中国物理B ›› 2018, Vol. 27 ›› Issue (2): 24206-024206.doi: 10.1088/1674-1056/27/2/024206

• ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS • 上一篇    下一篇

Spectral redshift of high-order harmonics by adding a weak pulse in the falling part of the trapezoidal laser pulse

Xue-Fei Pan(潘雪飞), Jun Zhang(张军), Shuai Ben(贲帅), Tong-Tong Xu(徐彤彤), Xue-Shen Liu(刘学深)   

  1. Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China
  • 收稿日期:2017-09-17 修回日期:2017-10-13 出版日期:2018-02-05 发布日期:2018-02-05
  • 通讯作者: Xue-Shen Liu E-mail:liuxs@jlu.edu.cn
  • 基金资助:

    Project supported by the National Natural Science Foundation of China (Grant No. 61575077) and the Graduate Innovation Fund of Jilin University (Grant No. 2017107).

Spectral redshift of high-order harmonics by adding a weak pulse in the falling part of the trapezoidal laser pulse

Xue-Fei Pan(潘雪飞), Jun Zhang(张军), Shuai Ben(贲帅), Tong-Tong Xu(徐彤彤), Xue-Shen Liu(刘学深)   

  1. Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China
  • Received:2017-09-17 Revised:2017-10-13 Online:2018-02-05 Published:2018-02-05
  • Contact: Xue-Shen Liu E-mail:liuxs@jlu.edu.cn
  • About author:42.65.Ky; 32.80.Rm; 78.67.Bf
  • Supported by:

    Project supported by the National Natural Science Foundation of China (Grant No. 61575077) and the Graduate Innovation Fund of Jilin University (Grant No. 2017107).

摘要:

We investigate the spectral redshift of high-order harmonics of the H2+ (D2+) molecule by numerically solving the non-Born-Oppenheimer time-dependent Schrödinger equation (TDSE). The results show that the spectral redshift of high-order harmonics can be observed by adding a weak pulse in the falling part of the trapezoidal laser pulses. Comparing with the H2+ molecule, the shift of high-order harmonic generation (HHG) spectrum for the D2+ molecule is more obvious. We employ the spatial distribution in HHG and time-frequency analysis to illustrate the physical mechanism of the spectral redshift of high-order harmonics.

关键词: high-order harmonic generation, spectral redshift, trapezoidal laser pulse, spatial distribution

Abstract:

We investigate the spectral redshift of high-order harmonics of the H2+ (D2+) molecule by numerically solving the non-Born-Oppenheimer time-dependent Schrödinger equation (TDSE). The results show that the spectral redshift of high-order harmonics can be observed by adding a weak pulse in the falling part of the trapezoidal laser pulses. Comparing with the H2+ molecule, the shift of high-order harmonic generation (HHG) spectrum for the D2+ molecule is more obvious. We employ the spatial distribution in HHG and time-frequency analysis to illustrate the physical mechanism of the spectral redshift of high-order harmonics.

Key words: high-order harmonic generation, spectral redshift, trapezoidal laser pulse, spatial distribution

中图分类号:  (Frequency conversion; harmonic generation, including higher-order harmonic generation)

  • 42.65.Ky
32.80.Rm (Multiphoton ionization and excitation to highly excited states) 78.67.Bf (Nanocrystals, nanoparticles, and nanoclusters)