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Abstract Physical models of ion diffusion at different interfaces are reviewed. The use of impedance spectroscopy (IS), nuclear magnetic resonance (NMR), and secondary ion mass spectrometry (SIMS) techniques are also discussed. The diffusion of ions is fundamental to the operation of lithium-ion batteries, taking place not only within the grains but also across different interfaces. Interfacial ion transport usually contributes to the majority of the resistance in lithium-ion batteries. A greater understanding of the interfacial diffusion of ions is crucial to improving battery performance.
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Received: 03 June 2015
Revised: 11 August 2015
Accepted manuscript online:
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PACS:
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82.45.Gj
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(Electrolytes)
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66.30.H-
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(Self-diffusion and ionic conduction in nonmetals)
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| Fund: Project supported by the Beijing S&T Project, China (Grant No. Z13111000340000), the National Natural Science Foundation of China (Grant Nos. 51325206 and 11234013) and the National Basic Research Program of China (Grant No. 2012CB932900). |
Corresponding Authors:
Shaofei Wang
E-mail: wsfwsry@163.com
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Cite this article:
Shaofei Wang(王少飞) and Liquan Chen(陈立泉) Interfacial transport in lithium-ion conductors 2016 Chin. Phys. B 25 018202
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