Efficiently enhanced energy storage performance of Ba2Bi4Ti5O18 film by co-doping Fe3+ and Ta5+ ion with larger radius

doi:10.1088/1674-1056/ac5393

Abstract We present an efficient strategy, that is the co-substitution of Fe³⁺ and Ta⁵⁺ ions with large radius for Ti⁴⁺ ion, to enhance energy storage performance of Ba₂Bi₄Ti₅O₁₈ film. For the films co-doped with Fe³⁺ and Ta⁵⁺ ions, the maximum polarization under the same external electric field is improved because the radius of Fe³⁺ and Ta⁵⁺ ions is larger than that of Ti⁴⁺ ion. Moreover, due to the composition and chemical disorder, the relaxor properties are also slightly improved, which can not be achieved by the film doped with Fe³⁺ ions only. What is more, for the films doped with Fe³⁺ ion only, the leakage current density increases greatly due to the charge imbalance, resulting in a significant decrease in breakdown strength. It is worth mentioning that the breakdown strength of Fe³⁺ and Ta⁵⁺ ions co-doped film does not decrease due to the charge balance. Another important point is the recoverable energy storage density of the films co-doped with Fe³⁺ and Ta⁵⁺ ions has been greatly improved based on the fact that the maximum external electric field does not decrease and the maximum polarization under the same external electric field increases. On top of that, the hysteresis of the polarization has also been improved. Finally, the co-doped films with Fe³⁺ and Ta⁵⁺ ions have good frequency and temperature stability.

Keywords: Ba₂Bi₄Ti₅O₁₈ film ferroelectrics energy storage co-doped radius

Received: 26 November 2021
Revised: 17 January 2022
Accepted manuscript online: 10 February 2022

PACS:	77.80.-e	(Ferroelectricity and antiferroelectricity)
	68.55.-a	(Thin film structure and morphology)
	84.60.Ve	(Energy storage systems, including capacitor banks)

Fund: This work was financially supported by the National Natural Science Foundation of China (Grant Nos. 12074204, 11864028, and 11904054) and the Natural Science Foundation of Inner Mongolia, China (Grant No. 2022ZD06).

Corresponding Authors: Shifeng Zhao
E-mail: zhsf@imu.edu.cn

Cite this article:

Qiong Wu(吴琼), Lei Zhao(赵雷), Xinghao Chen(陈兴豪), and Shifeng Zhao(赵世峰)^† Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius 2022 Chin. Phys. B 31 097701

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Efficiently enhanced energy storage performance of Ba2Bi4Ti5O18 film by co-doping Fe3+ and Ta5+ ion with larger radius

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Efficiently enhanced energy storage performance of Ba₂Bi₄Ti₅O₁₈ film by co-doping Fe³⁺ and Ta⁵⁺ ion with larger radius