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Chinese Physics, 2004, Vol. 13(7): 1129-1133    DOI: 10.1088/1009-1963/13/7/029
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Prev   Next  

Magnetism and magnetoresistance of Er1-xSmxMn6Ge6(x=0.2-1.0) compounds

Wang Ru-Wu (汪汝武)ab, Zhang Shao-Ying (张绍英)b, Zhang Li-Gang (张立刚)a, Yao Jin-Lei (姚金雷)bc, Li Yun-Bao (李云宝)a, Shen Bao-Gen (沈保根)b 
a Department of Applied Physics, University of Science and Technology of Wuhan, Wuhan 430081, China; b State Key Laboratory of Magnetism, Institute of Physics and Centre for Condensed Matter Physics, Chinese Academy of Sciences, Beijing 100080, China; c State Key Laboratory of Silicon Materials, Zhejiang University, Hangzhou 310027, China
Abstract  Magnetic and transport properties of Er$_{1-x}$Sm$_x$Mn$_6$Ge$_6$($x$=0.2-1.0) have been investigated by x-ray diffraction (XRD) and magnetization measurement. Analysis of the XRD patterns indicates that the samples with x≤0.4 mainly consist of HfFe$_6$Ge$_6$-type phase and the samples with 0.6≤x≤1.0 mainly consist of YCo$_6$Ge$_6$-type phase (P6/mmm). The lattice constants and the unit cell volume increase with increasing Sm content. The antiferro-ferri-ferromagnetic transitions can be observed with increasing Sm content. The samples with x=0.2 and 0.4 order antiferromagnetically at 420 and 425K, respectively. The samples with x=0.6, 0.8 and 1.0 order from ferri- to ferromagnetically over the whole magnetic ordering temperature range. The corresponding Curie temperatures are 435, 441 and 446K, respectively. The magnetoresistance (MR) isotherms of the sample with x=0.8, measured at various temperatures, are analysed. The magnitude of MR is found to be positive below 55K and gradually increases to a relatively large value of about 5.02% at 5K in a field of 5T as the temperature is lowered. A possible explanation for the positive MR is given.
Keywords:  magnetism      positive magnetoresistance  
Received:  13 November 2003      Revised:  12 December 2003      Accepted manuscript online: 
PACS:  75.60.Ej (Magnetization curves, hysteresis, Barkhausen and related effects)  
  75.47.Np (Metals and alloys)  
  75.30.Kz (Magnetic phase boundaries (including classical and quantum magnetic transitions, metamagnetism, etc.))  
  75.40.Cx (Static properties (order parameter, static susceptibility, heat capacities, critical exponents, etc.))  
  61.66.Dk (Alloys )  
Fund: Project supported by the National Natural Science Foundation of China (Grant No 50071041), and the State Key Development Programme for Basic Research of China (Grant No G1998061303).

Cite this article: 

Wang Ru-Wu (汪汝武), Zhang Shao-Ying (张绍英), Zhang Li-Gang (张立刚), Yao Jin-Lei (姚金雷), Li Yun-Bao (李云宝), Shen Bao-Gen (沈保根) Magnetism and magnetoresistance of Er1-xSmxMn6Ge6(x=0.2-1.0) compounds 2004 Chinese Physics 13 1129

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