Control of the photoionization/photodissociation processes of cyclopentanone with trains of femtosecond laser pulses

doi:10.1088/1674-1056/22/10/103301

Abstract A train of three equally spaced femtosecond laser pulses is employed to control the photoionization/photodissociation processes of cyclopentanone. With the increase of pulse separation, a strong modulation of product ion yield is observed. More than ten-fold changes of ion yield ratio between different products can be realized. The experimental observations further explain the compositions and formation pathways of peaks in the mass spectra. The controlling mechanisms are also discussed.

Keywords: shaped femtosecond pulse coherent control time-of-flight mass spectra photoionization and photodissociation

Received: 03 February 2013
Revised: 03 April 2013
Accepted manuscript online:

PACS:

33.80.R

Fund: Project supported by the National Basic Research Program of China (973 Program) (Grant No. 2013CB922200), the National Natural Science Foundation of China, (Grant Nos. 10774056 and 10974070), the Fundamental Research Funds for the Central Universities, China (Grant No. 200903371), and the Specialized Research Fund for the Doctoral Program of Higher Education, China (Grant No. 20100061110045).

Corresponding Authors: Hu Zhan
E-mail: huzhan@jlu.edu.cn

Cite this article:

Song Yao-Dong (宋耀东), Chen Zhou (陈洲), Yang Xue (杨雪), Sun Chang-Kai (孙长凯), Zhang Cong-Cong (张丛丛), Hu Zhan (胡湛) Control of the photoionization/photodissociation processes of cyclopentanone with trains of femtosecond laser pulses 2013 Chin. Phys. B 22 103301

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Control of the photoionization/photodissociation processes of cyclopentanone with trains of femtosecond laser pulses

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