Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH3NH3PbI3-xClx prepared onZnO/FTO substrates using a two-step method

doi:10.1088/1674-1056/26/1/017802

中国物理B ›› 2017, Vol. 26 ›› Issue (1): 17802-017802.doi: 10.1088/1674-1056/26/1/017802

• CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES • 上一篇下一篇

Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method

Shiwei Zhuang(庄仕伟), Deqian Xu(徐德前), Jiaxin Xu(徐佳新), Bin Wu(伍斌), Yuantao Zhang(张源涛), Xin Dong(董鑫), Guoxing Li(李国兴), Baolin Zhang(张宝林), Guotong Du(杜国同)

State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, Changchun 130012, China

收稿日期:2016-08-27 修回日期:2016-10-13 出版日期:2017-01-05 发布日期:2017-01-05
通讯作者: Baolin Zhang E-mail:zbl@jlu.edu.cn
基金资助:
Project supported by the International Science and Technology Cooperation Program of Science and Technology Bureau of Changchun City, China (Grant No. 12ZX68).

Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method

Shiwei Zhuang(庄仕伟), Deqian Xu(徐德前), Jiaxin Xu(徐佳新), Bin Wu(伍斌), Yuantao Zhang(张源涛), Xin Dong(董鑫), Guoxing Li(李国兴), Baolin Zhang(张宝林), Guotong Du(杜国同)

State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, Changchun 130012, China

Received:2016-08-27 Revised:2016-10-13 Online:2017-01-05 Published:2017-01-05
Contact: Baolin Zhang E-mail:zbl@jlu.edu.cn
Supported by:
Project supported by the International Science and Technology Cooperation Program of Science and Technology Bureau of Changchun City, China (Grant No. 12ZX68).

摘要/Abstract

摘要： Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH₃NH₃PbI_3-xCl_x films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and absorption characteristics of the films were also studied. Scanning electron microscopy revealed large crystals and substrate coverage. The orthorhombic-to-tetragonal phase transition temperature was ~140 K. The films' exciton binding energy was 77.6±10.9 meV and the energy of optical phonons was 38.8±2.5 meV. These results suggest that perovskite CH₃NH₃PbI_3-xCl_x films have excellent optoelectronic characteristics which further suggests their potential usage in perovskitebased optoelectronic devices.

关键词: perovskite, temperature-dependent photoluminescence, two-step method, ZnO

Abstract: Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH₃NH₃PbI_3-xCl_x films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and absorption characteristics of the films were also studied. Scanning electron microscopy revealed large crystals and substrate coverage. The orthorhombic-to-tetragonal phase transition temperature was ~140 K. The films' exciton binding energy was 77.6±10.9 meV and the energy of optical phonons was 38.8±2.5 meV. These results suggest that perovskite CH₃NH₃PbI_3-xCl_x films have excellent optoelectronic characteristics which further suggests their potential usage in perovskitebased optoelectronic devices.

Key words: perovskite, temperature-dependent photoluminescence, two-step method, ZnO

中图分类号:

78.20.-e 78.55.-m

庄仕伟, 徐德前, 徐佳新, 伍斌, 张源涛, 董鑫, 李国兴, 张宝林, 杜国同. Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method[J]. 中国物理B, 2017, 26(1): 17802-017802.

Shiwei Zhuang(庄仕伟), Deqian Xu(徐德前), Jiaxin Xu(徐佳新), Bin Wu(伍斌), Yuantao Zhang(张源涛), Xin Dong(董鑫), Guoxing Li(李国兴), Baolin Zhang(张宝林), Guotong Du(杜国同). Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method[J]. Chin. Phys. B, 2017, 26(1): 17802-017802.

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Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method

Temperature-dependent photoluminescence on organic-inorganicmetal halide perovskite CH₃NH₃PbI_3-xCl_x prepared onZnO/FTO substrates using a two-step method

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