Shock temperature and reflectivity of precompressed H2O up to 350 GPa:Approaching the interior of planets

doi:10.1088/1674-1056/27/12/126202

Abstract

Using a combination of static precompression and laser-driven shock compression, shock temperature and reflectivity of H₂O have been measured up to 350 GPa and 2.1×10⁴ K. Here, two calibration standards were applied to enhance temperature measurement reliability. Additionally, in temperature calculations, the discrepancy in reflectivity between active probe beam wavelength and self-emission wavelength has been taken into account to improve the data's precision. Precompressed water's temperature-pressure data are in very good agreement with our quantum molecular dynamics model, suggesting a superionic conductor of H₂O in the icy planets' deep interior. A sluggish slope gradually approaching Dulong-Petit limit at high temperature was found at a specific heat capacity. Also, high reflectivity and conductivity were observed at the same state. By analyzing the temperature-pressure diagram, reflectivity, conductivity and specific heat comprehensively at conditions simulating the interior of planets in this work, we found that as the pressure rises, a change in ionization appears; it is supposedly attributed to energetics of bond-breaking in the H₂O as it transforms from a bonded molecular fluid to an ionic state. Such molecular dissociation in H₂O is associated with the conducting transition because the dissociated hydrogen atoms contribute to electrical properties.

Keywords: high temperature measurement equation of state of water laser-driven shock diamond anvil cell

Received: 23 July 2018
Revised: 20 September 2018
Accepted manuscript online:

PACS:	62.50.-p	(High-pressure effects in solids and liquids)
	51.30.+i	(Thermodynamic properties, equations of state)
	64.30.-t	(Equations of state of specific substances)
	52.25.Kn	(Thermodynamics of plasmas)

Fund:

Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0403200) and the Science Challenge Project (Grant No. TZ2016001).

Corresponding Authors: Fan Zhang
E-mail: innocentman001@163.com

Cite this article:

Zhi-Yu He(贺芝宇), Hua Shu(舒桦), Xiu-Guang Huang(黄秀光), Qi-Li Zhang(张其黎), Guo Jia(贾果), Fan Zhang(张帆), Yu-Chun Tu(涂昱淳), Jun-Yue Wang(王寯越), Jun-Jian Ye(叶君建), Zhi-Yong Xie(谢志勇), Zhi-Heng Fang(方智恒), Wen-Bing Pei(裴文兵), Si-Zu Fu(傅思祖) Shock temperature and reflectivity of precompressed H₂O up to 350 GPa:Approaching the interior of planets 2018 Chin. Phys. B 27 126202

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Shock temperature and reflectivity of precompressed H2O up to 350 GPa:Approaching the interior of planets

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Shock temperature and reflectivity of precompressed H₂O up to 350 GPa:Approaching the interior of planets