Preparation and the physical properties of antiperovskite-type compounds Cd1-xInxNNi3 (0≤x≤0.2) and Cd1-yCuyNNi3 (0≤y≤0.2)

doi:10.1088/1674-1056/21/4/047401

Abstract Two series of Cd_1-xIn_xNNi₃ (0≤x≤0.2) and Cd_1-yCu_yNNi₃ (0≤y≤0.2) samples were prepared from CdO, In₂O₃, CuO, and nickel powders under NH₃ atmosphere at 773 K. The structural and physical properties were investigated by means of X-ray powder diffraction temperature-dependent resistivity and magnetic measurements. X-ray powder diffraction results showed that the Cd_1-xIn_xNNi₃ and Cd_1-yCu_yNNi₃ compounds have a typical antiperovskite structure, and the CdNNi₃, Cd_0.9In_0.1NNi₃, and Cd_0.9Cu_0.1NNi₃ compounds show metallic temperature-dependent resistivity and exhibit a Fermi liquid behavior at low temperature. In contrast to the paramagnetism previously reported, the CdNNi₃ sample exhibits very soft and weak ferromagnetism, and no superconductivity was found in the Cd_1-xIn_xNNi₃ and Cd_1-yCu_yNNi₃ samples down to 2 K. Each sample exhibited very soft and weak ferromagnetism, and the temperature dependence of the magnetization of the Cd_1-xIn_xNNi₃ and Cd_1-yCu_yNNi₃ samples can be well fitted to the combination of a Bloch term and a Curie-Weiss term.

Keywords: nitride antiperovskite weak ferromagnetism Fermi liquid

Received: 27 November 2011
Revised: 06 January 2012
Accepted manuscript online:

PACS:	74.70.Dd	(Ternary, quaternary, and multinary compounds)
	75.50.Gg	(Ferrimagnetics)

Fund: Project supported by the National Natural Science Foundation of China (Grant No. 20871119), the National Basic Research Program of China (973 Program) (Grant Nos. 2011CBA00112 and 2011CB808202), and the Natural Science Foundation of Luzhou Medical College.

Corresponding Authors: He Bing,hebing@ssc.iphy.ac.cn
E-mail: hebing@ssc.iphy.ac.cn

Cite this article:

He Bing(贺兵), Dong Cheng(董成), Yang Li-Hong(杨立红), Ge Lin-Hui(葛林慧), Mu Li-Bin(慕利斌), Chen Xiao-Chao(陈晓超) Preparation and the physical properties of antiperovskite-type compounds Cd_1-xIn_xNNi₃ (0≤x≤0.2) and Cd_1-yCu_yNNi₃ (0≤y≤0.2) 2012 Chin. Phys. B 21 047401

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Preparation and the physical properties of antiperovskite-type compounds Cd1-xInxNNi3 (0≤x≤0.2) and Cd1-yCuyNNi3 (0≤y≤0.2)

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Preparation and the physical properties of antiperovskite-type compounds Cd_1-xIn_xNNi₃ (0≤x≤0.2) and Cd_1-yCu_yNNi₃ (0≤y≤0.2)