402400).

摘要/Abstract

摘要： This paper uses a nonperturbative scattering theory to study photoelectron angular distributions of homonuclear diatomic molecules irradiated by circularly polarized laser fields. This study shows that the nonisotropic feature of photoelectron angular distributions is not due to the polarization of the laser field but the internuclear vector of the molecules. It suggests a method to measure the molecular orientation and the internuclear distance of molecules through the measurement of photoelectron angular distributions.

Abstract: This paper uses a nonperturbative scattering theory to study photoelectron angular distributions of homonuclear diatomic molecules irradiated by circularly polarized laser fields. This study shows that the nonisotropic feature of photoelectron angular distributions is not due to the polarization of the laser field but the internuclear vector of the molecules. It suggests a method to measure the molecular orientation and the internuclear distance of molecules through the measurement of photoelectron angular distributions.

Key words: photoelectron angular distributions, internuclear distance, photoionization

中图分类号: (Photoelectron spectra )

33.60.+q

33.80.Eh (Autoionization, photoionization, and photodetachment)

任向河, 张敬涛, 王懿, 徐至展, J. T.Wang, D. S.Guo. How to measure the internuclear vector from photoelectron angular distributions[J]. 中国物理B, 2010, 19(2): 23202-023202.

Ren Xiang-He(任向河), Zhang Jing-Tao(张敬涛), Wang Yi(王懿), Xu Zhi-Zhan(徐至展), J.~T. Wang, and D.~S. Guo. How to measure the internuclear vector from photoelectron angular distributions[J]. Chin. Phys. B, 2010, 19(2): 23202-023202.

参考文献 37

[1]	Agostini P, Fabre F, Mainfray G, Petite G and Rahman N K 1979 Phys. Rev. Lett.42 1127
[2]	Freeman R R, Bucksbaum P H, Milchberg H, Darack S, Schumacher D andGeusic M E 1987 Phys. Rev. Lett. 59 1092
[3]	Zuo T, Bandrauk A D and Corkum P B 1996 Chem. Phys. Lett. 259 313
[4]	Muth-B?hm J, Becker A and Faisal F H M 2000 Phys. Rev. Lett. 85 2280
[5]	Grasbon F, Paulus G G, Chin S L, Walther H, Muth-B?hm J, Becker A andFaisal F H M 2001 Phys. Rev. A 6 3 041402(R)
[6]	Weber T, Czasch A O, Jagutzki O, M?ller A K, Mergel V, Kheifet A,Rotenberg E, Meigs G, Prior M H, Daveau S, Landers A, Cocke C L, Osipov T,D?ez Muiń o R, Schmidt-B?cking H and D?rner R 2004 Nature (London) 431437
[7]	Posthumus J H 2004 Rep. Prog. Phys. 67 623
[8]	Esry B D, Sayler A M, Wang P Q, Carnes K D and Ben-Itzhak I 2006 Phys. Rev. Lett.97 }013003
[9]	Litvinyuk I V, Lee K F, Dooley P W, Rayner D M, Villeneuve D M andCorkum P B 2003 Phys. Rev. Lett. 90 233003
[10]	Torres R, Kajumba N, Underwood J G, Robinson J S, Baker S, Tisch J W G,Nalda R, Bryan W A, Velotta R, Altucci C, Turcu I C E and Marangos J P 2007 Phys. Rev. Lett. 98 203007
[11]	Wu J, Zeng H and Guo C 2006 Phys. Rev. Lett. 96 243002
[12]	Fischer R, Lein M and Keitel C H 2006 Phys. Rev. Lett. 97 143901
[13]	Matos-Abiague A and Berakdar J 2003 Chem. Phys. Lett. 382 475
[14]	Stapelfeldt H and Seideman T 2003 Rev. Mod. Phys. 75543
[15]	Pavicic D, Lee K F, Rayner D M, Corkum P B and Villeneuve D M 2007 Phys. Rev. Lett. 98 243001
[16]	Dundas D and Rost J M 2005 Phys. Rev. A 71 013421
[17]	Faisal F H M, Abdurrouf A, Miyazaki K and Miyaji G 2007 Phys. Rev. Lett. 98 143001
[18]	McKenna J, Suresh M, Srigengan B, Williams I D, Bryan W A, English E ML, Stebbings S L, Newell W R, Turcu I C E, Smith J M, Divall E J, Hooker CJ, Langley A J and Collier J L 2006 Phys. Rev. A 7 3 043401
[19]	Roothaan C C J 1951 Rev. Mod. Phys. 23 69
[19a]	Cohen H D and Fano U 1966 Phys. Rev. 150 30
[20]	Zhang J T, Zhang W Q, Xu Z Z, Li X F, Fu P M, Guo D S and Freeman R R2002 J. Phys. B 35 4809
[21]	Zhang X M, Zhang J T, Gong Q H and Xu Z Z 2009 Chin. Phys. B 18 1014
[22]	Guo D S, Zhang J T, Xu Z Z, Li X F, Fu P M and Freeman R R 2003 Phys. Rev. A 68 043404
[23]	Zhang J T, Bai L H, Gong S Q, Xu Z Z and Guo D S 2007 Opt. Express 15 7261
[24]	Rolles D, Braune M, Cvejanovic S, Gepner O, Hentges R, Korica S, LangerB, Lischke T, Prumper G, Reinkoster A, Viefhaus J, Zimmermann B, McKoy V andBecker U 2005 Nature (London) 437 711
[25]	Milosevic D B 2006 Phys. Rev. A 74 063404
[26]	Kjeldsen T K, Bisgaard C Z, Madsen L B and Stapelfeldt H 2003 Phys. Rev. A 68 063407
[27]	Foster M, Colgan J, Al-Hagan O, Peacher J L, Madison D H and Pindzola MS 2007 Phys. Rev. A 75062707
[28]	Guo D S, Aberg T and Crasemann B 1989 Phys. Rev. A 40 4997
[29]	Bucksbaum P H, Schumacher D W and Bashkansky M 1988 Phys. Rev. Lett. 61 1182
[30]	Guo D S and Drake G W F 1992 Phys. Rev. A 45 6622
[31]	Nandor M J, Walker M A and Woerkom van L D 1998 J. Phys. B 31 4617
[32]	Reichle R, Helm H and Kiyan I Y 2001 Phys. Rev. Lett. 87 243001
[33]	Zhang J T, Woerkom van L D, Guo D S and Freeman R R 2007 Phys. Rev. A 76015401
[34]	Bai L H, Zhang J T and Xu Z Z 2005 Chin. Phys. 141114
[35]	Gao J, Guo D S and Wu Y S 2000 Phys. Rev. A 61 043406
[36]	Ren X H, Zhang J T, Wang Y, Xu Z Z and Guo D S 2009 Eur. Phys. J. D 51 401
[37]	Peek J M 1965 J. Chem. Phys. 4 3 3004

