Investigation of fluorescence resonance energy transfer ultrafast dynamics in electrostatically repulsed and attracted exciton-plasmon systems

doi:10.1088/1674-1056/abb802

Abstract Following the gradual maturation of synthetic techniques for nanomaterials, exciton-plasmon composites have become a research hot-spot due to their controllable energy transfer through electromagnetic fields on the nanoscale. However, most reports ignore fluorescence resonance energy transfer (FRET) under electrostatic repulsion conditions. In this study, the FRET process is investigated in both electrostatic attraction and electrostatic repulsion systems. By changing the Au:quantum dot ratio, local-field induced FRET can be observed with a lifetime of ns and a fast component of hundreds of ps. These results indicate that the intrinsic transfer process can only elucidated by considering both steady and transient state information.

Keywords: fluorescence resonance energy transfer (FRET) quantum dots excitons-plasmon composites

Received: 06 August 2020
Revised: 02 September 2020
Accepted manuscript online: 14 September 2020

PACS:	78.67.Hc	(Quantum dots)
	33.20.-t	(Molecular spectra)

Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 10904049 and 61575079), the Science and Technology Development Program of Jilin Province, China (Grant No. 20180101230JC), the Fundamental Research Funds for the Central Universities (Grant No. JCKYQKJC45), China Postdoctoral Science Foundation (Grant No. 201003537), and the Scientific Research Foundation for the Returned Overseas Chinese Scholars, the Ministry of Education, China.

Corresponding Authors: ^†Corresponding author. E-mail: ply@jlu.edu.cn

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Hong-Yu Tu(屠宏宇), Ji-Chao Cheng(程基超), Gen-Cai Pan(潘根才), Lu Han(韩露), Bin Duan(段彬), Hai-Yu Wang(王海宇), Qi-Dai Chen(陈岐岱), Shu-Ping Xu(徐抒平), Zhen-Wen Dai(戴振文), and Ling-Yun Pan(潘凌云) Investigation of fluorescence resonance energy transfer ultrafast dynamics in electrostatically repulsed and attracted exciton-plasmon systems 2021 Chin. Phys. B 30 027802

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Investigation of fluorescence resonance energy transfer ultrafast dynamics in electrostatically repulsed and attracted exciton-plasmon systems

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