How to measure the internuclear vector from photoelectron angular distributions

How to measure the internuclear vector from photoelectron angular distributions

PDF (PC)

赞

可视化

摘要/Abstract

引用本文

使用本文

参考文献 37

相关文章 14

Metrics

本文评价

推荐阅读 0

[1]	宋乐乐, 孙亚楠, 王艳辉, 王晓春, 赫兰海, 罗嗣佐, 胡文惠, 佟秋男, 丁大军, 刘福春. Photoelectron imaging of resonance-enhanced multiphoton ionization and above-threshold ionization of ammonia molecules in a strong 800-nm laser pulse[J]. 中国物理B, 2019, 28(6): 63201-063201.
[2]	常志强, 李昌明, 郭玮, 姚洪斌. Delay time dependence of wave packet motion and population transfer of four-level K₂ molecule in pump-pump-probe pulses[J]. 中国物理B, 2018, 27(5): 53301-053301.
[3]	张鹏, 冯正鹏, 罗四强, 王哲. Influence of the interaction volume on the kinetic energy resolution of a velocity map imaging spectrometer[J]. 中国物理B, 2016, 25(3): 33202-033202.
[4]	郭玮, 路兴强, 王新林, 姚洪斌. Effect of pump-1 laser on Autler–Townes splitting in photoelectron spectrum of K₂ molecule[J]. 中国物理B, 2015, 24(1): 13302-013302.
[5]	冯立强, 楚天舒, 王利. Low-energy structure in the ionization of argon: Comparison of experiment with theory[J]. 中国物理B, 2013, 22(2): 23302-023302.
[6]	于建宁, 张民艳, 李崇, 尚玉柱, 吕燕芳, 魏斌, 黄维. Fine-tuning the thicknesses of organic layers to realize high-efficiency and long-lifetime blue organic light-emitting diodes[J]. 中国物理B, 2012, 21(8): 83303-083303.
[7]	姚洪斌,郑雨军. [J]. 中国物理B, 2012, 21(2): 23302-023302.
[8]	许洪光, 吴苗苗, 张增光, 孙强, 郑卫军. Structural and bonding properties of ScSi_n^- (n=2～6) clusters: photoelectron spectroscopy and density functional calculations[J]. 中国物理B, 2011, 20(4): 43102-043102.
[9]	刘玉芳, 刘瑞琼, 丁俊霞. Study on wave packet dynamics of E¹∑_g⁺ state of Li₂ with femtosecond-resolved photoelectron spectra[J]. 中国物理B, 2010, 19(3): 33301-033301.
[10]	马晓光, 杨传路, 龚玉兵, 王美山. An alternative view of condensed-phase photoionization[J]. 中国物理B, 2009, 18(12): 5296-5300.
[11]	岳大光, 郑晓云, 刘浩, 王春兴, 孟庆田. Time-dependent theoretical approach to the influence of laser fields on the resonance enhanced multi-photon ionization of SH radical[J]. 中国物理B, 2009, 18(4): 1479-1485.
[12]	张永风, 王美山, 杨传路, 马美仲, 庞伟秀, 马荣彩. Ab initio calculations of the ionization spectrum of SO₂[J]. 中国物理B, 2008, 17(11): 4163-4169.
[13]	闫冰, 潘守甫, 郭庆群. Spin--orbit ab initio curves of ⁸⁰Se₂⁺ ion and theassignment of photoelectron spectra of ⁸⁰Se₂ molecule[J]. 中国物理B, 2008, 17(9): 3318-3321.
[14]	陈桂英, 袁义哲, 梁心, 许棠, 张春平, 宋期望. The behaviours of optical novelty filter based on bacteriorhodopsin film[J]. 中国物理B, 2006, 15(9): 2007-2011.